Articles | Volume 14, issue 16
https://doi.org/10.5194/acp-14-8323-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-8323-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Molecular corridors and kinetic regimes in the multiphase chemical evolution of secondary organic aerosol
M. Shiraiwa
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
T. Berkemeier
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
K. A. Schilling-Fahnestock
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125, USA
J. H. Seinfeld
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125, USA
U. Pöschl
Multiphase Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany
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Cited
72 citations as recorded by crossref.
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- Chemodiversity of organic nitrogen emissions from light-duty gasoline vehicles is governed by engine displacements and driving speed H. Han et al. 10.1016/j.scitotenv.2024.170792
- Acidification impacts on the molecular composition of dissolved organic matter revealed by FT-ICR MS H. Han et al. 10.1016/j.scitotenv.2021.150284
- Plasma–liquid interactions: a review and roadmap P. Bruggeman et al. 10.1088/0963-0252/25/5/053002
- On the implications of aerosol liquid water and phase separation for organic aerosol mass H. Pye et al. 10.5194/acp-17-343-2017
- Effect of relative humidity on the composition of secondary organic aerosol from the oxidation of toluene M. Hinks et al. 10.5194/acp-18-1643-2018
- Characterization of Organosulfates (OSs) in typical urban areas in Eastern China: Source, Process, and Volatility Y. Du et al. 10.1016/j.atmosres.2024.107258
- Large differences of highly oxygenated organic molecules (HOMs) and low-volatile species in secondary organic aerosols (SOAs) formed from ozonolysis of β-pinene and limonene D. Liu et al. 10.5194/acp-23-8383-2023
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa 10.1021/cr500487s
- Molecular Characterization of Brown Carbon in Biomass Burning Aerosol Particles P. Lin et al. 10.1021/acs.est.6b03024
- Changing shapes and implied viscosities of suspended submicron particles Y. Zhang et al. 10.5194/acp-15-7819-2015
- Joint Impacts of Acidity and Viscosity on the Formation of Secondary Organic Aerosol from Isoprene Epoxydiols (IEPOX) in Phase Separated Particles Y. Zhang et al. 10.1021/acsearthspacechem.9b00209
- Why would apparent κ linearly change with O/C? Assessing the role of volatility, solubility, and surface activity of organic aerosols S. Nakao 10.1080/02786826.2017.1352082
- The Cooling Rate- and Volatility-Dependent Glass-Forming Properties of Organic Aerosols Measured by Broadband Dielectric Spectroscopy Y. Zhang et al. 10.1021/acs.est.9b03317
- Volatility and Viscosity Are Correlated in Terpene Secondary Organic Aerosol Formed in a Flow Reactor W. Champion et al. 10.1021/acs.estlett.9b00412
- ORACLE 2-D (v2.0): an efficient module to compute the volatility and oxygen content of organic aerosol with a global chemistry–climate model A. Tsimpidi et al. 10.5194/gmd-11-3369-2018
- Transformation Mechanism of Organic Matter in the Treatment of Petroleum-Based Drilling Cuttings by the Hammermill Thermal Desorption Cutting Treatment System D. Lin et al. 10.1061/JOEEDU.EEENG-7723
- Molecular corridors and parameterizations of volatility in the chemical evolution of organic aerosols Y. Li et al. 10.5194/acp-16-3327-2016
- The origin of potential precursors of secondary organic aerosols during combustion of biochar and softwood in residential heating J. Růžičková et al. 10.1016/j.psep.2022.03.036
