Articles | Volume 22, issue 15
https://doi.org/10.5194/acp-22-10077-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-10077-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
05 Aug 2022
Research article |
| 05 Aug 2022
Seasonal variation in oxygenated organic molecules in urban Beijing and their contribution to secondary organic aerosol
Yishuo Guo
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Joint International Research Laboratory of Atmospheric and Earth
System Research, School of Atmospheric Sciences, Nanjing University, Nanjing, China
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Yuliang Liu
Joint International Research Laboratory of Atmospheric and Earth
System Research, School of Atmospheric Sciences, Nanjing University, Nanjing, China
Xiaohui Qiao
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, China
Feixue Zheng
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Ying Zhang
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Ying Zhou
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Chang Li
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Xiaolong Fan
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Zhuohui Lin
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Zemin Feng
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Yusheng Zhang
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Penggang Zheng
Division of Environment and Sustainability, The Hong Kong University of Science and Technology, Hong Kong SAR, China
Department of Civil and Environmental Engineering, The Hong Kong
Polytechnic University, Hong Kong SAR, China
Linhui Tian
Department of Civil and Environmental Engineering, Faculty of Science and Technology, University of Macau, Taipa, Macau SAR, China
Wei Nie
Joint International Research Laboratory of Atmospheric and Earth
System Research, School of Atmospheric Sciences, Nanjing University, Nanjing, China
Division of Environment and Sustainability, The Hong Kong University of Science and Technology, Hong Kong SAR, China
Dandan Huang
State Environmental Protection Key Laboratory of Formation and
Prevention of Urban Air Pollution Complex, Shanghai Academy of Environmental
Sciences, Shanghai, China
Kaspar R. Daellenbach
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Lubna Dada
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, Switzerland
Federico Bianchi
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Jingkun Jiang
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing, China
Yongchun Liu
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Veli-Matti Kerminen
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Markku Kulmala
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology, Beijing, China
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
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Cited
9 citations as recorded by crossref.
- Exploring condensable organic vapors and their co-occurrence with PM2.5 and O3 in winter in Eastern China Y. Liu et al. 10.1039/D2EA00143H
- Impact of urbanization on gas-phase pollutant concentrations: a regional-scale, model-based analysis of the contributing factors P. Huszar et al. 10.5194/acp-22-12647-2022
- Molecular Characterization of Oxygenated Organic Molecules and Their Dominating Roles in Particle Growth in Hong Kong P. Zheng et al. 10.1021/acs.est.2c09252
- New Particle Formation Occurrence in the Urban Atmosphere of Beijing During 2013–2020 D. Shang et al. 10.1029/2022JD038334
- Enigma of Urban Gaseous Oxygenated Organic Molecules: Precursor Type, Role of NOx, and Degree of Oxygenation L. Tian et al. 10.1021/acs.est.2c05047
- Underestimated Contribution of Heavy Aromatics to Secondary Organic Aerosol Revealed by Comparative Assessments Using New and Traditional Methods L. Tian et al. 10.1021/acsearthspacechem.2c00252
- Measurement report: The 4-year variability and influence of the Winter Olympics and other special events on air quality in urban Beijing during wintertime Y. Guo et al. 10.5194/acp-23-6663-2023
- Recent advances in mass spectrometry techniques for atmospheric chemistry research on molecular‐level W. Zhang et al. 10.1002/mas.21857
- Field Detection of Highly Oxygenated Organic Molecules in Shanghai by Chemical Ionization–Orbitrap Y. Zhang et al. 10.1021/acs.est.1c08346
8 citations as recorded by crossref.
- Exploring condensable organic vapors and their co-occurrence with PM2.5 and O3 in winter in Eastern China Y. Liu et al. 10.1039/D2EA00143H
- Impact of urbanization on gas-phase pollutant concentrations: a regional-scale, model-based analysis of the contributing factors P. Huszar et al. 10.5194/acp-22-12647-2022
- Molecular Characterization of Oxygenated Organic Molecules and Their Dominating Roles in Particle Growth in Hong Kong P. Zheng et al. 10.1021/acs.est.2c09252
- New Particle Formation Occurrence in the Urban Atmosphere of Beijing During 2013–2020 D. Shang et al. 10.1029/2022JD038334
- Enigma of Urban Gaseous Oxygenated Organic Molecules: Precursor Type, Role of NOx, and Degree of Oxygenation L. Tian et al. 10.1021/acs.est.2c05047
- Underestimated Contribution of Heavy Aromatics to Secondary Organic Aerosol Revealed by Comparative Assessments Using New and Traditional Methods L. Tian et al. 10.1021/acsearthspacechem.2c00252
- Measurement report: The 4-year variability and influence of the Winter Olympics and other special events on air quality in urban Beijing during wintertime Y. Guo et al. 10.5194/acp-23-6663-2023
- Recent advances in mass spectrometry techniques for atmospheric chemistry research on molecular‐level W. Zhang et al. 10.1002/mas.21857
1 citations as recorded by crossref.
Latest update: 03 Oct 2023
Short summary
Gaseous oxygenated organic molecules (OOMs) are able to form atmospheric aerosols, which will impact on human health and climate change. Here, we find that OOMs in urban Beijing are dominated by anthropogenic sources, i.e. aromatic (29 %–41 %) and aliphatic (26 %–41 %) OOMs. They are also the main contributors to the condensational growth of secondary organic aerosols (SOAs). Therefore, the restriction on anthropogenic VOCs is crucial for the reduction of SOAs and haze formation.
Gaseous oxygenated organic molecules (OOMs) are able to form atmospheric aerosols, which will...
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