Articles | Volume 15, issue 17
https://doi.org/10.5194/acp-15-10183-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-10183-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
14 Sep 2015
Research article |
| 14 Sep 2015
Chemical aging of single and multicomponent biomass burning aerosol surrogate particles by OH: implications for cloud condensation nucleus activity
J. H. Slade
Institute for Terrestrial and Planetary Atmospheres, School of Marine and Atmospheric Sciences, State University of New York at Stony Brook, Stony Brook, NY 11794, USA
R. Thalman
Brookhaven National Laboratory, Department of Environmental and Climate Sciences, Upton, NY 11973, USA
Brookhaven National Laboratory, Department of Environmental and Climate Sciences, Upton, NY 11973, USA
Institute for Terrestrial and Planetary Atmospheres, School of Marine and Atmospheric Sciences, State University of New York at Stony Brook, Stony Brook, NY 11794, USA
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Cited
27 citations as recorded by crossref.
- Skyfall—neglected roles of volcano ash and black carbon rich aerosols for microbial plankton in the ocean M. Weinbauer et al. 10.1093/plankt/fbw100
- The particle phase state during the biomass burning events Y. Liu et al. 10.1016/j.scitotenv.2021.148035
- Kinetics study of heterogeneous reactions of ozone with unsaturated fatty acid single droplets using micro-FTIR spectroscopy X. He et al. 10.1039/C6RA25255A
- Effects of Relative Humidity and Particle Phase Water on the Heterogeneous OH Oxidation of 2-Methylglutaric Acid Aqueous Droplets M. Chim et al. 10.1021/acs.jpca.6b11606
- Effects of inorganic salts on the heterogeneous OH oxidation of organic compounds: insights from methylglutaric acid–ammonium sulfate H. Lam et al. 10.5194/acp-19-9581-2019
- Case study evaluation of size-resolved molecular composition and phase state of carbonaceous particles in wildfire influenced smoke from the Pacific Northwest G. Vandergrift et al. 10.1039/D3EA00058C
- Characterization of the temperature and humidity-dependent phase diagram of amorphous nanoscale organic aerosols N. Rothfuss & M. Petters 10.1039/C6CP08593H
- Black carbon linked aerosol hygroscopic growth: Size and mixing state are crucial B. Sarangi et al. 10.1016/j.atmosenv.2018.12.001
- How Asian slum emissions impact local microclimates in polluted air masses S. Ghosh et al. 10.1002/asl.1124
- Synthesis and spin trapping properties of polystyrene supported trifluoromethylated cyclic nitrones A. Earla et al. 10.1080/10715762.2019.1683171
- Influence of relative humidity on the heterogeneous oxidation of secondary organic aerosol Z. Li et al. 10.5194/acp-18-14585-2018
- Effects of liquid–liquid phase separation and relative humidity on the heterogeneous OH oxidation of inorganic–organic aerosols: insights from methylglutaric acid and ammonium sulfate particles H. Lam et al. 10.5194/acp-21-2053-2021
- Size Dependence of the Physical Characteristics of Particles Containing Refractory Black Carbon in Diesel Vehicle Exhaust C. Han et al. 10.1021/acs.est.8b04603
- Hygroscopicity of Secondary Brown Carbon Aerosol from Aqueous Photo-Oxidation of Phenolic Precursors K. Betz et al. 10.1021/acsearthspacechem.2c00132
- Cloud droplet activation through oxidation of organic aerosol influenced by temperature and particle phase state J. Slade et al. 10.1002/2016GL072424
- Diffusive confinement of free radical intermediates in the OH radical oxidation of semisolid aerosols A. Wiegel et al. 10.1039/C7CP00696A
- Properties and emission factors of cloud condensation nuclei from biomass cookstoves – observations of a strong dependency on potassium content in the fuel T. Kristensen et al. 10.5194/acp-21-8023-2021
- Effects of Atmospheric Aging Processes on Nascent Sea Spray Aerosol Physicochemical Properties C. Kaluarachchi et al. 10.1021/acsearthspacechem.2c00258
- Desorption lifetimes and activation energies influencing gas–surface interactions and multiphase chemical kinetics D. Knopf et al. 10.5194/acp-24-3445-2024
- Size-Dependent Nascent Sea Spray Aerosol Bounce Fractions and Estimated Viscosity: The Role of Divalent Cation Enrichment, Surface Tension, and the Kelvin Effect P. Tumminello et al. 10.1021/acs.est.4c04312
- Short review on PM-bound water. Its presence in the atmosphere, forms of occurrence and determination by Karl Fischer coulometric titration K. Widziewicz et al. 10.1051/e3sconf/20184400187
- Changes in Light Absorptivity of Molecular Weight Separated Brown Carbon Due to Photolytic Aging J. Wong et al. 10.1021/acs.est.7b01739
- Condensed-phase biogenic–anthropogenic interactions with implications for cold cloud formation J. Charnawskas et al. 10.1039/C7FD00010C
- Characteristics of Scanning Flow Condensation Particle Counter (SFCPC): A rapid approach for retrieving hygroscopicity and chemical composition of sub-10 nm aerosol particles K. Zhang et al. 10.1080/02786826.2023.2245859
- Microphysical characteristics of black carbon from various emission sources H. Liu et al. 10.1016/j.atmosenv.2023.119825
- Predicting Aerosol Reactivity Across Scales: from the Laboratory to the Atmosphere F. Houle et al. 10.1021/acs.est.8b04688
- Anhydrosugars as tracers in the Earth system L. Suciu et al. 10.1007/s10533-019-00622-0
27 citations as recorded by crossref.
