Articles | Volume 15, issue 7
https://doi.org/10.5194/acp-15-3687-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue:
https://doi.org/10.5194/acp-15-3687-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
02 Apr 2015
Research article |
| 02 Apr 2015
Submicron particle mass concentrations and sources in the Amazonian wet season (AMAZE-08)
School of Engineering and Applied Sciences & Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
now at: State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing, China
D. K. Farmer
Department of Chemistry and Biochemistry & Cooperative Institute for Research in Environmental Science, University of Colorado, Boulder, CO, USA
now at: Department of Chemistry, Colorado State University, Fort Collins, CO, USA
L. V. Rizzo
Department of Natural and Earth Sciences, Federal University of São Paulo, Diadema, Brazil
T. Pauliquevis
Department of Natural and Earth Sciences, Federal University of São Paulo, Diadema, Brazil
M. Kuwata
School of Engineering and Applied Sciences & Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
now at: Earth Observatory of Singapore, Nanyang Technological University, Singapore
T. G. Karl
National Center for Atmospheric Research, Boulder, CO, USA
now at: Institute of Meteorology and Geophysics, University of Innsbruck, Austria
A. Guenther
National Center for Atmospheric Research, Boulder, CO, USA
now at: Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USA
J. D. Allan
National Centre for Atmospheric Science & School of Earth, Atmospheric and Environmental Sciences, University of Manchester, Manchester, UK
National Centre for Atmospheric Science & School of Earth, Atmospheric and Environmental Sciences, University of Manchester, Manchester, UK
M. O. Andreae
Biogeochemistry and Multiphase Chemistry Departments, Max Planck Institute for Chemistry, Mainz, Germany
U. Pöschl
Biogeochemistry and Multiphase Chemistry Departments, Max Planck Institute for Chemistry, Mainz, Germany
J. L. Jimenez
Department of Chemistry and Biochemistry & Cooperative Institute for Research in Environmental Science, University of Colorado, Boulder, CO, USA
Applied Physics Department & Atmospheric Science Department, University of São Paulo, São Paulo, Brazil
S. T. Martin
CORRESPONDING AUTHOR
School of Engineering and Applied Sciences & Department of Earth and Planetary Sciences, Harvard University, Cambridge, MA, USA
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- Modeling the Size Distribution and Chemical Composition of Secondary Organic Aerosols during the Reactive Uptake of Isoprene-Derived Epoxydiols under Low-Humidity Condition M. Octaviani et al. 10.1021/acsearthspacechem.1c00303
- Sub-micrometre particulate matter is primarily in liquid form over Amazon rainforest A. Bateman et al. 10.1038/ngeo2599
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- Mixing order of sulfate aerosols and isoprene epoxydiols affects secondary organic aerosol formation in chamber experiments T. Nah et al. 10.1016/j.atmosenv.2019.116953
- Strong anthropogenic control of secondary organic aerosol formation from isoprene in Beijing D. Bryant et al. 10.5194/acp-20-7531-2020
- Modeling Volatility-Based Aerosol Phase State Predictions in the Amazon Rainforest Q. Rasool et al. 10.1021/acsearthspacechem.1c00255
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- Assessing the Potential Mechanisms of Isomerization Reactions of Isoprene Epoxydiols on Secondary Organic Aerosol A. Watanabe et al. 10.1021/acs.est.8b01780
- Properties and Atmospheric Oxidation of Norpinic Acid Aerosol E. Kostenidou et al. 10.3390/atmos13091481
- Lability of secondary organic particulate matter P. Liu et al. 10.1073/pnas.1603138113
- Observations of sesquiterpenes and their oxidation products in central Amazonia during the wet and dry seasons L. Yee et al. 10.5194/acp-18-10433-2018
- Anthropogenic influences on the physical state of submicron particulate matter over a tropical forest A. Bateman et al. 10.5194/acp-17-1759-2017
- Chemical Characterization of Water-Soluble Organic Aerosol in Contrasting Rural and Urban Environments in the Southeastern United States L. Xu et al. 10.1021/acs.est.6b05002
- Organosulfates in aerosols downwind of an urban region in central Amazon M. Glasius et al. 10.1039/C8EM00413G
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- Observations of Manaus urban plume evolution and interaction with biogenic emissions in GoAmazon 2014/5 G. Cirino et al. 10.1016/j.atmosenv.2018.08.031