- Impact of phase state and non-ideal mixing on equilibration timescales of secondary organic aerosol partitioning M. Schervish & M. Shiraiwa 10.5194/acp-23-221-2023
- Chemical and Toxicological Evolution of Carbon Nanotubes During Atmospherically Relevant Aging Processes Y. Liu et al. 10.1021/es505298d
- Reactive oxygen species formed in aqueous mixtures of secondary organic aerosols and mineral dust influencing cloud chemistry and public health in the Anthropocene H. Tong et al. 10.1039/C7FD00023E
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- Size-Dependent Morphology, Composition, Phase State, and Water Uptake of Nascent Submicrometer Sea Spray Aerosols during a Phytoplankton Bloom C. Kaluarachchi et al. 10.1021/acsearthspacechem.1c00306
- Predictions of the glass transition temperature and viscosity of organic aerosols from volatility distributions Y. Li et al. 10.5194/acp-20-8103-2020
- Heterogeneous Oxidation of Atmospheric Organic Aerosol: Kinetics of Changes to the Amount and Oxidation State of Particle-Phase Organic Carbon J. Kroll et al. 10.1021/acs.jpca.5b06946
- Secondary organic aerosols derived from intermediate-volatility n-alkanes adopt low-viscous phase state T. Galeazzo et al. 10.5194/acp-24-5549-2024
- Technical note: Monte Carlo genetic algorithm (MCGA) for model analysis of multiphase chemical kinetics to determine transport and reaction rate coefficients using multiple experimental data sets T. Berkemeier et al. 10.5194/acp-17-8021-2017
- Nanoparticle growth by particle-phase chemistry M. Apsokardu & M. Johnston 10.5194/acp-18-1895-2018
- Aging Effects on Biomass Burning Aerosol Mass and Composition: A Critical Review of Field and Laboratory Studies A. Hodshire et al. 10.1021/acs.est.9b02588
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- Global distribution of particle phase state in atmospheric secondary organic aerosols M. Shiraiwa et al. 10.1038/ncomms15002
- The effects of humidity and ammonia on the chemical composition of secondary aerosols from toluene/NOx photo-oxidation L. Chen et al. 10.1016/j.scitotenv.2020.138671
- Model–measurement comparison of functional group abundance in <i>α</i>-pinene and 1,3,5-trimethylbenzene secondary organic aerosol formation G. Ruggeri et al. 10.5194/acp-16-8729-2016
- Dwindling Aromatic Compounds in Fine Aerosols from Chunk Coal to Briquette Combustion W. Wei et al. 10.2139/ssrn.4015408
- Quantification of environmentally persistent free radicals and reactive oxygen species in atmospheric aerosol particles A. Arangio et al. 10.5194/acp-16-13105-2016
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- Increase of nitrooxy organosulfates in firework-related urban aerosols during Chinese New Year's Eve Q. Xie et al. 10.5194/acp-21-11453-2021
- Predicting the glass transition temperature and viscosity of secondary organic material using molecular composition W. DeRieux et al. 10.5194/acp-18-6331-2018
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- Studying volatility from composition, dilution, and heating measurements of secondary organic aerosols formed during <i>α</i>-pinene ozonolysis K. Sato et al. 10.5194/acp-18-5455-2018
- Effects of Photolysis on the Chemical and Optical Properties of Secondary Organic Material Over Extended Time Scales E. Walhout et al. 10.1021/acsearthspacechem.9b00109
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- Seasonal contributions to size-resolved n-alkanes (C8–C40) in the Shanghai atmosphere from regional anthropogenic activities and terrestrial plant waxes Y. Lyu et al. 10.1016/j.scitotenv.2016.11.201
