Articles | Volume 21, issue 12
https://doi.org/10.5194/acp-21-9859-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-9859-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Jul 2021
Research article |
| 01 Jul 2021
| 01 Jul 2021
Quantification of solid fuel combustion and aqueous chemistry contributions to secondary organic aerosol during wintertime haze events in Beijing
Yandong Tong
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Veronika Pospisilova
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
now at: Tofwerk AG, Uttigenstrasse 22, 3600 Thun, Switzerland
Lu Qi
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Jing Duan
Key Lab of Aerosol Chemistry & Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
Yifang Gu
Key Lab of Aerosol Chemistry & Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
Varun Kumar
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Pragati Rai
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Giulia Stefenelli
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Liwei Wang
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Ying Wang
Key Lab of Aerosol Chemistry & Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
Haobin Zhong
Key Lab of Aerosol Chemistry & Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Junji Cao
Key Lab of Aerosol Chemistry & Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
Ru-Jin Huang
Key Lab of Aerosol Chemistry & Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an, China
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
Jay G. Slowik
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen, Switzerland
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26 citations as recorded by crossref.
- Aerosol liquid water in PM2.5 and its roles in secondary aerosol formation at a regional site of Yangtze River Delta R. Shi et al. 10.1016/j.jes.2023.04.030
- Measurement report: On the difference in aerosol hygroscopicity between high and low relative humidity conditions in the North China Plain J. Shi et al. 10.5194/acp-22-4599-2022
- Size distributions of molecular markers for biogenic secondary organic aerosol in urban Beijing D. Liu et al. 10.1016/j.envpol.2023.121569
- Composition and Sources of Organic Aerosol in Two Megacities in Western China Using Complementary Mass Spectrometric and Statistical Techniques T. Cui et al. 10.1021/acsestair.4c00051
- Displacement of Strong Acids or Bases by Weak Acids or Bases in Aerosols: Thermodynamics and Kinetics Z. Chen et al. 10.1021/acs.est.2c03719
- Measurement report: Ambient volatile organic compound (VOC) pollution in urban Beijing: characteristics, sources, and implications for pollution control L. Cui et al. 10.5194/acp-22-11931-2022
- Major source categories of PM2.5 oxidative potential in wintertime Beijing and surroundings based on online dithiothreitol-based field measurements R. Cheung et al. 10.1016/j.scitotenv.2024.172345
- Characteristics of sub-micron aerosols in the Yellow Sea and its environmental implications A. Loh et al. 10.1016/j.marpolbul.2024.116556
- Precursors and Pathways Leading to Enhanced Secondary Organic Aerosol Formation during Severe Haze Episodes Y. Zheng et al. 10.1021/acs.est.1c04255
- Substantial contribution of transported emissions to organic aerosol in Beijing K. Daellenbach et al. 10.1038/s41561-024-01493-3
- The characterization of ambient levoglucosan in Beijing during summertime: Dynamic variation and source contributions under strong cooking influences J. Wang et al. 10.1016/j.jes.2024.08.029
- Characterization of carbonaceous substances emitted from residential solid fuel combustion using real-world data from the Beijing-Tianjin-Hebei region M. Cui et al. 10.1016/j.scitotenv.2022.155529
- Bulk and molecular-level composition of primary organic aerosol from wood, straw, cow dung, and plastic burning J. Zhang et al. 10.5194/acp-23-14561-2023
- Weakened Gas-to-Particle Partitioning of Oxygenated Organic Molecules in Liquified Aerosol Particles W. Ma et al. 10.1021/acs.estlett.2c00556
- Chemical composition, sources and optical properties of nitrated aromatic compounds in fine particulate matter during winter foggy days in Nanjing, China C. Gu et al. 10.1016/j.envres.2022.113255
- Response of organic aerosol in Beijing to emission reductions during the XXIV Olympic Winter Games Q. Qu et al. 10.1016/j.scitotenv.2024.170033
- Organic aerosol sources in the Milan metropolitan area – Receptor modelling based on field observations and air quality modelling K. Daellenbach et al. 10.1016/j.atmosenv.2023.119799
- Applications of environmental mass spectrometry in atmospheric haze chemistry T. Chen et al. 10.1016/j.trac.2024.117614
- Quantification of primary and secondary organic aerosol sources by combined factor analysis of extractive electrospray ionisation and aerosol mass spectrometer measurements (EESI-TOF and AMS) Y. Tong et al. 10.5194/amt-15-7265-2022
- Highly time-resolved chemical speciation and source apportionment of organic aerosol components in Delhi, India, using extractive electrospray ionization mass spectrometry V. Kumar et al. 10.5194/acp-22-7739-2022
- Large contribution of in-cloud production of secondary organic aerosol from biomass burning emissions T. Wang et al. 10.1038/s41612-024-00682-6
- Emissions from ships’ activities in the anchorage zone: A potential source of sub-micron aerosols in port areas A. Loh et al. 10.1016/j.jhazmat.2023.131775
- Chemical composition and sources of organic aerosol on the Adriatic coast in Croatia R. Casotto et al. 10.1016/j.aeaoa.2022.100159
- Hygroscopic growth and collision studies of atmospheric aerosols across scaled particle sizes Y. Lu et al. 10.1016/j.powtec.2023.119258
- Opinion: How will advances in aerosol science inform our understanding of the health impacts of outdoor particulate pollution? I. El Haddad et al. 10.5194/acp-24-11981-2024
- Influences of meteorology on emission sources and physicochemical properties of particulate matter in Seoul, Korea during the heating period J. Jeon et al. 10.1016/j.atmosenv.2023.119733
2 citations as recorded by crossref.
- Airborne extractive electrospray mass spectrometry measurements of the chemical composition of organic aerosol D. Pagonis et al. 10.5194/amt-14-1545-2021
- Quantification of solid fuel combustion and aqueous chemistry contributions to secondary organic aerosol during wintertime haze events in Beijing Y. Tong et al. 10.5194/acp-21-9859-2021
Latest update: 23 Nov 2024
Short summary
We investigate SOA sources and formation processes by a field deployment of the EESI-TOF-MS and L-TOF AMS in Beijing in late autumn and early winter. Our study shows that the sources and processes giving rise to haze events in Beijing are variable and seasonally dependent: (1) in the heating season, SOA formation is driven by oxidation of aromatics from solid fuel combustion; and (2) under high-NOx and RH conditions, aqueous-phase chemistry can be a major contributor to SOA formation.
We investigate SOA sources and formation processes by a field deployment of the EESI-TOF-MS and...
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