Articles | Volume 14, issue 22 
            
                
                    
                    
            
            
            https://doi.org/10.5194/acp-14-12479-2014
                    © Author(s) 2014. This work is distributed under 
the Creative Commons Attribution 3.0 License.
                the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-14-12479-2014
                    © Author(s) 2014. This work is distributed under 
the Creative Commons Attribution 3.0 License.
                the Creative Commons Attribution 3.0 License.
Stratospheric lifetime ratio of CFC-11 and CFC-12 from satellite and model climatologies
                                            Jülich Supercomputing Centre, Forschungszentrum Jülich,   Jülich, Germany
                                        
                                    C. M. Hoppe
                                            Institut für Energie- und   Klimaforschung, Forschungszentrum Jülich, Jülich, Germany
                                        
                                    R. Müller
                                            Institut für Energie- und   Klimaforschung, Forschungszentrum Jülich, Jülich, Germany
                                        
                                    G. S. Dutton
                                            NOAA Earth System Research Laboratory, Global Monitoring   Division, Boulder, CO, USA
                                        
                                    J. C. Gille
                                            National Center for   Atmospheric Research, Boulder, CO, USA
                                        
                                    
                                            Center for Limb   Atmospheric Sounding, University of Colorado, Boulder, CO, USA
                                        
                                    S. Griessbach
                                            Jülich Supercomputing Centre, Forschungszentrum Jülich,   Jülich, Germany
                                        
                                    A. Jones
                                            Department of Physics, University of Toronto, Toronto,   Canada
                                        
                                    C. I. Meyer
                                            Jülich Supercomputing Centre, Forschungszentrum Jülich,   Jülich, Germany
                                        
                                    
                                            Institut für Energie- und   Klimaforschung, Forschungszentrum Jülich, Jülich, Germany
                                        
                                    C. M. Volk
                                            Bergische Universität Wuppertal, Fachbereich   Physik, Wuppertal, Germany
                                        
                                    K. A. Walker
                                            Department of Physics, University of Toronto, Toronto,   Canada
                                        
                                    
                                            Department of Chemistry,   University of Waterloo, Waterloo, Ontario, Canada
                                        
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Cited
14 citations as recorded by crossref.
- Retrieval of atmospheric CFC-11 and CFC-12 from high-resolution FTIR observations at Hefei and comparisons with other independent datasets X. Zeng et al. 10.5194/amt-15-6739-2022
- Individual and interactive effects of ocean acidification, global warming, and UV radiation on phytoplankton K. Gao et al. 10.1007/s10811-017-1329-6
- No severe ozone depletion in the tropical stratosphere in recent decades J. Kuttippurath et al. 10.5194/acp-24-6743-2024
- Interactions of anthropogenic stress factors on marine phytoplankton D. Häder & K. Gao 10.3389/fenvs.2015.00014
- Possible implications of enhanced chlorofluorocarbon-11 concentrations on ozone M. Dameris et al. 10.5194/acp-19-13759-2019
- New and improved infrared absorption cross sections for dichlorodifluoromethane (CFC-12) J. Harrison 10.5194/amt-8-3197-2015
- Stratospheric ozone loss in the Arctic winters between 2005 and 2013 derived with ACE-FTS measurements D. Griffin et al. 10.5194/acp-19-577-2019
- Monitoring of Solar Irradiance in the High Andes D. Häder & N. Cabrol 10.1111/php.13276
- Evaluation of stratospheric age of air from CF4, C2F6, C3F8, CHF3, HFC-125, HFC-227ea and SF6; implications for the calculations of halocarbon lifetimes, fractional release factors and ozone depletion potentials E. Leedham Elvidge et al. 10.5194/acp-18-3369-2018
- Tropical troposphere to stratosphere transport of carbon monoxide and long-lived trace species in the Chemical Lagrangian Model of the Stratosphere (CLaMS) R. Pommrich et al. 10.5194/gmd-7-2895-2014
- Assessing stratospheric transport in the CMAM30 simulations using ACE-FTS measurements F. Kolonjari et al. 10.5194/acp-18-6801-2018
- New and improved infrared absorption cross sections for trichlorofluoromethane (CFC-11) J. Harrison 10.5194/amt-11-5827-2018
- The generality of the GUGA MRCI approach in COLUMBUS for treating complex quantum chemistry H. Lischka et al. 10.1063/1.5144267
- The implementation of the CLaMS Lagrangian transport core into the chemistry climate model EMAC 2.40.1: application on age of air and transport of long-lived trace species C. Hoppe et al. 10.5194/gmd-7-2639-2014
13 citations as recorded by crossref.
- Retrieval of atmospheric CFC-11 and CFC-12 from high-resolution FTIR observations at Hefei and comparisons with other independent datasets X. Zeng et al. 10.5194/amt-15-6739-2022
- Individual and interactive effects of ocean acidification, global warming, and UV radiation on phytoplankton K. Gao et al. 10.1007/s10811-017-1329-6
- No severe ozone depletion in the tropical stratosphere in recent decades J. Kuttippurath et al. 10.5194/acp-24-6743-2024
- Interactions of anthropogenic stress factors on marine phytoplankton D. Häder & K. Gao 10.3389/fenvs.2015.00014
- Possible implications of enhanced chlorofluorocarbon-11 concentrations on ozone M. Dameris et al. 10.5194/acp-19-13759-2019
- New and improved infrared absorption cross sections for dichlorodifluoromethane (CFC-12) J. Harrison 10.5194/amt-8-3197-2015
- Stratospheric ozone loss in the Arctic winters between 2005 and 2013 derived with ACE-FTS measurements D. Griffin et al. 10.5194/acp-19-577-2019
- Monitoring of Solar Irradiance in the High Andes D. Häder & N. Cabrol 10.1111/php.13276
- Evaluation of stratospheric age of air from CF4, C2F6, C3F8, CHF3, HFC-125, HFC-227ea and SF6; implications for the calculations of halocarbon lifetimes, fractional release factors and ozone depletion potentials E. Leedham Elvidge et al. 10.5194/acp-18-3369-2018
- Tropical troposphere to stratosphere transport of carbon monoxide and long-lived trace species in the Chemical Lagrangian Model of the Stratosphere (CLaMS) R. Pommrich et al. 10.5194/gmd-7-2895-2014
- Assessing stratospheric transport in the CMAM30 simulations using ACE-FTS measurements F. Kolonjari et al. 10.5194/acp-18-6801-2018
- New and improved infrared absorption cross sections for trichlorofluoromethane (CFC-11) J. Harrison 10.5194/amt-11-5827-2018
- The generality of the GUGA MRCI approach in COLUMBUS for treating complex quantum chemistry H. Lischka et al. 10.1063/1.5144267
Saved (final revised paper)
Latest update: 31 Oct 2025
Short summary
                    Stratospheric lifetimes determine the global warming and ozone depletion potentials of chlorofluorocarbons. We present new estimates of the CFC-11/CFC-12 lifetime ratio from satellite and model data (ACE-FTS, HIRDLS, MIPAS, and EMAC/CLaMS). Our estimates of 0.46+/-0.04 (satellites) and 0.48+/-0.07 (model) are in excellent agreement with the recent SPARC reassessment. Having smaller uncertainties than other studies, our results can help to better constrain future CFC lifetime recommendations.
                    Stratospheric lifetimes determine the global warming and ozone depletion potentials of...
                    
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