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. 10.1039/D0EA00020E
- Overlooked Trace Molecules in Organic Aerosol Revealed by Gas Chromatography–Orbitrap Mass Spectrometry T. Wang et al. 10.1021/acs.est.4c03171
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- Exploring Volatility Properties of Discrete Secondary Organic Aerosol Constituents of α-Pinene and Polycyclic Aromatic Hydrocarbons Z. Babar et al. 10.1021/acsearthspacechem.0c00210
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- Predicting glass transition temperature and melting point of organic compounds via machine learning and molecular embeddings T. Galeazzo & M. Shiraiwa 10.1039/D1EA00090J
- A study of volatility by composition, heating, and dilution measurements of secondary organic aerosol from 1,3,5-trimethylbenzene K. Sato et al. 10.5194/acp-19-14901-2019
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Multiphase Chemical Kinetics of OH Radical Uptake by Molecular Organic Markers of Biomass Burning Aerosols: Humidity and Temperature Dependence, Surface Reaction, and Bulk Diffusion A. Arangio et al. 10.1021/jp510489z
- Annual dynamics of aerosol organic components in the free atmosphere over South-Western Siberia M. Arshinov et al. 10.1134/S1024856016010036
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. 10.1039/C6CP00634E
- Molecular-Level Insights into the Relationship between Volatility of Organic Aerosol Constituents and PM2.5 Air Pollution Levels: A Study with Ultrahigh-Resolution Mass Spectrometry K. Wang et al. 10.1021/acs.est.3c10662
- Connecting the solubility and CCN activation of complex organic aerosols: a theoretical study using solubility distributions I. Riipinen et al. 10.5194/acp-15-6305-2015
- Dwindling aromatic compounds in fine aerosols from chunk coal to honeycomb briquette combustion W. Wei et al. 10.1016/j.scitotenv.2022.155971
- Aqueous Photochemistry of Secondary Organic Aerosol of α-Pinene and α-Humulene Oxidized with Ozone, Hydroxyl Radical, and Nitrate Radical D. Romonosky et al. 10.1021/acs.jpca.6b10900
- Impacts of additional HONO sources on O<sub>3</sub> and PM<sub>2.5</sub> chemical coupling and control strategies in the Beijing–Tianjin–Hebei region of China Y. Li et al. 10.3402/tellusb.v67.23930
- Mass accommodation and gas–particle partitioning in secondary organic aerosols: dependence on diffusivity, volatility, particle-phase reactions, and penetration depth M. Shiraiwa & U. Pöschl 10.5194/acp-21-1565-2021
- Growth of Aitken mode ammonium sulfate particles by α-pinene ozonolysis J. Krasnomowitz et al. 10.1080/02786826.2019.1568381
- Deciphering 13C and 34S Isotopes of Organosulfates in Urban Aerosols by FT-ICR Mass Spectrometry Q. Xie et al. 10.1021/acs.estlett.2c00255
- Organic Vapors from Residential Biomass Combustion: Emission Characteristics and Conversion to Secondary Organic Aerosols R. Li et al. 10.3390/atmos15060692
- Increase of High Molecular Weight Organosulfate With Intensifying Urban Air Pollution in the Megacity Beijing Q. Xie et al. 10.1029/2019JD032200
- Accelerating models for multiphase chemical kinetics through machine learning with polynomial chaos expansion and neural networks T. Berkemeier et al. 10.5194/gmd-16-2037-2023
- Estimating mean molecular weight, carbon number, and OM∕OC with mid-infrared spectroscopy in organic particulate matter samples from a monitoring network A. Yazdani et al. 10.5194/amt-14-4805-2021
72 citations as recorded by crossref.
