the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Non-agricultural ammonia emissions in urban China
Abstract. The non-agricultural ammonia (NH3) emissions in cities have received little attention but could rival agricultural sources in term of the efficiency in PM formation. The starting point for finding credible solutions is to comprehensively establish a city-specific Non-agricultural Ammonia Emission Inventory (NAEI) and identify the largest sources where efforts can be directed to deliver the largest impact. In this paper, I present a NAEI of 113 national key cities targeted on environmental protection in China in 2010, which for the first time covers NH3 emissions from pets, infants, smokers, green land, and household products. Results show that totally 210 478 Mg, the NH3 emissions from traffic, fuel combustion, waste disposal, pets, green land, human, and household products are 67 671 Mg, 56 275 Mg, 44 289 Mg, 23 355 Mg, 7509 Mg, 7312 Mg, and 4069 Mg, respectively. The NH3 emission intensity from the municipal districts ranges from 0.08 to 3.13 Mg km−2 yr−1, with a average of 0.84 Mg km−2 yr−1. The high NH3 emission intensities in Beijing-Tianjin-Hebei region, Yangtze River Delta region and Pearl River Delta region support the view that non-agricultural NH3 sources play a key role in city-scale NH3 emissions and thus have potentially important implications for secondary PM formation (ammonium-sulfate-nitrate system) in urban agglomeration of China. Therefore, in addition to current SO2 and NOx controls, China also needs to allocate more scientific, technical, and legal resources on controlling non-agricultural NH3 emissions in the future.
- Preprint
(4911 KB) - Metadata XML
-
Supplement
(185 KB) - BibTeX
- EndNote
- SC C962: 'Beijing Ammonia measurments from Aura TES', John Worden, 31 Mar 2014
- RC C1659: 'Review comments for manuscript titled "Non-agricultural ammonia emissions in urban China"', Anonymous Referee #1, 23 Apr 2014
- RC C2889: 'Anonymous Referee #2', Anonymous Referee #2, 29 May 2014
- AC C3142: 'Withdrawal Request Letter', Yunhua Chang, 03 Jun 2014
- SC C962: 'Beijing Ammonia measurments from Aura TES', John Worden, 31 Mar 2014
- RC C1659: 'Review comments for manuscript titled "Non-agricultural ammonia emissions in urban China"', Anonymous Referee #1, 23 Apr 2014
- RC C2889: 'Anonymous Referee #2', Anonymous Referee #2, 29 May 2014
- AC C3142: 'Withdrawal Request Letter', Yunhua Chang, 03 Jun 2014
Viewed
HTML | XML | Total | BibTeX | EndNote | |
---|---|---|---|---|---|
2,520 | 5,329 | 182 | 8,031 | 142 | 159 |
- HTML: 2,520
- PDF: 5,329
- XML: 182
- Total: 8,031
- BibTeX: 142
- EndNote: 159
Cited
20 citations as recorded by crossref.
- Underestimated ammonia vehicular emissions in metropolitan city revealed by on-road mobile measurement C. Gu et al. 10.1088/1748-9326/acf94a
- Wet deposition of sulfur and nitrogen in Jiuzhaigou National Nature Reserve, Sichuan, China during 2015–2016: Possible effects from regional emission reduction and local tourist activities X. Qiao et al. 10.1016/j.envpol.2017.08.041
- High-resolution ammonia emission inventories with comprehensive analysis and evaluation in Henan, China, 2006–2016 C. Wang et al. 10.1016/j.atmosenv.2018.08.063
- Evidence of a Large Bias in Rooftop Measurements of Atmospheric Ammonia Y. Kuang et al. 10.1021/acsearthspacechem.1c00331
- Gaseous Ammonia Emissions from Coal and Biomass Combustion in Household Stoves with Different Combustion Efficiencies Q. Li et al. 10.1021/acs.estlett.6b00013
- Overlooked Nonagricultural and Wintertime Agricultural NH3 Emissions in Quzhou County, North China Plain: Evidence from 15N-Stable Isotopes S. Feng et al. 10.1021/acs.estlett.1c00935
- Assessment of carbonaceous aerosols in Shanghai, China – Part 1: long-term evolution, seasonal variations, and meteorological effects Y. Chang et al. 10.5194/acp-17-9945-2017
- Human Excreta as a Stable and Important Source of Atmospheric Ammonia in the Megacity of Shanghai Y. Chang et al. 10.1371/journal.pone.0144661
- Recent development of a refined multiple air pollutant emission inventory of vehicles in the Central Plains of China X. Gu et al. 10.1016/j.jes.2019.04.010
- Developing Nitrogen Isotopic Source Profiles of Atmospheric Ammonia for Source Apportionment of Ammonia in Urban Beijing C. Wang et al. 10.3389/fenvs.2022.903013
- High-resolution ammonia emissions inventories in Fujian, China, 2009–2015 S. Wu et al. 10.1016/j.atmosenv.2017.04.027
- Source apportionment of atmospheric ammonia before, during, and after the 2014 APEC summit in Beijing using stable nitrogen isotope signatures Y. Chang et al. 10.5194/acp-16-11635-2016
- Comment on “Fossil Fuel Combustion-Related Emissions Dominate Atmospheric Ammonia Sources during Severe Haze Episodes: Evidence from 15N-Stable Isotope in Size-Resolved Aerosol Ammonium” Y. Chang & H. Ma 10.1021/acs.est.6b03458
- PM2.5 pollution is substantially affected by ammonia emissions in China Y. Wu et al. 10.1016/j.envpol.2016.08.027
- The importance of vehicle emissions as a source of atmospheric ammonia in the megacity of Shanghai Y. Chang et al. 10.5194/acp-16-3577-2016
- Process-Based Isolation of Pyrogenic Ammonia in Urban Atmosphere and Implications for Ammonium Nitrate Control Y. Feng et al. 10.1021/acsearthspacechem.2c00372
- Assessing Contributions of Agricultural and Nonagricultural Emissions to Atmospheric Ammonia in a Chinese Megacity Y. Chang et al. 10.1021/acs.est.8b05984
- Source apportionment of PM2.5 across China using LOTOS-EUROS R. Timmermans et al. 10.1016/j.atmosenv.2017.06.003
- A temporal-spatial analysis and future trends of ammonia emissions in China H. Fu et al. 10.1016/j.scitotenv.2020.138897
- Ammonia Emissions from Mudflats of River, Lake, and Sea Y. Chang et al. 10.1021/acsearthspacechem.0c00017