Articles | Volume 15, issue 6
https://doi.org/10.5194/acp-15-2953-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-2953-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Gaseous products and secondary organic aerosol formation during long term oxidation of isoprene and methacrolein
L. Brégonzio-Rozier
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
F. Siekmann
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331, Marseille, France
C. Giorio
Department of Chemistry, University of Cambridge, Cambridge CB2 1EW, UK
Dipartimento di Scienze Chimiche, Università degli Studi di Padova, Padova, 35131, Italy
E. Pangui
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
S. B. Morales
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
B. Temime-Roussel
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331, Marseille, France
A. Gratien
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
V. Michoud
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
S. Ravier
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331, Marseille, France
M. Cazaunau
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
A. Tapparo
Dipartimento di Scienze Chimiche, Università degli Studi di Padova, Padova, 35131, Italy
A. Monod
Aix-Marseille Université, CNRS, LCE FRE 3416, 13331, Marseille, France
J.-F. Doussin
Laboratoire Interuniversitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS, Université Paris-Est-Créteil (UPEC) et Université Paris Diderot (UPD), Institut Pierre Simon Laplace (IPSL), Créteil, France
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- Secondary organic aerosol formation from isoprene photooxidation during cloud condensation–evaporation cycles L. Brégonzio-Rozier et al. 10.5194/acp-16-1747-2016
- Aqueous-phase oligomerization of methyl vinyl ketone through photooxidation – Part 1: Aging processes of oligomers P. Renard et al. 10.5194/acp-15-21-2015
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34 citations as recorded by crossref.
- Investigation of the formation of benzoyl peroxide, benzoic anhydride, and other potential aerosol products from gas–phase reactions of benzoylperoxy radicals C. Strollo & P. Ziemann 10.1016/j.atmosenv.2016.01.011
- Secondary organic aerosol yields from the oxidation of benzyl alcohol S. Charan et al. 10.5194/acp-20-13167-2020
- Effect of oxidant concentration, exposure time, and seed particles on secondary organic aerosol chemical composition and yield A. Lambe et al. 10.5194/acp-15-3063-2015
- Secondary organic aerosol from VOC mixtures in an oxidation flow reactor E. Ahlberg et al. 10.1016/j.atmosenv.2017.05.005
- The production of formaldehyde and hydroxyacetone in methacrolein photooxidation: New insights into mechanism and effects of water vapor Y. Xing et al. 10.1016/j.jes.2017.05.037
- Aqueous-phase oligomerization of methyl vinyl ketone through photooxidation – Part 2: Development of the chemical mechanism and atmospheric implications B. Ervens et al. 10.5194/acp-15-9109-2015
- Aqueous-Phase Oxidation of cis-β-Isoprene Epoxydiol by Hydroxyl Radicals and Its Impact on Atmospheric Isoprene Processing T. Otto et al. 10.1021/acs.jpca.9b08836
- Homologous series of low molecular weight (C1-C10) monocarboxylic acids, benzoic acid and hydroxyacids in fine-mode (PM2.5) aerosols over the Bay of Bengal: Influence of heterogeneity in air masses and formation pathways S. Boreddy et al. 10.1016/j.atmosenv.2017.08.008
- High-NOxPhotooxidation ofn-Dodecane: Temperature Dependence of SOA Formation H. Lamkaddam et al. 10.1021/acs.est.6b03821
- Forest-atmosphere BVOC exchange in diverse and structurally complex canopies: 1-D modeling of a mid-successional forest in northern Michigan A. Bryan et al. 10.1016/j.atmosenv.2015.08.094
- Spectral- and size-resolved mass absorption efficiency of mineral dust aerosols in the shortwave spectrum: a simulation chamber study L. Caponi et al. 10.5194/acp-17-7175-2017
- Recent advances in understanding secondary organic aerosol: Implications for global climate forcing M. Shrivastava et al. 10.1002/2016RG000540
- Secondary organic aerosol from chlorine-initiated oxidation of isoprene D. Wang & L. Ruiz 10.5194/acp-17-13491-2017
