Articles | Volume 21, issue 9
https://doi.org/10.5194/acp-21-7135-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-7135-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
10 May 2021
Research article |
| 10 May 2021
| 10 May 2021
Interactions of organosulfates with water vapor under sub- and supersaturated conditions
Chao Peng
State Key Laboratory of Organic Geochemistry, Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, and
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and
Control, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences,
Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
Patricia N. Razafindrambinina
Department of Chemistry and Biochemistry, College of Computer,
Mathematical and Natural Sciences, University of Maryland, College Park, MD 20742, USA
Kotiba A. Malek
Department of Chemical and Biomolecular Engineering, A. James Clark
School of Engineering, University of Maryland, College Park, MD 20742, USA
Lanxiadi Chen
State Key Laboratory of Organic Geochemistry, Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, and
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and
Control, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences,
Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Weigang Wang
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Beijing National Laboratory for Molecular Sciences, CAS
Research/Education Center for Excellence in Molecular Sciences, Institute of
Chemistry, Chinese Academy of Sciences, Beijing 100190, China
Ru-Jin Huang
Key Laboratory of Aerosol Chemistry and Physics, State Key Laboratory of Loess and Quaternary Geology, Institute of Earth and Environment, Chinese Academy of Sciences, Xi'an 710061, China
Yuqing Zhang
State Key Laboratory of Organic Geochemistry, Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, and
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and
Control, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences,
Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
Xiang Ding
State Key Laboratory of Organic Geochemistry, Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, and
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and
Control, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences,
Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Beijing National Laboratory for Molecular Sciences, CAS
Research/Education Center for Excellence in Molecular Sciences, Institute of
Chemistry, Chinese Academy of Sciences, Beijing 100190, China
Xinming Wang
State Key Laboratory of Organic Geochemistry, Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, and
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and
Control, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences,
Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
Akua A. Asa-Awuku
Department of Chemistry and Biochemistry, College of Computer,
Mathematical and Natural Sciences, University of Maryland, College Park, MD 20742, USA
Department of Chemical and Biomolecular Engineering, A. James Clark
School of Engineering, University of Maryland, College Park, MD 20742, USA
State Key Laboratory of Organic Geochemistry, Guangdong Key
Laboratory of Environmental Protection and Resources Utilization, and
Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and
Control, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences,
Guangzhou 510640, China
CAS Center for Excellence in Deep Earth Science, Guangzhou 510640,
China
University of Chinese Academy of Sciences, Beijing 100049, China
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Cited
23 citations as recorded by crossref.
- Chemical Insights into the Molecular Composition of Organic Aerosols in the Urban Region of Houston, Texas T. Gautam et al. 10.1021/acsestair.4c00141
- Using particle-resolved aerosol model simulations to guide the interpretations of cloud condensation nuclei experimental data P. Razafindrambinina et al. 10.1080/02786826.2023.2202741
- Waste plastic-derived aerogel modified with graphene oxide for hygroscopic material and oil spill treatment P. Tu et al. 10.1016/j.molstruc.2023.135737
- Beyond the formation: unveiling the atmospheric transformation of organosulfatesviaheterogeneous OH oxidation S. Ng & M. Chan 10.1039/D3CC03700B
- Cloud condensation nuclei (CCN) activity analysis of low-hygroscopicity aerosols using the aerodynamic aerosol classifier (AAC) K. Gohil & A. Asa-Awuku 10.5194/amt-15-1007-2022
- Hygroscopicity and cloud condensation nucleation activities of hydroxyalkylsulfonates C. Peng et al. 10.1016/j.scitotenv.2022.154767
- Application of the QuEChERS method for the determination of pesticides, PAHs and PCBs in fish in Senegal C. Tidiane Dione et al. 10.1080/10934529.2022.2123188
- Toward an Understanding of Uric Acid Particle Dissolution: Surface and Bulk-Driven Water Activity D. Rastogi et al. 10.1021/acs.jpca.4c02388
- A single-parameter hygroscopicity model for functionalized insoluble aerosol surfaces C. Mao et al. 10.5194/acp-22-13219-2022
- OH Radical Oxidation of Organosulfates in the Atmospheric Aqueous Phase D. Gweme & S. Styler 10.1021/acs.jpca.4c02877
- Formation mechanism of typical aromatic sulfuric anhydrides and their potential role in atmospheric nucleation process H. Zhang et al. 10.1016/j.jes.2022.01.015
- The Role of Organic Vapor in the Water Uptake of Organic Aerosols K. Malek et al. 10.1021/acsearthspacechem.4c00017
- Physical properties of short chain aqueous organosulfate aerosol A. Bain et al. 10.1039/D3EA00088E
- Nontarget Screening Exhibits a Seasonal Cycle of PM2.5 Organic Aerosol Composition in Beijing J. Ma et al. 10.1021/acs.est.1c06905
- Reconsideration of surface tension and phase state effects on cloud condensation nuclei activity based on the atomic force microscopy measurement C. Xiong et al. 10.5194/acp-22-16123-2022
- Molecular interaction between ammonium sulfate and secondary organic aerosol from styrene S. Yu et al. 10.1016/j.scitotenv.2024.176414
- Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm Z. Li et al. 10.5194/acp-24-11717-2024
- Reactivity of aminophenols in forming nitrogen-containing brown carbon from iron-catalyzed reactions H. Al-Abadleh et al. 10.1038/s42004-022-00732-1
- Molecular Characteristics of Atmospheric Organosulfates During Summer and Winter Seasons in Two Cities of Southern and Northern China Y. Lin et al. 10.1029/2022JD036672
- The light absorbing and molecule characteristic of PM2.5 brown carbon observed in urban Shanghai Z. Bai et al. 10.1016/j.envpol.2022.120874
- Chemical Fate of Particulate Sulfur from Nighttime Oxidation of Thiophene M. Lum et al. 10.1021/acsestair.4c00164
- Second-Order Kinetic Rate Coefficients for the Aqueous-Phase Sulfate Radical (SO4•–) Oxidation of Some Atmospherically Relevant Organic Compounds L. Tran et al. 10.1021/acs.jpca.2c04964
- Molecular characteristics, sources, and formation pathways of organosulfur compounds in ambient aerosol in Guangzhou, South China H. Jiang et al. 10.5194/acp-22-6919-2022
23 citations as recorded by crossref.
