Articles | Volume 23, issue 9
https://doi.org/10.5194/acp-23-5251-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-5251-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
10 May 2023
Research article |
| 10 May 2023
| 10 May 2023
Sulfate formation via aerosol-phase SO2 oxidation by model biomass burning photosensitizers: 3,4-dimethoxybenzaldehyde, vanillin and syringaldehyde using single-particle mixing-state analysis
School of Energy and Environment, City University of Hong Kong, Hong Kong SAR 999077, China
Shenzhen Research Institute, City University of Hong Kong, Shenzhen 518057, China
Zhancong Liang
School of Energy and Environment, City University of Hong Kong, Hong Kong SAR 999077, China
Shenzhen Research Institute, City University of Hong Kong, Shenzhen 518057, China
Brix Raphael Go
School of Energy and Environment, City University of Hong Kong, Hong Kong SAR 999077, China
Shenzhen Research Institute, City University of Hong Kong, Shenzhen 518057, China
Rosemarie Ann Infante Cuevas
School of Energy and Environment, City University of Hong Kong, Hong Kong SAR 999077, China
Shenzhen Research Institute, City University of Hong Kong, Shenzhen 518057, China
Rongzhi Tang
School of Energy and Environment, City University of Hong Kong, Hong Kong SAR 999077, China
Shenzhen Research Institute, City University of Hong Kong, Shenzhen 518057, China
Mei Li
Institute of Mass Spectrometry and Atmospheric Environment, Guangdong Provincial Engineering Research Center for On-line Source Apportionment System of Air Pollution, Jinan University, Guangzhou 510632, China
Guangdong–Hong Kong–Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 510632, China
Chunlei Cheng
Institute of Mass Spectrometry and Atmospheric Environment, Guangdong Provincial Engineering Research Center for On-line Source Apportionment System of Air Pollution, Jinan University, Guangzhou 510632, China
Guangdong–Hong Kong–Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou 510632, China
Chak K. Chan
CORRESPONDING AUTHOR
School of Energy and Environment, City University of Hong Kong, Hong Kong SAR 999077, China
Shenzhen Research Institute, City University of Hong Kong, Shenzhen 518057, China
Low-Carbon and Climate Impact Research Centre of School of Energy and Environment, City University of Hong Kong, Hong Kong SAR 999077, China
current address: Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology, Thuwal, 23955-6900, Saudi Arabia
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Cited
17 citations as recorded by crossref.
- Insights into the seasonal characteristics of single particle aerosols in Chengdu based on SPAMS J. Zhang et al. 10.1016/j.jes.2024.01.018
- Enhanced Sulfate Formation through Synergistic Effects of Chlorine Chemistry and Photosensitization in Atmospheric Particles R. Zhang & C. Chan 10.1021/acsestair.3c00030
- Significantly Accelerated Photosensitized Formation of Atmospheric Sulfate at the Air–Water Interface of Microdroplets W. Wang et al. 10.1021/jacs.3c11892
- Enhanced sulfate formation in mixed biomass burning and sea-salt interactions mediated by photosensitization: effects of chloride, nitrogen-containing compounds, and atmospheric aging R. Tang et al. 10.5194/acp-25-425-2025
- Acidity of Atmospheric Waters Induces Enhanced H2O2 Production through Photosensitized Chemistry of Phenolic Substances Y. Xie et al. 10.1021/acsearthspacechem.4c00318
- Significantly surfactant-enhanced photochemical conversion of SO2 to sulfates on photosensitive substances H. Yang et al. 10.1016/j.jes.2024.10.014
- Aqueous Photosensitization of Syringaldehyde: Reactivity, Effects of Environmental Factors, and Formation of Brown Carbon Products F. Li et al. 10.1021/acsearthspacechem.4c00004
- Secondary aerosol formation in incense burning particles by O3 and OH oxidation via single particle mixing state analysis Z. Liang et al. 10.1016/j.scitotenv.2023.164942
- Measurements of Water-Soluble Ions in Particulate Matter 2.5 in Polish Rural Areas: Identifying Possible Sources D. Chyzhykov & B. Mathews 10.1007/s11270-024-07265-4
- Unequal toxic effects of size-segregated single particles emitted from typical industrial plants, vehicles, and road dust Q. Zhang et al. 10.1016/j.jhazmat.2024.136419
- Evaporation-Induced Transformations in Volatile Chemical Product-Derived Secondary Organic Aerosols: Browning Effects and Alterations in Oxidative Reactivity L. Zhou et al. 10.1021/acs.est.4c02316
- Complexities of Photosensitization in Atmospheric Particles Z. Liang et al. 10.1021/acsestair.4c00112
- Aqueous-Phase Photoreactions of Mixed Aromatic Carbonyl Photosensitizers Yield More Oxygenated, Oxidized, and less Light-Absorbing Secondary Organic Aerosol (SOA) than Single Systems B. Go et al. 10.1021/acs.est.3c10199
- Biomass-burning organic aerosols as a pool of atmospheric reactive triplets to drive multiphase sulfate formation Z. Liang et al. 10.1073/pnas.2416803121
- Strong electric field force at the air/water interface drives fast sulfate production in the atmosphere Y. Liu et al. 10.1016/j.chempr.2023.09.019
- Sulfate Formation by Photosensitization in Mixed Incense Burning–Sodium Chloride Particles: Effects of RH, Light Intensity, and Aerosol Aging R. Tang et al. 10.1021/acs.est.3c02225
- Heterogeneous photochemical uptake of SO2 on typical brown carbon species: A significant sulfate source H. Yang et al. 10.1016/j.atmosenv.2024.120425
17 citations as recorded by crossref.