- Low-volatility compounds contribute significantly to isoprene secondary organic aerosol (SOA) under high-NO<sub><i>x</i></sub> conditions R. Schwantes et al. 10.5194/acp-19-7255-2019
- Conformer-Specific Photolysis of Pyruvic Acid and the Effect of Water S. Blair et al. 10.1021/acs.jpca.9b10613
- Aqueous phase oligomerization of α,β-unsaturated carbonyls and acids investigated using ion mobility spectrometry coupled to mass spectrometry (IMS-MS) P. Renard et al. 10.1016/j.atmosenv.2015.10.060
- Enhanced levels of atmospheric low-molecular weight monocarboxylic acids in gas and particulates over Mt. Tai, North China, during field burning of agricultural wastes T. Mochizuki et al. 10.1016/j.atmosenv.2017.10.026
- Missing ozone-induced potential aerosol formation in a suburban deciduous forest T. Nakayama et al. 10.1016/j.atmosenv.2017.10.014
- Preliminary results from the FARCE 2015 campaign: multidisciplinary study of the forest–gas–aerosol–cloud system on the tropical island of La Réunion V. Duflot et al. 10.5194/acp-19-10591-2019
- Tropospheric Aqueous-Phase Oxidation of Isoprene-Derived Dihydroxycarbonyl Compounds T. Otto et al. 10.1021/acs.jpca.7b05879
- Cloud Processing of Secondary Organic Aerosol from Isoprene and Methacrolein Photooxidation C. Giorio et al. 10.1021/acs.jpca.7b05933
- Proton-Transfer-Reaction Mass Spectrometry: Applications in Atmospheric Sciences B. Yuan et al. 10.1021/acs.chemrev.7b00325
- Multiphase Photochemistry of Pyruvic Acid under Atmospheric Conditions A. Reed Harris et al. 10.1021/acs.jpca.7b01107
- Development and Evaluation of a Detailed Mechanism for Gas-Phase Atmospheric Reactions of Furans J. Jiang et al. 10.1021/acsearthspacechem.0c00058
- Chemistry and Photochemistry of Pyruvic Acid at the Air–Water Interface K. Kappes et al. 10.1021/acs.jpca.0c09096
- Atmospheric Simulation Chamber Studies of the Gas-Phase Photolysis of Pyruvic Acid A. Reed Harris et al. 10.1021/acs.jpca.7b05139
- Comparison of Measurement-Based Methodologies to Apportion Secondary Organic Carbon (SOC) in PM2.5: A Review of Recent Studies D. Srivastava et al. 10.3390/atmos9110452
- The MCM v3.3.1 degradation scheme for isoprene M. Jenkin et al. 10.5194/acp-15-11433-2015
- Quantifying Atmospheric Parameter Ranges for Ambient Secondary Organic Aerosol Formation W. Porter et al. 10.1021/acsearthspacechem.1c00090
- Large contribution to secondary organic aerosol from isoprene cloud chemistry H. Lamkaddam et al. 10.1126/sciadv.abe2952
- Low molecular weight dicarboxylic acids, oxocarboxylic acids and α-dicarbonyls as ozonolysis products of isoprene: Implication for the gaseous-phase formation of secondary organic aerosols S. Bikkina et al. 10.1016/j.scitotenv.2020.144472
- Formation of Metal–Cyanide Complexes in Deliquescent Airborne Particles: A New Possible Sink for HCN in Urban Environments C. Giorio et al. 10.1021/acs.est.7b03123
- Effect of NO2 on nocturnal chemistry of isoprene: Gaseous oxygenated products and secondary organic aerosol formation Y. Chen et al. 10.1016/j.scitotenv.2022.156908
- Secondary organic aerosol formation from isoprene photooxidation during cloud condensation–evaporation cycles L. Brégonzio-Rozier et al. 10.5194/acp-16-1747-2016
2 citations as recorded by crossref.
- Aqueous-phase oligomerization of methyl vinyl ketone through photooxidation – Part 1: Aging processes of oligomers P. Renard et al. 10.5194/acp-15-21-2015
- Emissions of biogenic volatile organic compounds and subsequent photochemical production of secondary organic aerosol in mesocosm studies of temperate and tropical plant species K. Wyche et al. 10.5194/acp-14-12781-2014
Saved (final revised paper)
Latest update: 27 Dec 2024
Short summary
First- and higher order -generation products formed from the oxidation of isoprene and methacrolein with OH radicals in the presence of NOx have been studied in a simulation chamber. Differences in light source are proposed to partially explain the discrepancies observed between different studies in the literature for both isoprene- and methacrolein-SOA mass yields. According to our results, these SOA yields in the atmosphere could be lower than suggested by most of the current chamber studies.
First- and higher order -generation products formed from the oxidation of isoprene and...
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