- Modeling the Effects of Dimerization and Bulk Diffusion on the Evaporative Behavior of Secondary Organic Aerosol Formed from α-Pinene and 1,3,5-Trimethylbenzene Y. Morino et al. 10.1021/acsearthspacechem.0c00106
- Chemodiversity of organic nitrogen emissions from light-duty gasoline vehicles is governed by engine displacements and driving speed H. Han et al. 10.1016/j.scitotenv.2024.170792
- Acidification impacts on the molecular composition of dissolved organic matter revealed by FT-ICR MS H. Han et al. 10.1016/j.scitotenv.2021.150284
- Plasma–liquid interactions: a review and roadmap P. Bruggeman et al. 10.1088/0963-0252/25/5/053002
- On the implications of aerosol liquid water and phase separation for organic aerosol mass H. Pye et al. 10.5194/acp-17-343-2017
- Effect of relative humidity on the composition of secondary organic aerosol from the oxidation of toluene M. Hinks et al. 10.5194/acp-18-1643-2018
- Characterization of Organosulfates (OSs) in typical urban areas in Eastern China: Source, Process, and Volatility Y. Du et al. 10.1016/j.atmosres.2024.107258
- Large differences of highly oxygenated organic molecules (HOMs) and low-volatile species in secondary organic aerosols (SOAs) formed from ozonolysis of β-pinene and limonene D. Liu et al. 10.5194/acp-23-8383-2023
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa 10.1021/cr500487s
- Molecular Characterization of Brown Carbon in Biomass Burning Aerosol Particles P. Lin et al. 10.1021/acs.est.6b03024
- Changing shapes and implied viscosities of suspended submicron particles Y. Zhang et al. 10.5194/acp-15-7819-2015
- Joint Impacts of Acidity and Viscosity on the Formation of Secondary Organic Aerosol from Isoprene Epoxydiols (IEPOX) in Phase Separated Particles Y. Zhang et al. 10.1021/acsearthspacechem.9b00209
- Why would apparent κ linearly change with O/C? Assessing the role of volatility, solubility, and surface activity of organic aerosols S. Nakao 10.1080/02786826.2017.1352082
- The Cooling Rate- and Volatility-Dependent Glass-Forming Properties of Organic Aerosols Measured by Broadband Dielectric Spectroscopy Y. Zhang et al. 10.1021/acs.est.9b03317
- Volatility and Viscosity Are Correlated in Terpene Secondary Organic Aerosol Formed in a Flow Reactor W. Champion et al. 10.1021/acs.estlett.9b00412
- ORACLE 2-D (v2.0): an efficient module to compute the volatility and oxygen content of organic aerosol with a global chemistry–climate model A. Tsimpidi et al. 10.5194/gmd-11-3369-2018
- Transformation Mechanism of Organic Matter in the Treatment of Petroleum-Based Drilling Cuttings by the Hammermill Thermal Desorption Cutting Treatment System D. Lin et al. 10.1061/JOEEDU.EEENG-7723
- Molecular corridors and parameterizations of volatility in the chemical evolution of organic aerosols Y. Li et al. 10.5194/acp-16-3327-2016
- The origin of potential precursors of secondary organic aerosols during combustion of biochar and softwood in residential heating J. Růžičková et al. 10.1016/j.psep.2022.03.036
- Impact of phase state and non-ideal mixing on equilibration timescales of secondary organic aerosol partitioning M. Schervish & M. Shiraiwa 10.5194/acp-23-221-2023
- Chemical and Toxicological Evolution of Carbon Nanotubes During Atmospherically Relevant Aging Processes Y. Liu et al. 10.1021/es505298d
- Reactive oxygen species formed in aqueous mixtures of secondary organic aerosols and mineral dust influencing cloud chemistry and public health in the Anthropocene H. Tong et al. 10.1039/C7FD00023E
- Desorption lifetimes and activation energies influencing gas–surface interactions and multiphase chemical kinetics D. Knopf et al. 10.5194/acp-24-3445-2024
- Size-Dependent Morphology, Composition, Phase State, and Water Uptake of Nascent Submicrometer Sea Spray Aerosols during a Phytoplankton Bloom C. Kaluarachchi et al. 10.1021/acsearthspacechem.1c00306
