Articles | Volume 15, issue 20
https://doi.org/10.5194/acp-15-11773-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-11773-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Sensitivity analysis of the potential impact of discrepancies in stratosphere–troposphere exchange on inferred sources and sinks of CO2
Department of Physics, University of Toronto, Toronto, ON, Canada
D. B. A. Jones
Department of Physics, University of Toronto, Toronto, ON, Canada
Joint Institute for Regional Earth System Science and Engineering, University of California, Los Angeles, CA, USA
T. W. Walker
Department of Physics, University of Toronto, Toronto, ON, Canada
M. Keller
Department of Physics, University of Toronto, Toronto, ON, Canada
K. W. Bowman
Joint Institute for Regional Earth System Science and Engineering, University of California, Los Angeles, CA, USA
Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA, USA
D. K. Henze
Department of Mechanical Engineering, University of Colorado, Boulder, CO, USA
R. Nassar
Climate Research Division, Environment Canada, Toronto, ON, Canada
E. A. Kort
Department of Atmospheric, Oceanic and Space Sciences, University of Michigan, Ann Arbor, MI, USA
S. C. Wofsy
Harvard University, Cambridge, MA, USA
K. A. Walker
Department of Physics, University of Toronto, Toronto, ON, Canada
A. E. Bourassa
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatoon, Canada
D. A. Degenstein
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatoon, Canada
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Latest update: 07 Nov 2025
Short summary
The upper troposphere and lower stratosphere (UTLS) is characterized by strong gradients in the distribution of long-lived tracers, which are sensitive to discrepancies in transport in models. We found that our model overestimates CO2 in the polar UTLS through comparison of modeled CO2 with aircraft observations. We then corrected the modeled CO2 and quantified the impact of the correction on the flux estimates using an atmospheric model together with atmospheric CO2 measured from a satellite.
The upper troposphere and lower stratosphere (UTLS) is characterized by strong gradients in the...
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