Articles | Volume 21, issue 11
https://doi.org/10.5194/acp-21-8915-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-8915-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
11 Jun 2021
Research article |
| 11 Jun 2021
| 11 Jun 2021
Radiative and chemical implications of the size and composition of aerosol particles in the existing or modified global stratosphere
Daniel M. Murphy
CORRESPONDING AUTHOR
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Karl D. Froyd
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Ilann Bourgeois
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Charles A. Brock
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Agnieszka Kupc
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Faculty of Physics, Aerosol Physics and Environmental Physics, University of Vienna, 1090 Vienna, Austria
Jeff Peischl
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Gregory P. Schill
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Chelsea R. Thompson
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Christina J. Williamson
NOAA Chemical Sciences Laboratory, Boulder, CO 80305, USA
Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO 80309, USA
Pengfei Yu
Institute for Environment and Climate Research, Jinan University, Guangzhou, China
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28 citations as recorded by crossref.
- Stratospheric Aerosol Composition Observed by the Atmospheric Chemistry Experiment Following the 2019 Raikoke Eruption C. Boone et al. 10.1029/2022JD036600
- Effects of local aerosol and transported dust pollution on the surface energy balance over farmland in eastern China during spring C. Zhou et al. 10.3389/fenvs.2022.1059292
- Baseline Balloon Stratospheric Aerosol Profiles (B2SAP)—Systematic Measurements of Aerosol Number Density and Size M. Todt et al. 10.1029/2022JD038041
- Global distribution of Asian, Middle Eastern, and North African dust simulated by CESM1/CARMA S. Lian et al. 10.5194/acp-22-13659-2022
- Climate-relevant properties of black carbon aerosols revealed by in situ measurements: a review N. Moteki 10.1186/s40645-023-00544-4
- Secondary Organic Aerosol Formation Regulates Cloud Condensation Nuclei in the Global Remote Troposphere M. Liu & H. Matsui 10.1029/2022GL100543
- Opinion: Stratospheric ozone – depletion, recovery and new challenges M. Chipperfield & S. Bekki 10.5194/acp-24-2783-2024
- Metals from spacecraft reentry in stratospheric aerosol particles D. Murphy et al. 10.1073/pnas.2313374120
- The potential environmental and climate impacts of stratospheric aerosol injection: a review H. Huynh & V. McNeill 10.1039/D3EA00134B
- Description and performance of a sectional aerosol microphysical model in the Community Earth System Model (CESM2) S. Tilmes et al. 10.5194/gmd-16-6087-2023
- Particle number concentrations and size distributions in the stratosphere: implications of nucleation mechanisms and particle microphysics F. Yu et al. 10.5194/acp-23-1863-2023
- Atlas of ACE spectra of clouds and aerosols M. Lecours et al. 10.1016/j.jqsrt.2022.108361
- Stratospheric chlorine processing after the 2020 Australian wildfires derived from satellite data P. Wang et al. 10.1073/pnas.2213910120
- A Novel Network‐Based Approach to Determining Measurement Representation Error for Model Evaluation of Aerosol Microphysical Properties E. Asher et al. 10.1029/2021JD035485
- Sulfate aerosol properties derived from combining coincident ACE-FTS and SAGE III/ISS measurements C. Boone et al. 10.1016/j.jqsrt.2023.108815
- Prolonged and Pervasive Perturbations in the Composition of the Southern Hemisphere Midlatitude Lower Stratosphere From the Australian New Year's Fires M. Santee et al. 10.1029/2021GL096270
- Does the Asian summer monsoon play a role in the stratospheric aerosol budget of the Arctic? S. Graßl et al. 10.5194/acp-24-7535-2024
- Composition Dependence of Stratospheric Aerosol Shortwave Radiative Forcing in Northern Midlatitudes Y. Li et al. 10.1029/2021GL094427
- In situ measurements of perturbations to stratospheric aerosol and modeled ozone and radiative impacts following the 2021 La Soufrière eruption Y. Li et al. 10.5194/acp-23-15351-2023
- Unexpected Repartitioning of Stratospheric Inorganic Chlorine After the 2020 Australian Wildfires S. Strahan et al. 10.1029/2022GL098290
- Characteristics of Atmospheric Ice Nucleation during Spring: A Case Study on Huangshan K. Chen et al. 10.3390/atmos15060629
- Unexpectedly rapid aerosol formation in the Hunga Tonga plume E. Asher et al. 10.1073/pnas.2219547120
- Ambient aerosol properties in the remote atmosphere from global-scale in situ measurements C. Brock et al. 10.5194/acp-21-15023-2021
- Contrasting Stratospheric Smoke Mass and Lifetime From 2017 Canadian and 2019/2020 Australian Megafires: Global Simulations and Satellite Observations G. D’Angelo et al. 10.1029/2021JD036249
- Measurement report: Violent biomass burning and volcanic eruptions – a new period of elevated stratospheric aerosol over central Europe (2017 to 2023) in a long series of observations T. Trickl et al. 10.5194/acp-24-1997-2024
- On the stratospheric chemistry of midlatitude wildfire smoke S. Solomon et al. 10.1073/pnas.2117325119
- Chlorine activation and enhanced ozone depletion induced by wildfire aerosol S. Solomon et al. 10.1038/s41586-022-05683-0
- The importance of acid-processed meteoric smoke relative to meteoric fragments for crystal nucleation in polar stratospheric clouds A. James et al. 10.5194/acp-23-2215-2023
28 citations as recorded by crossref.