- Predictions of the glass transition temperature and viscosity of organic aerosols from volatility distributions Y. Li et al. 10.5194/acp-20-8103-2020
- Heterogeneous Oxidation of Atmospheric Organic Aerosol: Kinetics of Changes to the Amount and Oxidation State of Particle-Phase Organic Carbon J. Kroll et al. 10.1021/acs.jpca.5b06946
- Secondary organic aerosols derived from intermediate-volatility n-alkanes adopt low-viscous phase state T. Galeazzo et al. 10.5194/acp-24-5549-2024
- Technical note: Monte Carlo genetic algorithm (MCGA) for model analysis of multiphase chemical kinetics to determine transport and reaction rate coefficients using multiple experimental data sets T. Berkemeier et al. 10.5194/acp-17-8021-2017
- Nanoparticle growth by particle-phase chemistry M. Apsokardu & M. Johnston 10.5194/acp-18-1895-2018
- Aging Effects on Biomass Burning Aerosol Mass and Composition: A Critical Review of Field and Laboratory Studies A. Hodshire et al. 10.1021/acs.est.9b02588
- Multi-instrument comparison and compilation of non-methane organic gas emissions from biomass burning and implications for smoke-derived secondary organic aerosol precursors L. Hatch et al. 10.5194/acp-17-1471-2017
- Global distribution of particle phase state in atmospheric secondary organic aerosols M. Shiraiwa et al. 10.1038/ncomms15002
- The effects of humidity and ammonia on the chemical composition of secondary aerosols from toluene/NOx photo-oxidation L. Chen et al. 10.1016/j.scitotenv.2020.138671
- Model–measurement comparison of functional group abundance in <i>α</i>-pinene and 1,3,5-trimethylbenzene secondary organic aerosol formation G. Ruggeri et al. 10.5194/acp-16-8729-2016
- Dwindling Aromatic Compounds in Fine Aerosols from Chunk Coal to Briquette Combustion W. Wei et al. 10.2139/ssrn.4015408
- Quantification of environmentally persistent free radicals and reactive oxygen species in atmospheric aerosol particles A. Arangio et al. 10.5194/acp-16-13105-2016
- 100 Years of Progress in Gas-Phase Atmospheric Chemistry Research T. Wallington et al. 10.1175/AMSMONOGRAPHS-D-18-0008.1
- Compilation and evaluation of gas phase diffusion coefficients of reactive trace gases in the atmosphere: Volume 2. Diffusivities of organic compounds, pressure-normalised mean free paths, and average Knudsen numbers for gas uptake calculations M. Tang et al. 10.5194/acp-15-5585-2015
- Increase of nitrooxy organosulfates in firework-related urban aerosols during Chinese New Year's Eve Q. Xie et al. 10.5194/acp-21-11453-2021
- Predicting the glass transition temperature and viscosity of secondary organic material using molecular composition W. DeRieux et al. 10.5194/acp-18-6331-2018
- Solid, Semisolid, and Liquid Phase States of Individual Submicrometer Particles Directly Probed Using Atomic Force Microscopy H. Lee et al. 10.1021/acs.analchem.7b02755
- Impact of organic molecular structure on the estimation of atmospherically relevant physicochemical parameters G. Isaacman-VanWertz & B. Aumont 10.5194/acp-21-6541-2021
- Studying volatility from composition, dilution, and heating measurements of secondary organic aerosols formed during <i>α</i>-pinene ozonolysis K. Sato et al. 10.5194/acp-18-5455-2018
- Effects of Photolysis on the Chemical and Optical Properties of Secondary Organic Material Over Extended Time Scales E. Walhout et al. 10.1021/acsearthspacechem.9b00109
- Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements A. Maclean et al. 10.1021/acsearthspacechem.1c00296
- Seasonal contributions to size-resolved n-alkanes (C8–C40) in the Shanghai atmosphere from regional anthropogenic activities and terrestrial plant waxes Y. Lyu et al. 10.1016/j.scitotenv.2016.11.201
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. 10.1039/D0EA00020E
- Overlooked Trace Molecules in Organic Aerosol Revealed by Gas Chromatography–Orbitrap Mass Spectrometry T. Wang et al. 10.1021/acs.est.4c03171
