Articles | Volume 22, issue 7
https://doi.org/10.5194/acp-22-4539-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-4539-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Apr 2022
Research article |
| 08 Apr 2022
| 08 Apr 2022
The formation and mitigation of nitrate pollution: comparison between urban and suburban environments
Suxia Yang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Yuwen Peng
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Shan Huang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Wei Chen
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Weiwei Hu
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Chenglei Pei
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou, 510640,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Guangzhou Ecological and Environmental Monitoring Center of Guangdong Province, Guangzhou 510060, China
Jun Zhou
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
David D. Parrish
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Wenjie Wang
State Joint Key Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Xianjun He
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Chunlei Cheng
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Institute of Mass Spectrometry and Atmospheric Environment, Guangdong Provincial Engineering Research Center for on-line Source Apportionment
System of Air Pollution, Jinan University, Guangzhou 510632, China
Xiao-Bing Li
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Xiaoyun Yang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Yu Song
State Joint Key Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Haichao Wang
School of Atmospheric Sciences, Sun Yat-Sen University, Guangzhou
510275, China
Jipeng Qi
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Baolin Wang
School of Environmental Science and Engineering, Qilu University of Technology, Jinan 250353, China
Chen Wang
School of Environmental Science and Engineering, Qilu University of Technology, Jinan 250353, China
Chaomin Wang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Zelong Wang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Tiange Li
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
E Zheng
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Sihang Wang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Caihong Wu
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Mingfu Cai
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Chenshuo Ye
State Joint Key Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Wei Song
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Peng Cheng
Institute of Mass Spectrometry and Atmospheric Environment, Guangdong Provincial Engineering Research Center for on-line Source Apportionment
System of Air Pollution, Jinan University, Guangzhou 510632, China
Duohong Chen
Guangzhou Ecological and Environmental Monitoring Center of Guangdong Province, Guangzhou 510060, China
Xinming Wang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Zhanyi Zhang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Xuemei Wang
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Junyu Zheng
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
Min Shao
CORRESPONDING AUTHOR
Institute for Environmental and Climate Research, Jinan University,
Guangzhou 511443, China
Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation
for Environmental Quality, Jinan University, Guangzhou 511443, China
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- Regime‐Dependence of Nocturnal Nitrate Formation via N2O5 Hydrolysis and Its Implication for Mitigating Nitrate Pollution P. Ma et al. 10.1029/2023GL106183
- Nighttime ozone in the lower boundary layer: insights from 3-year tower-based measurements in South China and regional air quality modeling G. He et al. 10.5194/acp-23-13107-2023
- Control of fine particulate nitrate during severe winter haze in “2+26” cities C. Qin et al. 10.1016/j.jes.2022.12.016
- Assessment of long tubing in measuring atmospheric trace gases: applications on tall towers X. Li et al. 10.1039/D2EA00110A
- Fast nitrate formation aloft supported by typical synoptic weather patterns and complex terrain in the North China Plain C. Qin et al. 10.1016/j.atmosenv.2023.120170
