Articles | Volume 15, issue 6
https://doi.org/10.5194/acp-15-3063-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-3063-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
18 Mar 2015
Research article |
| 18 Mar 2015
Effect of oxidant concentration, exposure time, and seed particles on secondary organic aerosol chemical composition and yield
Aerodyne Research Inc., Billerica, MA, USA
Chemistry Department, Boston College, Chestnut Hill, MA, USA
P. S. Chhabra
Aerodyne Research Inc., Billerica, MA, USA
now at: Department of Chemical Engineering, University of Texas, Austin, Texas, USA
T. B. Onasch
Aerodyne Research Inc., Billerica, MA, USA
Chemistry Department, Boston College, Chestnut Hill, MA, USA
W. H. Brune
Department of Meteorology and Atmospheric Sciences, Pennsylvania State University, State College, PA, USA
J. F. Hunter
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
J. H. Kroll
Department of Civil and Environmental Engineering, Massachusetts Institute of Technology, Cambridge, MA, USA
M. J. Cummings
Chemistry Department, Boston College, Chestnut Hill, MA, USA
J. F. Brogan
Chemistry Department, Boston College, Chestnut Hill, MA, USA
Y. Parmar
Chemistry Department, Boston College, Chestnut Hill, MA, USA
D. R. Worsnop
Aerodyne Research Inc., Billerica, MA, USA
C. E. Kolb
Aerodyne Research Inc., Billerica, MA, USA
P. Davidovits
Chemistry Department, Boston College, Chestnut Hill, MA, USA
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Short summary
We compared the chemistry and yields of SOA generated from OH oxidation of gas-phase precursors in a flow reactor (high OH, short residence time) and environmental chambers (low OH, long residence time). We find that chemical composition of SOA produced in the flow reactor and in chambers is similar. SOA yields measured in the flow reactor are lower than in chambers. Seed particles increase the yield of SOA produced in the flow reactor and may account in part for higher SOA yields in chambers.
We compared the chemistry and yields of SOA generated from OH oxidation of gas-phase precursors...
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