Secondary reactions of aromatics-derived oxygenated organic molecules lead to plentiful highly oxygenated organic molecules within an intraday OH exposure
Yuwei Wang,Chuang Li,Ying Zhang,Yueyang Li,Gan Yang,Xueyan Yang,Yizhen Wu,Lei Yao,Hefeng Zhang,and Lin Wang
Yuwei Wang
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Ying Zhang
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Yueyang Li
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Gan Yang
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Xueyan Yang
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Yizhen Wu
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China
State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation, Vehicle Emission Control Center of Ministry of Ecology and Environment, Chinese Research Academy of Environmental Sciences, Beijing 100012, China
Department of Environmental Science and Engineering, Jiangwan Campus, Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP), Fudan University, Shanghai 200438, China
Shanghai Institute of Pollution Control and Ecological Security, Shanghai 200092, China
IRDR International Center of Excellence on Risk Interconnectivity and Governance on Weather/Climate Extremes Impact and Public Health, Fudan University, Shanghai, China
National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Shanghai, China
Collaborative Innovation Center of Climate Change, Nanjing, 210023, China
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The formation and evolution mechanisms of aromatics-derived highly oxygenated organic molecules (HOMs) are essential to understand the formation of secondary organic aerosol pollution. Our conclusion highlights an underappreciated formation pathway of aromatics-derived HOMs and elucidates detailed formation mechanisms of certain HOMs, which advances our understanding of HOMs and potentially explains the existing gap between model prediction and ambient measurement of the HOMs' concentrations.
The formation and evolution mechanisms of aromatics-derived highly oxygenated organic molecules...