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- Contribution of anthropogenic emission changes to the evolution of PM2.5 concentrations and composition in the Pearl River Delta during the period of 2006–2020 J. Zhang et al. 10.1016/j.atmosenv.2023.120228
- The significant contribution of nitrate to a severe haze event in the winter of Guangzhou, China C. Cheng et al. 10.1016/j.scitotenv.2023.168582
- Impact of aging on the sources, volatility, and viscosity of organic aerosols in Chinese outflows T. Feng et al. 10.5194/acp-23-611-2023
- Insight into Secondary Inorganic Aerosol (SIA) production enhanced by domestic ozone using a machine learning technique G. Lin et al. 10.1016/j.atmosenv.2023.120194
- Ozone pollution mitigation strategy informed by long-term trends of atmospheric oxidation capacity W. Wang et al. 10.1038/s41561-023-01334-9
- Pollution characteristics, source appointment and environmental effect of oxygenated volatile organic compounds in Guangdong-Hong Kong-Macao Greater Bay Area: Implication for air quality management G. Liu et al. 10.1016/j.scitotenv.2024.170836
- Concurrent measurements of nitrate at urban and suburban sites identify local nitrate formation as a driver for urban episodic PM2.5 pollution J. Li et al. 10.1016/j.scitotenv.2023.165351
- Achievements and challenges in improving air quality in China: Analysis of the long-term trends from 2014 to 2022 H. Zheng et al. 10.1016/j.envint.2023.108361
- Double-Edged Role of VOCs Reduction in Nitrate Formation: Insights from Observations during the China International Import Expo 2018 Y. Zhang et al. 10.1021/acs.est.3c04629
- Short-term source apportionment of fine particulate matter with time-dependent profiles using SoFi Pro: exploring the reliability of rolling positive matrix factorization (PMF) applied to bihourly molecular and elemental tracer data Q. Wang et al. 10.5194/acp-24-475-2024
- Measurement report: Atmospheric nitrate radical chemistry in the South China Sea influenced by the urban outflow of the Pearl River Delta J. Wang et al. 10.5194/acp-24-977-2024
- Wintertime fine aerosol particles composition and its evolution in two megacities of southern and northern China Y. Cheng et al. 10.1016/j.scitotenv.2023.169778
- Implications of differences between recent anthropogenic aerosol emission inventories for diagnosed AOD and radiative forcing from 1990 to 2019 M. Lund et al. 10.5194/acp-23-6647-2023
- A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz S. Atabakhsh et al. 10.5194/acp-23-6963-2023
- Secondary aerosol formation drives atmospheric particulate matter pollution over megacities (Beijing and Seoul) in East Asia Y. Qiu et al. 10.1016/j.atmosenv.2023.119702
- Formation and impacts of nitryl chloride in Pearl River Delta H. Wang et al. 10.5194/acp-22-14837-2022
- New insights into the formation of ammonium nitrate from a physical and chemical level perspective Y. Wei et al. 10.1007/s11783-023-1737-6
- Photolysis frequency of nitrophenols derived from ambient measurements Y. Peng et al. 10.1016/j.scitotenv.2023.161810
- Box Model Applications for Secondary Inorganic Aerosol: A Review Focused on Nitrate Formation S. Park 10.5572/KOSAE.2024.40.1.1
- Insights into characteristics and formation mechanisms of secondary organic aerosols in the Guangzhou urban area M. Zhai et al. 10.5194/acp-23-5119-2023
28 citations as recorded by crossref.
- Observational Evidence of the Vertical Exchange of Ozone within the Urban Planetary Boundary Layer in Shanghai, China Y. Gu et al. 10.3390/atmos15030248
- Regime‐Dependence of Nocturnal Nitrate Formation via N2O5 Hydrolysis and Its Implication for Mitigating Nitrate Pollution P. Ma et al. 10.1029/2023GL106183
- Nighttime ozone in the lower boundary layer: insights from 3-year tower-based measurements in South China and regional air quality modeling G. He et al. 10.5194/acp-23-13107-2023
- Control of fine particulate nitrate during severe winter haze in “2+26” cities C. Qin et al. 10.1016/j.jes.2022.12.016
- Assessment of long tubing in measuring atmospheric trace gases: applications on tall towers X. Li et al. 10.1039/D2EA00110A
- Fast nitrate formation aloft supported by typical synoptic weather patterns and complex terrain in the North China Plain C. Qin et al. 10.1016/j.atmosenv.2023.120170
- High-time-resolution chemical composition and source apportionment of PM2.5 in northern Chinese cities: implications for policy Y. Zhang et al. 10.5194/acp-23-9455-2023
