Articles | Volume 25, issue 21
https://doi.org/10.5194/acp-25-15121-2025
© Author(s) 2025. This work is distributed under the Creative Commons Attribution 4.0 License.
Special issue:
High-resolution regional inversion reveals overestimation of anthropogenic methane emissions in China
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- Final revised paper (published on 07 Nov 2025)
- Supplement to the final revised paper
- Preprint (discussion started on 07 Jul 2025)
- Supplement to the preprint
Interactive discussion
Status: closed
Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor
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RC1: 'Comment on egusphere-2025-2669', Anonymous Referee #1, 24 Jul 2025
- AC1: 'Reply on RC1', Shuzhuang Feng, 28 Sep 2025
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RC2: 'Comment on egusphere-2025-2669', Anonymous Referee #2, 19 Aug 2025
- AC2: 'Reply on RC2', Shuzhuang Feng, 28 Sep 2025
Peer review completion
AR: Author's response | RR: Referee report | ED: Editor decision | EF: Editorial file upload
AR by Shuzhuang Feng on behalf of the Authors (28 Sep 2025)
Author's response
Author's tracked changes
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ED: Publish as is (06 Oct 2025) by Chris Wilson
AR by Shuzhuang Feng on behalf of the Authors (07 Oct 2025)
Feng et al. performed a high-resolution inversion to quantify methane emissions from China. The authors have employed nested WRF-CMAQ simulations, with particular fine resolution (9 km) over Shanxi, the major coal mining province in China. They found that the prior inventory severely overestimates coal mining emissions in North China. The study is overall well executed and clearly presented. I am happy to recommend publication of the manuscript after the following comments are addressed, mainly regarding clarification of the methodology.
Main comments:
1. The study discussed methane emissions from different sectors, but how the sector partitioning is done is not described. I'd suggest authors to provide further methodological details.
2. The authors have applied TROPOMI XCH4 L2 data. An earlier version of the TROPOMI data have shown substantial regional biases over East China, which may cause errors in the inversion. It would be good if the authors can have some discussion or conduct evaluation on this issue, for instance, using TCCON sites in China.
3. I do appreciate that the authors have performed evaluation for meteorology parameters against independent data, which most of existing studies have not done. This is crucial for characterizing model transport errors and understanding the difference between inversion systems. However, the discussion is overly simple. I'd suggest the authors to expand the results on meteorology evaluation (especially wind). In particular, the evaluation over the D02 domain provides crucial information because of the complex terrain in Shanxi.
4. The authors used the optimized emissions from the D01 inversion as prior emissions for the D02 inversion. This implies that the observations over D02 are used twice in the optimization of emissions. From the Bayesian standpoint, this is problematic as it leads to over-confidence in observations.
5. The paper in general lacks uncertainty characterization for emission flux estimates. For regions with limited observation coverage (e.g., Southern China), it is unclear to what degree the posterior estimates depend on prior estimates.
Minor suggestions:
L80: key source-> "point source scale" or "local scale"?
L95: unclear -> uncertain
L103: To my knowledge, IMI is not an operational inversion system, but more like open-source software. So it may be improper to characterize it as a US system. Similar issues may exist for other listed systems.
L188-189: Any quantitative estimates how much error it will incur for D01 and for D02 respectively, by deactivating the chemical oxidation?
L230: How do you specify the R matrix? Also explain specifically that R is an error covariance matrix for what.
L232: Ep: Power plant sources? Seems something copied from a CO2 study.
L234: No need to capitalize O in oil
L251: Would 1 day be too short for adequate observation constraint, if you assume that prior errors are independent from one day to the next (L272-273)?
Table 1: What do the last two columns (building, mature) stand for?
Table 1 and related discussion (e.g., L360): EDGAR v8.0 is used as prior information. Recent studies have shown that EDGAR has large errors in the spatial and seasonal distribution in rice emissions (Chen et al., 2025; Liang et al., 2024). I'd suggest the authors to briefly discuss the impact on emission quantification and sector attribution in Northeast and East China.
Chen et al.: Global Rice Paddy Inventory (GRPI): a high-resolution inventory of methane emissions from rice agriculture based on Landsat satellite inundation data, Earth's Future, 2025.
Liang et al.: Satellite-based Monitoring of Methane Emissions from China's Rice Hub, Environmental Science & Technology, 2024.
Table 2: Just a comment: The comparison with local observations, which are sensitive to emission adjustment, is valuable.