- Stratospheric Aerosol Composition Observed by the Atmospheric Chemistry Experiment Following the 2019 Raikoke Eruption C. Boone et al. 10.1029/2022JD036600
- Effects of local aerosol and transported dust pollution on the surface energy balance over farmland in eastern China during spring C. Zhou et al. 10.3389/fenvs.2022.1059292
- Baseline Balloon Stratospheric Aerosol Profiles (B2SAP)—Systematic Measurements of Aerosol Number Density and Size M. Todt et al. 10.1029/2022JD038041
- Global distribution of Asian, Middle Eastern, and North African dust simulated by CESM1/CARMA S. Lian et al. 10.5194/acp-22-13659-2022
- Climate-relevant properties of black carbon aerosols revealed by in situ measurements: a review N. Moteki 10.1186/s40645-023-00544-4
- Secondary Organic Aerosol Formation Regulates Cloud Condensation Nuclei in the Global Remote Troposphere M. Liu & H. Matsui 10.1029/2022GL100543
- Opinion: Stratospheric ozone – depletion, recovery and new challenges M. Chipperfield & S. Bekki 10.5194/acp-24-2783-2024
- Metals from spacecraft reentry in stratospheric aerosol particles D. Murphy et al. 10.1073/pnas.2313374120
- The potential environmental and climate impacts of stratospheric aerosol injection: a review H. Huynh & V. McNeill 10.1039/D3EA00134B
- Description and performance of a sectional aerosol microphysical model in the Community Earth System Model (CESM2) S. Tilmes et al. 10.5194/gmd-16-6087-2023
- Particle number concentrations and size distributions in the stratosphere: implications of nucleation mechanisms and particle microphysics F. Yu et al. 10.5194/acp-23-1863-2023
- Atlas of ACE spectra of clouds and aerosols M. Lecours et al. 10.1016/j.jqsrt.2022.108361
- Stratospheric chlorine processing after the 2020 Australian wildfires derived from satellite data P. Wang et al. 10.1073/pnas.2213910120
- A Novel Network‐Based Approach to Determining Measurement Representation Error for Model Evaluation of Aerosol Microphysical Properties E. Asher et al. 10.1029/2021JD035485
- Sulfate aerosol properties derived from combining coincident ACE-FTS and SAGE III/ISS measurements C. Boone et al. 10.1016/j.jqsrt.2023.108815
- Prolonged and Pervasive Perturbations in the Composition of the Southern Hemisphere Midlatitude Lower Stratosphere From the Australian New Year's Fires M. Santee et al. 10.1029/2021GL096270
- Does the Asian summer monsoon play a role in the stratospheric aerosol budget of the Arctic? S. Graßl et al. 10.5194/acp-24-7535-2024
- Composition Dependence of Stratospheric Aerosol Shortwave Radiative Forcing in Northern Midlatitudes Y. Li et al. 10.1029/2021GL094427
- In situ measurements of perturbations to stratospheric aerosol and modeled ozone and radiative impacts following the 2021 La Soufrière eruption Y. Li et al. 10.5194/acp-23-15351-2023
- Unexpected Repartitioning of Stratospheric Inorganic Chlorine After the 2020 Australian Wildfires S. Strahan et al. 10.1029/2022GL098290
- Characteristics of Atmospheric Ice Nucleation during Spring: A Case Study on Huangshan K. Chen et al. 10.3390/atmos15060629
- Unexpectedly rapid aerosol formation in the Hunga Tonga plume E. Asher et al. 10.1073/pnas.2219547120
- Ambient aerosol properties in the remote atmosphere from global-scale in situ measurements C. Brock et al. 10.5194/acp-21-15023-2021
- Contrasting Stratospheric Smoke Mass and Lifetime From 2017 Canadian and 2019/2020 Australian Megafires: Global Simulations and Satellite Observations G. D’Angelo et al. 10.1029/2021JD036249
- Measurement report: Violent biomass burning and volcanic eruptions – a new period of elevated stratospheric aerosol over central Europe (2017 to 2023) in a long series of observations T. Trickl et al. 10.5194/acp-24-1997-2024
- On the stratospheric chemistry of midlatitude wildfire smoke S. Solomon et al. 10.1073/pnas.2117325119
- Chlorine activation and enhanced ozone depletion induced by wildfire aerosol S. Solomon et al. 10.1038/s41586-022-05683-0
- The importance of acid-processed meteoric smoke relative to meteoric fragments for crystal nucleation in polar stratospheric clouds A. James et al. 10.5194/acp-23-2215-2023
Latest update: 13 Dec 2024
Short summary
New measurements in the lower stratosphere highlight differences between particles that originated in the troposphere or the stratosphere. The stratospheric-origin particles have relatively large radiative effects because they are at nearly the optimum diameter for light scattering. The tropospheric particles contribute significantly to surface area. These and other chemical and physical properties are then extended to study the implications if material were to be added to the stratosphere.
New measurements in the lower stratosphere highlight differences between particles that...
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