- A roadmap to estimating agricultural ammonia volatilization over Europe using satellite observations and simulation data R. Abeed et al. 10.5194/acp-23-12505-2023
- Contribution of anthropogenic emission changes to the evolution of PM2.5 concentrations and composition in the Pearl River Delta during the period of 2006–2020 J. Zhang et al. 10.1016/j.atmosenv.2023.120228
- The significant contribution of nitrate to a severe haze event in the winter of Guangzhou, China C. Cheng et al. 10.1016/j.scitotenv.2023.168582
- Impact of aging on the sources, volatility, and viscosity of organic aerosols in Chinese outflows T. Feng et al. 10.5194/acp-23-611-2023
- Insight into Secondary Inorganic Aerosol (SIA) production enhanced by domestic ozone using a machine learning technique G. Lin et al. 10.1016/j.atmosenv.2023.120194
- Ozone pollution mitigation strategy informed by long-term trends of atmospheric oxidation capacity W. Wang et al. 10.1038/s41561-023-01334-9
- Pollution characteristics, source appointment and environmental effect of oxygenated volatile organic compounds in Guangdong-Hong Kong-Macao Greater Bay Area: Implication for air quality management G. Liu et al. 10.1016/j.scitotenv.2024.170836
- Concurrent measurements of nitrate at urban and suburban sites identify local nitrate formation as a driver for urban episodic PM2.5 pollution J. Li et al. 10.1016/j.scitotenv.2023.165351
- Achievements and challenges in improving air quality in China: Analysis of the long-term trends from 2014 to 2022 H. Zheng et al. 10.1016/j.envint.2023.108361
- Double-Edged Role of VOCs Reduction in Nitrate Formation: Insights from Observations during the China International Import Expo 2018 Y. Zhang et al. 10.1021/acs.est.3c04629
- Short-term source apportionment of fine particulate matter with time-dependent profiles using SoFi Pro: exploring the reliability of rolling positive matrix factorization (PMF) applied to bihourly molecular and elemental tracer data Q. Wang et al. 10.5194/acp-24-475-2024
- Measurement report: Atmospheric nitrate radical chemistry in the South China Sea influenced by the urban outflow of the Pearl River Delta J. Wang et al. 10.5194/acp-24-977-2024
- Wintertime fine aerosol particles composition and its evolution in two megacities of southern and northern China Y. Cheng et al. 10.1016/j.scitotenv.2023.169778
- Implications of differences between recent anthropogenic aerosol emission inventories for diagnosed AOD and radiative forcing from 1990 to 2019 M. Lund et al. 10.5194/acp-23-6647-2023
- A 1-year aerosol chemical speciation monitor (ACSM) source analysis of organic aerosol particle contributions from anthropogenic sources after long-range transport at the TROPOS research station Melpitz S. Atabakhsh et al. 10.5194/acp-23-6963-2023
- Secondary aerosol formation drives atmospheric particulate matter pollution over megacities (Beijing and Seoul) in East Asia Y. Qiu et al. 10.1016/j.atmosenv.2023.119702
- Formation and impacts of nitryl chloride in Pearl River Delta H. Wang et al. 10.5194/acp-22-14837-2022
- New insights into the formation of ammonium nitrate from a physical and chemical level perspective Y. Wei et al. 10.1007/s11783-023-1737-6
- Photolysis frequency of nitrophenols derived from ambient measurements Y. Peng et al. 10.1016/j.scitotenv.2023.161810
- Box Model Applications for Secondary Inorganic Aerosol: A Review Focused on Nitrate Formation S. Park 10.5572/KOSAE.2024.40.1.1
- Insights into characteristics and formation mechanisms of secondary organic aerosols in the Guangzhou urban area M. Zhai et al. 10.5194/acp-23-5119-2023
Latest update: 24 Apr 2024
Short summary
We use a model constrained using observations to study the formation of nitrate aerosol in and downwind of a representative megacity. We found different contributions of various chemical reactions to ground-level nitrate concentrations between urban and suburban regions. We also show that controlling VOC emissions are effective for decreasing nitrate formation in both urban and regional environments, although VOCs are not direct precursors of nitrate aerosol.
We use a model constrained using observations to study the formation of nitrate aerosol in and...
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