Influence of acidity on liquid–liquid phase transitions of mixed secondary organic aerosol (SOA) proxy–inorganic aerosol droplets
Yueling Chen,Xiangyu Pei,Huichao Liu,Yikan Meng,Zhengning Xu,Fei Zhang,Chun Xiong,Thomas C. Preston,and Zhibin Wang
Yueling Chen
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
Xiangyu Pei
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
Huichao Liu
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
Yikan Meng
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
Zhengning Xu
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
Chun Xiong
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
Thomas C. Preston
Department of Atmospheric and Oceanic Sciences, McGill University, 805 Sherbrooke Street West, Montréal, Quebec
H3A 0B9, Canada
Department of
Chemistry, McGill University, 805 Sherbrooke Street West, Montréal, Quebec
H3A 0B9, Canada
Zhejiang Provincial Key Laboratory of Organic Pollution Process and
Control, MOE Key Laboratory of Environment Remediation and Ecological
Health, College of Environmental and Resource Sciences, Zhejiang University,
Hangzhou 310058, China
ZJU-Hangzhou Global Scientific and Technological Innovation Center,
Zhejiang University, Hangzhou 311215, China
Viewed
Total article views: 2,335 (including HTML, PDF, and XML)
HTML
PDF
XML
Total
Supplement
BibTeX
EndNote
1,784
481
70
2,335
158
121
118
HTML: 1,784
PDF: 481
XML: 70
Total: 2,335
Supplement: 158
BibTeX: 121
EndNote: 118
Views and downloads (calculated since 21 Apr 2023)
Cumulative views and downloads
(calculated since 21 Apr 2023)
Total article views: 1,758 (including HTML, PDF, and XML)
HTML
PDF
XML
Total
Supplement
BibTeX
EndNote
1,363
349
46
1,758
109
112
106
HTML: 1,363
PDF: 349
XML: 46
Total: 1,758
Supplement: 109
BibTeX: 112
EndNote: 106
Views and downloads (calculated since 14 Sep 2023)
Cumulative views and downloads
(calculated since 14 Sep 2023)
Total article views: 577 (including HTML, PDF, and XML)
HTML
PDF
XML
Total
Supplement
BibTeX
EndNote
421
132
24
577
49
9
12
HTML: 421
PDF: 132
XML: 24
Total: 577
Supplement: 49
BibTeX: 9
EndNote: 12
Views and downloads (calculated since 21 Apr 2023)
Cumulative views and downloads
(calculated since 21 Apr 2023)
Viewed (geographical distribution)
Total article views: 2,335 (including HTML, PDF, and XML)
Thereof 2,298 with geography defined
and 37 with unknown origin.
Total article views: 1,758 (including HTML, PDF, and XML)
Thereof 1,733 with geography defined
and 25 with unknown origin.
Total article views: 577 (including HTML, PDF, and XML)
Thereof 565 with geography defined
and 12 with unknown origin.
The impact of acidity on the phase transition behavior of levitated aerosol particles was examined. Our results revealed that lower acidity decreases the separation relative humidity of aerosol droplets mixed with ammonium sulfate and secondary organic aerosol proxy. Our research suggests that in real atmospheric conditions, with the high acidity found in many ambient aerosol particles, droplets encounter heightened impediments to phase separation and tend to display a homogeneous structure.
The impact of acidity on the phase transition behavior of levitated aerosol particles was...
