Articles | Volume 22, issue 12
https://doi.org/10.5194/acp-22-8343-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-8343-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
A new assessment of global and regional budgets, fluxes, and lifetimes of atmospheric reactive N and S gases and aerosols
School of Chemistry, University of Edinburgh, Joseph Black Building,
David Brewster Road, Edinburgh EH9 3FJ, UK
UK Centre for Ecology & Hydrology, Bush Estate, Penicuik,
Midlothian EH26 0QB, UK
Massimo Vieno
UK Centre for Ecology & Hydrology, Bush Estate, Penicuik,
Midlothian EH26 0QB, UK
David S. Stevenson
School of GeoSciences, University of Edinburgh, Crew Building,
Alexander Crum Brown Road, Edinburgh EH9 3FF, UK
Peter Wind
The Norwegian Meteorological Institute, Henrik Mohns Plass 1, 0313
Oslo, Norway
School of Chemistry, University of Edinburgh, Joseph Black Building,
David Brewster Road, Edinburgh EH9 3FJ, UK
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Total article views: 3,780 (including HTML, PDF, and XML)
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Cited
20 citations as recorded by crossref.
- Data fusion of modelled and measured deposition in the US and Canada, part II: Dry deposition of sulfur, nitrogen and ozone A. Robichaud et al. https://doi.org/10.1016/j.atmosenv.2025.121656
- Effectiveness of agricultural interventions to minimise the health impacts of air pollution: a synopsis from a mixed method study H. Cowie et al. https://doi.org/10.3310/THGD2153
- Changing patterns of global nitrogen deposition driven by socio-economic development J. Zhu et al. https://doi.org/10.1038/s41467-024-55606-y
- Carbon dynamics and potential nutrient limitations in an oak forest under experimental canopy nitrogen deposition D. Minikaev et al. https://doi.org/10.1016/j.scitotenv.2025.180027
- Global atmospheric inversion of the anthropogenic NH3 emissions over 2019–2022 using the LMDZ-INCA chemistry transport model and the IASI NH3 observations P. Kumar et al. https://doi.org/10.5194/acp-25-12379-2025
- Lichens as spatially transferable bioindicators for monitoring nitrogen pollution J. Delves et al. https://doi.org/10.1016/j.envpol.2023.121575
- The influence of ammonia emission inventories on size-resolved global atmospheric aerosol composition and acidity X. Wang et al. https://doi.org/10.5194/acp-25-10559-2025
- Spatial patterns of environmental injustice in social vulnerability and ambient dust levels across Australia S. Nyadanu et al. https://doi.org/10.1088/1748-9326/ae4d5d
- Significant contributions of combustion-related sources to ammonia emissions Z. Chen et al. https://doi.org/10.1038/s41467-022-35381-4
- Evaluating present-day and future impacts of agricultural ammonia emissions on atmospheric chemistry and climate M. Beaudor et al. https://doi.org/10.5194/acp-25-2017-2025
- Unraveling the intra-annual pattern of wet and dry nitrogen deposition in contrasting temperate regions Y. Tian et al. https://doi.org/10.1016/j.atmosenv.2026.122082
- Anthropogenic transformation and flow of N in China's fertilizer system Y. Chai et al. https://doi.org/10.1016/j.jclepro.2026.148049
- "Environmental, health and economic benefits of emission reduction in residential sector – A case study for Poland" M. Werner et al. https://doi.org/10.1016/j.apr.2024.102360
- Changes in atmospheric oxidants teleconnect biomass burning and ammonium nitrate formation D. Tan et al. https://doi.org/10.1038/s41612-025-01150-5
- Implementation and evaluation of updated photolysis rates in the EMEP MSC-W chemistry-transport model using Cloud-J v7.3e W. van Caspel et al. https://doi.org/10.5194/gmd-16-7433-2023
- Impact of agricultural interventions on ammonia emissions and on PM2.5 concentrations in the UK: a local and regional modelling study M. Pommier et al. https://doi.org/10.5194/ar-4-189-2026
- Geographical Distribution of Atmospheric Nitrogen Deposition in China and Its Response to Emission Control Policy Z. Wen et al. https://doi.org/10.1007/s11769-024-1471-4
- The Impact of Farming Mitigation Measures on Ammonia Concentrations and Nitrogen Deposition in the UK M. Pommier et al. https://doi.org/10.3390/atmos16040353
- Global sensitivities of reactive N and S gas and particle concentrations and deposition to precursor emissions reductions Y. Ge et al. https://doi.org/10.5194/acp-23-6083-2023
- Long-term regional trends of nitrogen and sulfur deposition in the United States from 2002 to 2017 S. Benish et al. https://doi.org/10.5194/acp-22-12749-2022
20 citations as recorded by crossref.
