Articles | Volume 25, issue 14 
            
                
                    
            
            
            https://doi.org/10.5194/acp-25-7959-2025
                    © Author(s) 2025. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-25-7959-2025
                    © Author(s) 2025. This work is distributed under 
the Creative Commons Attribution 4.0 License.
                the Creative Commons Attribution 4.0 License.
Source-dependent optical properties and molecular characteristics of atmospheric brown carbon
Jinghao Zhai
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China
                                        
                                    Yin Zhang
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Pengfei Liu
                                            School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA 30332, USA
                                        
                                    Yujie Zhang
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Antai Zhang
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Yaling Zeng
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Baohua Cai
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Jingyi Zhang
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Chunbo Xing
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Honglong Yang
                                            Shenzhen National Climate Observatory, Meteorological Bureau of Shenzhen Municipality, Shenzhen 518040, China
                                        
                                    Xiaofei Wang
                                            Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China
                                        
                                    Jianhuai Ye
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Chen Wang
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Tzung-May Fu
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Huizhong Shen
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    Shu Tao
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
                                    
                                            Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
                                        
                                    
                                            Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, Shenzhen 518055, China
                                        
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Short summary
                    Our study shows that the optical properties of brown carbon depend on its source. Brown carbon from ozone pollution had the weakest light absorption but the strongest wavelength dependence, while biomass burning brown carbon showed the strongest absorption and the weakest wavelength dependence. Nitrogen-containing organic carbon compounds were identified as key light absorbers. These results improve understanding of brown carbon sources and help refine climate models.
                    Our study shows that the optical properties of brown carbon depend on its source. Brown carbon...
                    
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