Max Planck Institute for Chemistry, Biogeochemistry Dept., 55020 Mainz, Germany

now at: Richard Assmann Observatory Lindenberg, German Meteorological Service, Germany

Max Planck Institute for Chemistry, Biogeochemistry Dept., 55020 Mainz, Germany

now at: Agroscope ART, Air Pollution and Climate Group, 8046 Zürich, Switzerland

Max Planck Institute for Chemistry, Biogeochemistry Dept., 55020 Mainz, Germany

now at: United Nations Framework Convention on Climate Change, 53179 Bonn, Germany

Departamento de Meteorologia, Universidade Federal de Alagoas, Maceió, Brazil

University of Bayreuth, Micrometeorology Dept., 95440 Bayreuth, Germany

Max Planck Institute for Chemistry, Biogeochemistry Dept., 55020 Mainz, Germany

Max Planck Institute for Chemistry, Biogeochemistry Dept., 55020 Mainz, Germany