Research article
| Highlight paper
20 Nov 2014
Research article
| Highlight paper
| 20 Nov 2014
Missing SO2 oxidant in the coastal atmosphere? – observations from high-resolution measurements of OH and atmospheric sulfur compounds
H. Berresheim et al.
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Cited
31 citations as recorded by crossref.
- Sulfur Dioxide Modifies Aerosol Particle Formation and Growth by Ozonolysis of Monoterpenes and Isoprene C. Stangl et al. 10.1029/2018JD030064
- Contribution from biogenic organic compounds to particle growth during the 2010 BEACHON-ROCS campaign in a Colorado temperate needleleaf forest L. Zhou et al. 10.5194/acp-15-8643-2015
- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
- Characterisation and improvement of <i>j</i>(O<sup>1</sup>D) filter radiometers B. Bohn et al. 10.5194/amt-9-3455-2016
- Secondary aerosol formation from dimethyl sulfide – improved mechanistic understanding based on smog chamber experiments and modelling R. Wollesen de Jonge et al. 10.5194/acp-21-9955-2021
- Chemical characterization of atmospheric ions at the high altitude research station Jungfraujoch (Switzerland) C. Frege et al. 10.5194/acp-17-2613-2017
- Accurate Quantification of Radiosulfur in Chemically Complex Atmospheric Samples M. Lin & M. Thiemens 10.1021/acs.analchem.7b05079
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- Role of Criegee intermediates in the formation of sulfuric acid at a Mediterranean (Cape Corsica) site under influence of biogenic emissions A. Kukui et al. 10.5194/acp-21-13333-2021
- The Role of Oxalic Acid in New Particle Formation from Methanesulfonic Acid, Methylamine, and Water K. Arquero et al. 10.1021/acs.est.6b05056
- Theoretical Insight into the Reaction Mechanism and Kinetics for the Criegee Intermediate of anti-PhCHOO with SO2 B. Du & W. Zhang 10.3390/molecules25133041
- Particle formation and growth from oxalic acid, methanesulfonic acid, trimethylamine and water: a combined experimental and theoretical study K. Arquero et al. 10.1039/C7CP04468B
- Theoretical Chemical Kinetics in Tropospheric Chemistry: Methodologies and Applications L. Vereecken et al. 10.1021/cr500488p
- Kinetics of a Criegee intermediate that would survive high humidity and may oxidize atmospheric SO 2 H. Huang et al. 10.1073/pnas.1513149112
- Air quality changes in cities during the COVID-19 lockdown: A critical review M. Adam et al. 10.1016/j.atmosres.2021.105823
- Atmospheric isoprene ozonolysis: impacts of stabilised Criegee intermediate reactions with SO<sub>2</sub>, H<sub>2</sub>O and dimethyl sulfide M. Newland et al. 10.5194/acp-15-9521-2015
- The reaction of methyl peroxy and hydroxyl radicals as a major source of atmospheric methanol J. Müller et al. 10.1038/ncomms13213
- Nanoparticles grown from methanesulfonic acid and methylamine: microscopic structures and formation mechanism J. Xu et al. 10.1039/C7CP06489F
- Quantification of Gas-to-Particle Conversion Rates of Sulfur in the Terrestrial Atmosphere Using High-Sensitivity Measurements of Cosmogenic 35S M. Lin et al. 10.1021/acsearthspacechem.7b00047
- Integrated experimental and theoretical approach to probe the synergistic effect of ammonia in methanesulfonic acid reactions with small alkylamines V. Perraud et al. 10.1039/C9EM00431A
- Adsorption of SO2 on mineral dust particles influenced by atmospheric moisture T. Wang et al. 10.1016/j.atmosenv.2018.08.008
- Size-Resolved Chemical Composition of Sub-20 nm Particles from Methanesulfonic Acid Reactions with Methylamine and Ammonia V. Perraud et al. 10.1021/acsearthspacechem.0c00120
- An advanced modeling study on the impacts and atmospheric implications of multiphase dimethyl sulfide chemistry E. Hoffmann et al. 10.1073/pnas.1606320113
- New particle formation in the volcanic eruption plume of the Piton de la Fournaise: specific features from a long-term dataset C. Rose et al. 10.5194/acp-19-13243-2019
- Investigation of several proxies to estimate sulfuric acid concentration under volcanic plume conditions C. Rose et al. 10.5194/acp-21-4541-2021
- Low‐Volatility Vapors and New Particle Formation Over the Southern Ocean During the Antarctic Circumnavigation Expedition A. Baccarini et al. 10.1029/2021JD035126
- Criegee intermediates and their impacts on the troposphere M. Khan et al. 10.1039/C7EM00585G
- The atmospheric impacts of monoterpene ozonolysis on global stabilised Criegee intermediate budgets and SO<sub>2</sub> oxidation: experiment, theory and modelling M. Newland et al. 10.5194/acp-18-6095-2018
- Strong Negative Temperature Dependence of the Simplest Criegee Intermediate CH2OO Reaction with Water Dimer M. Smith et al. 10.1021/acs.jpclett.5b01109
- Competition between H2O and (H2O)2 reactions with CH2OO/CH3CHOO L. Lin et al. 10.1039/C5CP06446E
- Online Quantification of Criegee Intermediates of α-Pinene Ozonolysis by Stabilization with Spin Traps and Proton-Transfer Reaction Mass Spectrometry Detection C. Giorio et al. 10.1021/jacs.6b10981
28 citations as recorded by crossref.