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- Exploration of oxidative chemistry and secondary organic aerosol formation in the Amazon during the wet season: explicit modeling of the Manaus urban plume with GECKO-A C. Mouchel-Vallon et al. 10.5194/acp-20-5995-2020
- Insights into the formation and properties of secondary organic aerosol at a background site in Yangtze River Delta region of China: Aqueous-phase processing vs. photochemical oxidation D. Huang et al. 10.1016/j.atmosenv.2020.117716
- Relative humidity-dependent viscosities of isoprene-derived secondary organic material and atmospheric implications for isoprene-dominant forests M. Song et al. 10.5194/acp-15-5145-2015
- Seasonal characterization of submicron aerosol chemical composition and organic aerosol sources in the southeastern United States: Atlanta, Georgia,and Look Rock, Tennessee S. Budisulistiorini et al. 10.5194/acp-16-5171-2016
- Mesoscale variations of the chemical composition of submicron aerosols and its influence on the cloud condensation nuclei activation T. Ajith et al. 10.1016/j.atmosenv.2021.118778
- Aircraft-based observations of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX-SOA) in the tropical upper troposphere over the Amazon region C. Schulz et al. 10.5194/acp-18-14979-2018
- Secondary Formation of Submicron and Supermicron Organic and Inorganic Aerosols in a Highly Polluted Urban Area Y. Zheng et al. 10.1029/2022JD037865
- Urban influence on the concentration and composition of submicron particulate matter in central Amazonia S. de Sá et al. 10.5194/acp-18-12185-2018
- Examining the effects of anthropogenic emissions on isoprene-derived secondary organic aerosol formation during the 2013 Southern Oxidant and Aerosol Study (SOAS) at the Look Rock, Tennessee ground site S. Budisulistiorini et al. 10.5194/acp-15-8871-2015
- Introduction: Observations and Modeling of the Green Ocean Amazon (GoAmazon2014/5) S. Martin et al. 10.5194/acp-16-4785-2016
- Chemical Characterization of Secondary Organic Aerosol from Oxidation of Isoprene Hydroxyhydroperoxides M. Riva et al. 10.1021/acs.est.6b02511
- Observational evidence reveals the significance of nocturnal chemistry in seasonal secondary organic aerosol formation L. Liu et al. 10.1038/s41612-024-00747-6
- Enhanced formation of isoprene‐derived organic aerosol in sulfur‐rich power plant plumes during Southeast Nexus L. Xu et al. 10.1002/2016JD025156
- Regional Similarities and NOx‐Related Increases in Biogenic Secondary Organic Aerosol in Summertime Southeastern United States J. Liu et al. 10.1029/2018JD028491
- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Limited formation of isoprene epoxydiols‐derived secondary organic aerosol under NOx‐rich environments in Eastern China Y. Zhang et al. 10.1002/2016GL072368
- Ambient Gas-Particle Partitioning of Tracers for Biogenic Oxidation G. Isaacman-VanWertz et al. 10.1021/acs.est.6b01674
- Aircraft observations of the chemical composition and aging of aerosol in the Manaus urban plume during GoAmazon 2014/5 J. Shilling et al. 10.5194/acp-18-10773-2018
- A review of stereochemical implications in the generation of secondary organic aerosol from isoprene oxidation J. Cash et al. 10.1039/C6EM00354K
- Characterization of a real-time tracer for isoprene epoxydiols-derived secondary organic aerosol (IEPOX-SOA) from aerosol mass spectrometer measurements W. Hu et al. 10.5194/acp-15-11807-2015
- Effects of Aqueous-Phase and Photochemical Processing on Secondary Organic Aerosol Formation and Evolution in Beijing, China W. Xu et al. 10.1021/acs.est.6b04498
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Short summary
Submicron particle mass concentration in the Amazon during the wet season of 2008 was dominated by organic material. The PMF analysis finds a comparable importance of gas-phase (gas-to-particle condensation) and particle-phase (reactive uptake of isoprene oxidation products, especially of epoxydiols to acidic haze, fog, or cloud droplets) production of secondary organic material during the study period, together accounting for >70% of the organic-particle mass concentration.
Submicron particle mass concentration in the Amazon during the wet season of 2008 was dominated...
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