- Skyfall—neglected roles of volcano ash and black carbon rich aerosols for microbial plankton in the ocean M. Weinbauer et al. 10.1093/plankt/fbw100
- The particle phase state during the biomass burning events Y. Liu et al. 10.1016/j.scitotenv.2021.148035
- Kinetics study of heterogeneous reactions of ozone with unsaturated fatty acid single droplets using micro-FTIR spectroscopy X. He et al. 10.1039/C6RA25255A
- Effects of Relative Humidity and Particle Phase Water on the Heterogeneous OH Oxidation of 2-Methylglutaric Acid Aqueous Droplets M. Chim et al. 10.1021/acs.jpca.6b11606
- Effects of inorganic salts on the heterogeneous OH oxidation of organic compounds: insights from methylglutaric acid–ammonium sulfate H. Lam et al. 10.5194/acp-19-9581-2019
- Case study evaluation of size-resolved molecular composition and phase state of carbonaceous particles in wildfire influenced smoke from the Pacific Northwest G. Vandergrift et al. 10.1039/D3EA00058C
- Characterization of the temperature and humidity-dependent phase diagram of amorphous nanoscale organic aerosols N. Rothfuss & M. Petters 10.1039/C6CP08593H
- Black carbon linked aerosol hygroscopic growth: Size and mixing state are crucial B. Sarangi et al. 10.1016/j.atmosenv.2018.12.001
- How Asian slum emissions impact local microclimates in polluted air masses S. Ghosh et al. 10.1002/asl.1124
- Synthesis and spin trapping properties of polystyrene supported trifluoromethylated cyclic nitrones A. Earla et al. 10.1080/10715762.2019.1683171
- Influence of relative humidity on the heterogeneous oxidation of secondary organic aerosol Z. Li et al. 10.5194/acp-18-14585-2018
- Effects of liquid–liquid phase separation and relative humidity on the heterogeneous OH oxidation of inorganic–organic aerosols: insights from methylglutaric acid and ammonium sulfate particles H. Lam et al. 10.5194/acp-21-2053-2021
- Size Dependence of the Physical Characteristics of Particles Containing Refractory Black Carbon in Diesel Vehicle Exhaust C. Han et al. 10.1021/acs.est.8b04603
- Hygroscopicity of Secondary Brown Carbon Aerosol from Aqueous Photo-Oxidation of Phenolic Precursors K. Betz et al. 10.1021/acsearthspacechem.2c00132
- Cloud droplet activation through oxidation of organic aerosol influenced by temperature and particle phase state J. Slade et al. 10.1002/2016GL072424
- Diffusive confinement of free radical intermediates in the OH radical oxidation of semisolid aerosols A. Wiegel et al. 10.1039/C7CP00696A
- Properties and emission factors of cloud condensation nuclei from biomass cookstoves – observations of a strong dependency on potassium content in the fuel T. Kristensen et al. 10.5194/acp-21-8023-2021
- Effects of Atmospheric Aging Processes on Nascent Sea Spray Aerosol Physicochemical Properties C. Kaluarachchi et al. 10.1021/acsearthspacechem.2c00258
- Desorption lifetimes and activation energies influencing gas–surface interactions and multiphase chemical kinetics D. Knopf et al. 10.5194/acp-24-3445-2024
- Size-Dependent Nascent Sea Spray Aerosol Bounce Fractions and Estimated Viscosity: The Role of Divalent Cation Enrichment, Surface Tension, and the Kelvin Effect P. Tumminello et al. 10.1021/acs.est.4c04312
- Short review on PM-bound water. Its presence in the atmosphere, forms of occurrence and determination by Karl Fischer coulometric titration K. Widziewicz et al. 10.1051/e3sconf/20184400187
- Changes in Light Absorptivity of Molecular Weight Separated Brown Carbon Due to Photolytic Aging J. Wong et al. 10.1021/acs.est.7b01739
- Condensed-phase biogenic–anthropogenic interactions with implications for cold cloud formation J. Charnawskas et al. 10.1039/C7FD00010C
- Characteristics of Scanning Flow Condensation Particle Counter (SFCPC): A rapid approach for retrieving hygroscopicity and chemical composition of sub-10 nm aerosol particles K. Zhang et al. 10.1080/02786826.2023.2245859
- Microphysical characteristics of black carbon from various emission sources H. Liu et al. 10.1016/j.atmosenv.2023.119825
- Predicting Aerosol Reactivity Across Scales: from the Laboratory to the Atmosphere F. Houle et al. 10.1021/acs.est.8b04688
- Anhydrosugars as tracers in the Earth system L. Suciu et al. 10.1007/s10533-019-00622-0
Saved (final revised paper)
Saved (preprint)
Latest update: 13 Dec 2024
Short summary
Aerosol particles undergo chemical modification during atmospheric transport due to reactions with trace gas species such as OH radicals affecting cloud formation and, thus, prediction of climate. Here, the cloud formation potential of surrogate biomass burning aerosol (BBA) is studied as a function of particle composition and OH exposure. We find that OH oxidation can alter the cloud formation potential of BBA, but its significance depends on the available water-soluble particulate material.
Aerosol particles undergo chemical modification during atmospheric transport due to reactions...
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