- Data fusion of modelled and measured deposition in the US and Canada, part II: Dry deposition of sulfur, nitrogen and ozone A. Robichaud et al. https://doi.org/10.1016/j.atmosenv.2025.121656
- Effectiveness of agricultural interventions to minimise the health impacts of air pollution: a synopsis from a mixed method study H. Cowie et al. https://doi.org/10.3310/THGD2153
- Changing patterns of global nitrogen deposition driven by socio-economic development J. Zhu et al. https://doi.org/10.1038/s41467-024-55606-y
- Carbon dynamics and potential nutrient limitations in an oak forest under experimental canopy nitrogen deposition D. Minikaev et al. https://doi.org/10.1016/j.scitotenv.2025.180027
- Global atmospheric inversion of the anthropogenic NH3 emissions over 2019–2022 using the LMDZ-INCA chemistry transport model and the IASI NH3 observations P. Kumar et al. https://doi.org/10.5194/acp-25-12379-2025
- Lichens as spatially transferable bioindicators for monitoring nitrogen pollution J. Delves et al. https://doi.org/10.1016/j.envpol.2023.121575
- The influence of ammonia emission inventories on size-resolved global atmospheric aerosol composition and acidity X. Wang et al. https://doi.org/10.5194/acp-25-10559-2025
- Spatial patterns of environmental injustice in social vulnerability and ambient dust levels across Australia S. Nyadanu et al. https://doi.org/10.1088/1748-9326/ae4d5d
- Significant contributions of combustion-related sources to ammonia emissions Z. Chen et al. https://doi.org/10.1038/s41467-022-35381-4
- Evaluating present-day and future impacts of agricultural ammonia emissions on atmospheric chemistry and climate M. Beaudor et al. https://doi.org/10.5194/acp-25-2017-2025
- Unraveling the intra-annual pattern of wet and dry nitrogen deposition in contrasting temperate regions Y. Tian et al. https://doi.org/10.1016/j.atmosenv.2026.122082
- Anthropogenic transformation and flow of N in China's fertilizer system Y. Chai et al. https://doi.org/10.1016/j.jclepro.2026.148049
- "Environmental, health and economic benefits of emission reduction in residential sector – A case study for Poland" M. Werner et al. https://doi.org/10.1016/j.apr.2024.102360
- Changes in atmospheric oxidants teleconnect biomass burning and ammonium nitrate formation D. Tan et al. https://doi.org/10.1038/s41612-025-01150-5
- Implementation and evaluation of updated photolysis rates in the EMEP MSC-W chemistry-transport model using Cloud-J v7.3e W. van Caspel et al. https://doi.org/10.5194/gmd-16-7433-2023
- Impact of agricultural interventions on ammonia emissions and on PM2.5 concentrations in the UK: a local and regional modelling study M. Pommier et al. https://doi.org/10.5194/ar-4-189-2026
- Geographical Distribution of Atmospheric Nitrogen Deposition in China and Its Response to Emission Control Policy Z. Wen et al. https://doi.org/10.1007/s11769-024-1471-4
- The Impact of Farming Mitigation Measures on Ammonia Concentrations and Nitrogen Deposition in the UK M. Pommier et al. https://doi.org/10.3390/atmos16040353
- Global sensitivities of reactive N and S gas and particle concentrations and deposition to precursor emissions reductions Y. Ge et al. https://doi.org/10.5194/acp-23-6083-2023
- Long-term regional trends of nitrogen and sulfur deposition in the United States from 2002 to 2017 S. Benish et al. https://doi.org/10.5194/acp-22-12749-2022
Saved (final revised paper)
Latest update: 09 Jun 2026
Short summary
Reactive N and S gases and aerosols are critical determinants of air quality. We report a comprehensive analysis of the concentrations, wet and dry deposition, fluxes, and lifetimes of these species globally as well as for 10 world regions. We used the EMEP MSC-W model coupled with WRF meteorology and 2015 global emissions. Our work demonstrates the substantial regional variation in these quantities and the need for modelling to simulate atmospheric responses to precursor emissions.
Reactive N and S gases and aerosols are critical determinants of air quality. We report a...
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