- Sulfur Dioxide Modifies Aerosol Particle Formation and Growth by Ozonolysis of Monoterpenes and Isoprene C. Stangl et al. 10.1029/2018JD030064
- Contribution from biogenic organic compounds to particle growth during the 2010 BEACHON-ROCS campaign in a Colorado temperate needleleaf forest L. Zhou et al. 10.5194/acp-15-8643-2015
- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
- Characterisation and improvement of <i>j</i>(O<sup>1</sup>D) filter radiometers B. Bohn et al. 10.5194/amt-9-3455-2016
- Secondary aerosol formation from dimethyl sulfide – improved mechanistic understanding based on smog chamber experiments and modelling R. Wollesen de Jonge et al. 10.5194/acp-21-9955-2021
- Chemical characterization of atmospheric ions at the high altitude research station Jungfraujoch (Switzerland) C. Frege et al. 10.5194/acp-17-2613-2017
- Accurate Quantification of Radiosulfur in Chemically Complex Atmospheric Samples M. Lin & M. Thiemens 10.1021/acs.analchem.7b05079
- Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation L. Xu et al. 10.1007/s00376-020-0284-3
- Role of Criegee intermediates in the formation of sulfuric acid at a Mediterranean (Cape Corsica) site under influence of biogenic emissions A. Kukui et al. 10.5194/acp-21-13333-2021
- The Role of Oxalic Acid in New Particle Formation from Methanesulfonic Acid, Methylamine, and Water K. Arquero et al. 10.1021/acs.est.6b05056
- Theoretical Insight into the Reaction Mechanism and Kinetics for the Criegee Intermediate of anti-PhCHOO with SO2 B. Du & W. Zhang 10.3390/molecules25133041
- Particle formation and growth from oxalic acid, methanesulfonic acid, trimethylamine and water: a combined experimental and theoretical study K. Arquero et al. 10.1039/C7CP04468B
- Theoretical Chemical Kinetics in Tropospheric Chemistry: Methodologies and Applications L. Vereecken et al. 10.1021/cr500488p
- Kinetics of a Criegee intermediate that would survive high humidity and may oxidize atmospheric SO 2 H. Huang et al. 10.1073/pnas.1513149112
- Air quality changes in cities during the COVID-19 lockdown: A critical review M. Adam et al. 10.1016/j.atmosres.2021.105823
- Atmospheric isoprene ozonolysis: impacts of stabilised Criegee intermediate reactions with SO<sub>2</sub>, H<sub>2</sub>O and dimethyl sulfide M. Newland et al. 10.5194/acp-15-9521-2015
- The reaction of methyl peroxy and hydroxyl radicals as a major source of atmospheric methanol J. Müller et al. 10.1038/ncomms13213
- Nanoparticles grown from methanesulfonic acid and methylamine: microscopic structures and formation mechanism J. Xu et al. 10.1039/C7CP06489F
- Quantification of Gas-to-Particle Conversion Rates of Sulfur in the Terrestrial Atmosphere Using High-Sensitivity Measurements of Cosmogenic 35S M. Lin et al. 10.1021/acsearthspacechem.7b00047
- Integrated experimental and theoretical approach to probe the synergistic effect of ammonia in methanesulfonic acid reactions with small alkylamines V. Perraud et al. 10.1039/C9EM00431A
- Adsorption of SO2 on mineral dust particles influenced by atmospheric moisture T. Wang et al. 10.1016/j.atmosenv.2018.08.008
- Size-Resolved Chemical Composition of Sub-20 nm Particles from Methanesulfonic Acid Reactions with Methylamine and Ammonia V. Perraud et al. 10.1021/acsearthspacechem.0c00120
- An advanced modeling study on the impacts and atmospheric implications of multiphase dimethyl sulfide chemistry E. Hoffmann et al. 10.1073/pnas.1606320113
- New particle formation in the volcanic eruption plume of the Piton de la Fournaise: specific features from a long-term dataset C. Rose et al. 10.5194/acp-19-13243-2019
- Investigation of several proxies to estimate sulfuric acid concentration under volcanic plume conditions C. Rose et al. 10.5194/acp-21-4541-2021
- Low‐Volatility Vapors and New Particle Formation Over the Southern Ocean During the Antarctic Circumnavigation Expedition A. Baccarini et al. 10.1029/2021JD035126
- Criegee intermediates and their impacts on the troposphere M. Khan et al. 10.1039/C7EM00585G
- The atmospheric impacts of monoterpene ozonolysis on global stabilised Criegee intermediate budgets and SO<sub>2</sub> oxidation: experiment, theory and modelling M. Newland et al. 10.5194/acp-18-6095-2018
3 citations as recorded by crossref.
- Strong Negative Temperature Dependence of the Simplest Criegee Intermediate CH2OO Reaction with Water Dimer M. Smith et al. 10.1021/acs.jpclett.5b01109
- Competition between H2O and (H2O)2 reactions with CH2OO/CH3CHOO L. Lin et al. 10.1039/C5CP06446E
- Online Quantification of Criegee Intermediates of α-Pinene Ozonolysis by Stabilization with Spin Traps and Proton-Transfer Reaction Mass Spectrometry Detection C. Giorio et al. 10.1021/jacs.6b10981
Saved (final revised paper)
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Latest update: 04 Feb 2023
Short summary
Sulfuric acid plays a major role in the formation of aerosol particles and clouds. Measurements at the west coast of Ireland reveal that oxidation of SO2 by OH explains only 20%, on average, of H2SO4 formation in coastal marine air. Additional sources may be (a) oxidation by Criegee intermediates produced photolytically and/or (b) formation from SO3 instead of SO2 in the oxidation of dimethyl sulfide, suggesting an important role of marine emissions in the self-cleaning power of the atmosphere.
Sulfuric acid plays a major role in the formation of aerosol particles and clouds. Measurements...
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