Articles | Volume 22, issue 20
https://doi.org/10.5194/acp-22-13607-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-13607-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Oct 2022
Research article |
| 20 Oct 2022
| 20 Oct 2022
Chemical analysis of the Asian tropopause aerosol layer (ATAL) with emphasis on secondary aerosol particles using aircraft-based in situ aerosol mass spectrometry
Oliver Appel
Max Planck Institute for Chemistry, Mainz, Germany
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
Franziska Köllner
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
Antonis Dragoneas
Max Planck Institute for Chemistry, Mainz, Germany
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
Andreas Hünig
Max Planck Institute for Chemistry, Mainz, Germany
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
Sergej Molleker
Max Planck Institute for Chemistry, Mainz, Germany
Hans Schlager
Deutsches Zentrum für Luft- und Raumfahrt (DLR), Institut für Physik der Atmosphäre, Oberpfaffenhofen, Germany
Christoph Mahnke
Max Planck Institute for Chemistry, Mainz, Germany
now at: Institute of Energy and Climate Research (IEK-8), Forschungszentrum Jülich GmbH, Jülich, Germany
Ralf Weigel
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
Max Port
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
now at: Montessori Zentrum Hofheim, Germany
Christiane Schulz
Max Planck Institute for Chemistry, Mainz, Germany
now at: Leibniz-Zentrum für Agrarlandschaftsforschung, Müncheberg, Germany
Frank Drewnick
Max Planck Institute for Chemistry, Mainz, Germany
Bärbel Vogel
Institute of Energy and Climate Research (IEK-7), Forschungszentrum Jülich, Jülich, Germany
Fred Stroh
Institute of Energy and Climate Research (IEK-7), Forschungszentrum Jülich, Jülich, Germany
Stephan Borrmann
CORRESPONDING AUTHOR
Max Planck Institute for Chemistry, Mainz, Germany
Institute for Atmospheric Physics, Johannes Gutenberg University, Mainz, Germany
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- Evaluation of vertical transport in ERA5 and ERA-Interim reanalysis using high-altitude aircraft measurements in the Asian summer monsoon 2017 B. Vogel et al. 10.5194/acp-24-317-2024
- Investigating the convective transport possibilities of lower-atmospheric pollutants to the UTLS region using rainwater and aerosol chemical characterization C. Jain et al. 10.1016/j.apr.2024.102225
- The impact of ammonia on particle formation in the Asian Tropopause Aerosol Layer C. Xenofontos et al. 10.1038/s41612-024-00758-3
- Characterization of refractory aerosol particles collected in the tropical upper troposphere–lower stratosphere (UTLS) within the Asian tropopause aerosol layer (ATAL) M. Ebert et al. 10.5194/acp-24-4771-2024
- The influence of extratropical cross-tropopause mixing on the correlation between ozone and sulfate aerosol in the lowermost stratosphere P. Joppe et al. 10.5194/acp-24-7499-2024
- Long range transport of South and East Asian anthropogenic aerosols counteracting Arctic warming S. Fadnavis et al. 10.1038/s41612-024-00633-1
- A multi-scenario Lagrangian trajectory analysis to identify source regions of the Asian tropopause aerosol layer on the Indian subcontinent in August 2016 J. Clemens et al. 10.5194/acp-24-763-2024
- Does the Asian summer monsoon play a role in the stratospheric aerosol budget of the Arctic? S. Graßl et al. 10.5194/acp-24-7535-2024
- Role of deep convection and dynamics on the tracer distribution in the upper troposphere and lower stratosphere region during active and break phases of the Asian summer monsoon P. Satheesh Chandran & S. Sunilkumar 10.1007/s00382-023-07004-1
4 citations as recorded by crossref.
- Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques A. Hünig et al. 10.5194/amt-15-2889-2022
- Global distribution of Asian, Middle Eastern, and North African dust simulated by CESM1/CARMA S. Lian et al. 10.5194/acp-22-13659-2022
- The realization of autonomous, aircraft-based, real-time aerosol mass spectrometry in the upper troposphere and lower stratosphere A. Dragoneas et al. 10.5194/amt-15-5719-2022
- Abundant Nitrate and Nitric Acid Aerosol in the Upper Troposphere and Lower Stratosphere P. Yu et al. 10.1029/2022GL100258
Latest update: 20 Nov 2024
Short summary
This paper clarifies the chemical composition of the Asian tropopause aerosol layer (ATAL) by means of airborne in situ aerosol mass spectrometry (AMS). Ammonium nitrate and organics are found to significantly contribute to the particle layer, while sulfate does not show a layered structure. An analysis of the single-particle mass spectra suggests that secondary particle formation and subsequent growth dominate the particle composition, rather than condensation on pre-existing primary particles.
This paper clarifies the chemical composition of the Asian tropopause aerosol layer (ATAL) by...
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