- Technical Note: Development of chemoinformatic tools to enumerate functional groups in molecules for organic aerosol characterization G. Ruggeri & S. Takahama 10.5194/acp-16-4401-2016
- Exploring Volatility Properties of Discrete Secondary Organic Aerosol Constituents of α-Pinene and Polycyclic Aromatic Hydrocarbons Z. Babar et al. 10.1021/acsearthspacechem.0c00210
- Dwindling Aromatic Compounds in Fine Aerosols from Chunk Coal to Briquette Combustion W. Wei et al. 10.2139/ssrn.4045477
- Organic Enrichment, Physical Phase State, and Surface Tension Depression of Nascent Core–Shell Sea Spray Aerosols during Two Phytoplankton Blooms H. Lee et al. 10.1021/acsearthspacechem.0c00032
- Impact of Aerosol-Cloud Cycling on Aqueous Secondary Organic Aerosol Formation W. Tsui et al. 10.3390/atmos10110666
- Organic Nitrate Contribution to New Particle Formation and Growth in Secondary Organic Aerosols from α-Pinene Ozonolysis T. Berkemeier et al. 10.1021/acs.est.6b00961
- Predicting glass transition temperature and melting point of organic compounds via machine learning and molecular embeddings T. Galeazzo & M. Shiraiwa 10.1039/D1EA00090J
- A study of volatility by composition, heating, and dilution measurements of secondary organic aerosol from 1,3,5-trimethylbenzene K. Sato et al. 10.5194/acp-19-14901-2019
- Current State of Atmospheric Aerosol Thermodynamics and Mass Transfer Modeling: A Review K. Semeniuk & A. Dastoor 10.3390/atmos11020156
- Multiphase Chemical Kinetics of OH Radical Uptake by Molecular Organic Markers of Biomass Burning Aerosols: Humidity and Temperature Dependence, Surface Reaction, and Bulk Diffusion A. Arangio et al. 10.1021/jp510489z
- Annual dynamics of aerosol organic components in the free atmosphere over South-Western Siberia M. Arshinov et al. 10.1134/S1024856016010036
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. 10.1039/C6CP00634E
- Molecular-Level Insights into the Relationship between Volatility of Organic Aerosol Constituents and PM2.5 Air Pollution Levels: A Study with Ultrahigh-Resolution Mass Spectrometry K. Wang et al. 10.1021/acs.est.3c10662
- Connecting the solubility and CCN activation of complex organic aerosols: a theoretical study using solubility distributions I. Riipinen et al. 10.5194/acp-15-6305-2015
- Dwindling aromatic compounds in fine aerosols from chunk coal to honeycomb briquette combustion W. Wei et al. 10.1016/j.scitotenv.2022.155971
- Aqueous Photochemistry of Secondary Organic Aerosol of α-Pinene and α-Humulene Oxidized with Ozone, Hydroxyl Radical, and Nitrate Radical D. Romonosky et al. 10.1021/acs.jpca.6b10900
- Impacts of additional HONO sources on O<sub>3</sub> and PM<sub>2.5</sub> chemical coupling and control strategies in the Beijing–Tianjin–Hebei region of China Y. Li et al. 10.3402/tellusb.v67.23930
- Mass accommodation and gas–particle partitioning in secondary organic aerosols: dependence on diffusivity, volatility, particle-phase reactions, and penetration depth M. Shiraiwa & U. Pöschl 10.5194/acp-21-1565-2021
- Growth of Aitken mode ammonium sulfate particles by α-pinene ozonolysis J. Krasnomowitz et al. 10.1080/02786826.2019.1568381
- Deciphering 13C and 34S Isotopes of Organosulfates in Urban Aerosols by FT-ICR Mass Spectrometry Q. Xie et al. 10.1021/acs.estlett.2c00255
- Organic Vapors from Residential Biomass Combustion: Emission Characteristics and Conversion to Secondary Organic Aerosols R. Li et al. 10.3390/atmos15060692
- Increase of High Molecular Weight Organosulfate With Intensifying Urban Air Pollution in the Megacity Beijing Q. Xie et al. 10.1029/2019JD032200
- Accelerating models for multiphase chemical kinetics through machine learning with polynomial chaos expansion and neural networks T. Berkemeier et al. 10.5194/gmd-16-2037-2023
- Estimating mean molecular weight, carbon number, and OM∕OC with mid-infrared spectroscopy in organic particulate matter samples from a monitoring network A. Yazdani et al. 10.5194/amt-14-4805-2021
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