Articles | Volume 15, issue 24
https://doi.org/10.5194/acp-15-13993-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-13993-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Spring and summer contrast in new particle formation over nine forest areas in North America
Atmospheric Sciences Research Center, State University of New York, 251 Fuller Road, Albany, NY 12203, USA
Atmospheric Sciences Research Center, State University of New York, 251 Fuller Road, Albany, NY 12203, USA
S. C. Pryor
Department of Earth and Atmospheric Sciences, Cornell University, Ithaca, NY 14853, USA
P. R. Pillai
Department of Marine, Earth, and Atmospheric Sciences, North Carolina State University, Raleigh, NC 27695, USA
S. H. Lee
College of Public Health, Kent State University, Kent, OH, USA
J. Ortega
National Center for Atmospheric Research, P.O. Box 3000, Boulder, CO 80307, USA
J. J. Schwab
Atmospheric Sciences Research Center, State University of New York, 251 Fuller Road, Albany, NY 12203, USA
A. G. Hallar
Desert Research Institute, Storm Peak Laboratory, Steamboat Springs, CO 80488, USA
W. R. Leaitch
Environment Canada, Science and Technology Branch, Toronto, ON, Canada
V. P. Aneja
Department of Marine, Earth, and Atmospheric Sciences, North Carolina State University, Raleigh, NC 27695, USA
J. N. Smith
National Center for Atmospheric Research, P.O. Box 3000, Boulder, CO 80307, USA
Applied Physics Dept., University of Eastern Finland, P.O. Box 1627, Kuopio 70211, Finland
J. T. Walker
Department of Marine, Earth, and Atmospheric Sciences, North Carolina State University, Raleigh, NC 27695, USA
US Environmental Protection Agency, Office of Research and Development, Durham, NC 27711, USA
O. Hogrefe
Atmospheric Sciences Research Center, State University of New York, 251 Fuller Road, Albany, NY 12203, USA
currently at: Durham Technical Community College, Durham, NC 27703, USA
K. L. Demerjian
Atmospheric Sciences Research Center, State University of New York, 251 Fuller Road, Albany, NY 12203, USA
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Short summary
The role of low-volatility organics in new particle formation (NPF) in the atmosphere is assessed. An empirical formulation in which formation rate is a function of the concentrations of sulfuric acid and low-volatility organics significantly overpredicts NPF in the summer.
Two different schemes predict quite different nucleation rates (including their spatial patterns), concentrations of cloud condensation nuclei, and aerosol first indirect radiative forcing in North America.
The role of low-volatility organics in new particle formation (NPF) in the atmosphere is...
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