- Insights into the seasonal characteristics of single particle aerosols in Chengdu based on SPAMS J. Zhang et al. 10.1016/j.jes.2024.01.018
- Enhanced Sulfate Formation through Synergistic Effects of Chlorine Chemistry and Photosensitization in Atmospheric Particles R. Zhang & C. Chan 10.1021/acsestair.3c00030
- Significantly Accelerated Photosensitized Formation of Atmospheric Sulfate at the Air–Water Interface of Microdroplets W. Wang et al. 10.1021/jacs.3c11892
- Enhanced sulfate formation in mixed biomass burning and sea-salt interactions mediated by photosensitization: effects of chloride, nitrogen-containing compounds, and atmospheric aging R. Tang et al. 10.5194/acp-25-425-2025
- Acidity of Atmospheric Waters Induces Enhanced H2O2 Production through Photosensitized Chemistry of Phenolic Substances Y. Xie et al. 10.1021/acsearthspacechem.4c00318
- Significantly surfactant-enhanced photochemical conversion of SO2 to sulfates on photosensitive substances H. Yang et al. 10.1016/j.jes.2024.10.014
- Aqueous Photosensitization of Syringaldehyde: Reactivity, Effects of Environmental Factors, and Formation of Brown Carbon Products F. Li et al. 10.1021/acsearthspacechem.4c00004
- Secondary aerosol formation in incense burning particles by O3 and OH oxidation via single particle mixing state analysis Z. Liang et al. 10.1016/j.scitotenv.2023.164942
- Measurements of Water-Soluble Ions in Particulate Matter 2.5 in Polish Rural Areas: Identifying Possible Sources D. Chyzhykov & B. Mathews 10.1007/s11270-024-07265-4
- Unequal toxic effects of size-segregated single particles emitted from typical industrial plants, vehicles, and road dust Q. Zhang et al. 10.1016/j.jhazmat.2024.136419
- Evaporation-Induced Transformations in Volatile Chemical Product-Derived Secondary Organic Aerosols: Browning Effects and Alterations in Oxidative Reactivity L. Zhou et al. 10.1021/acs.est.4c02316
- Complexities of Photosensitization in Atmospheric Particles Z. Liang et al. 10.1021/acsestair.4c00112
- Aqueous-Phase Photoreactions of Mixed Aromatic Carbonyl Photosensitizers Yield More Oxygenated, Oxidized, and less Light-Absorbing Secondary Organic Aerosol (SOA) than Single Systems B. Go et al. 10.1021/acs.est.3c10199
- Biomass-burning organic aerosols as a pool of atmospheric reactive triplets to drive multiphase sulfate formation Z. Liang et al. 10.1073/pnas.2416803121
- Strong electric field force at the air/water interface drives fast sulfate production in the atmosphere Y. Liu et al. 10.1016/j.chempr.2023.09.019
- Sulfate Formation by Photosensitization in Mixed Incense Burning–Sodium Chloride Particles: Effects of RH, Light Intensity, and Aerosol Aging R. Tang et al. 10.1021/acs.est.3c02225
- Heterogeneous photochemical uptake of SO2 on typical brown carbon species: A significant sulfate source H. Yang et al. 10.1016/j.atmosenv.2024.120425
Latest update: 01 Apr 2025
Short summary
This study reveals the sulfate formation in photosensitized particles from biomass burning under UV and SO2, of which the relative atmospheric importance in sulfate production was qualitatively compared to nitrate photolysis. On the basis of single-particle aerosol mass spectrometry measurements, the number percentage of sulfate-containing particles and relative peak area of sulfate in single-particle spectra exhibited a descending order of 3,4-dimethoxybenzaldehyde > vanillin > syringaldehyde.
This study reveals the sulfate formation in photosensitized particles from biomass burning under...
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