- Chemical Insights into the Molecular Composition of Organic Aerosols in the Urban Region of Houston, Texas T. Gautam et al. 10.1021/acsestair.4c00141
- Using particle-resolved aerosol model simulations to guide the interpretations of cloud condensation nuclei experimental data P. Razafindrambinina et al. 10.1080/02786826.2023.2202741
- Waste plastic-derived aerogel modified with graphene oxide for hygroscopic material and oil spill treatment P. Tu et al. 10.1016/j.molstruc.2023.135737
- Beyond the formation: unveiling the atmospheric transformation of organosulfatesviaheterogeneous OH oxidation S. Ng & M. Chan 10.1039/D3CC03700B
- Cloud condensation nuclei (CCN) activity analysis of low-hygroscopicity aerosols using the aerodynamic aerosol classifier (AAC) K. Gohil & A. Asa-Awuku 10.5194/amt-15-1007-2022
- Hygroscopicity and cloud condensation nucleation activities of hydroxyalkylsulfonates C. Peng et al. 10.1016/j.scitotenv.2022.154767
- Application of the QuEChERS method for the determination of pesticides, PAHs and PCBs in fish in Senegal C. Tidiane Dione et al. 10.1080/10934529.2022.2123188
- Toward an Understanding of Uric Acid Particle Dissolution: Surface and Bulk-Driven Water Activity D. Rastogi et al. 10.1021/acs.jpca.4c02388
- A single-parameter hygroscopicity model for functionalized insoluble aerosol surfaces C. Mao et al. 10.5194/acp-22-13219-2022
- OH Radical Oxidation of Organosulfates in the Atmospheric Aqueous Phase D. Gweme & S. Styler 10.1021/acs.jpca.4c02877
- Formation mechanism of typical aromatic sulfuric anhydrides and their potential role in atmospheric nucleation process H. Zhang et al. 10.1016/j.jes.2022.01.015
- The Role of Organic Vapor in the Water Uptake of Organic Aerosols K. Malek et al. 10.1021/acsearthspacechem.4c00017
- Physical properties of short chain aqueous organosulfate aerosol A. Bain et al. 10.1039/D3EA00088E
- Nontarget Screening Exhibits a Seasonal Cycle of PM2.5 Organic Aerosol Composition in Beijing J. Ma et al. 10.1021/acs.est.1c06905
- Reconsideration of surface tension and phase state effects on cloud condensation nuclei activity based on the atomic force microscopy measurement C. Xiong et al. 10.5194/acp-22-16123-2022
- Molecular interaction between ammonium sulfate and secondary organic aerosol from styrene S. Yu et al. 10.1016/j.scitotenv.2024.176414
- Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm Z. Li et al. 10.5194/acp-24-11717-2024
- Reactivity of aminophenols in forming nitrogen-containing brown carbon from iron-catalyzed reactions H. Al-Abadleh et al. 10.1038/s42004-022-00732-1
- Molecular Characteristics of Atmospheric Organosulfates During Summer and Winter Seasons in Two Cities of Southern and Northern China Y. Lin et al. 10.1029/2022JD036672
- The light absorbing and molecule characteristic of PM2.5 brown carbon observed in urban Shanghai Z. Bai et al. 10.1016/j.envpol.2022.120874
- Chemical Fate of Particulate Sulfur from Nighttime Oxidation of Thiophene M. Lum et al. 10.1021/acsestair.4c00164
- Second-Order Kinetic Rate Coefficients for the Aqueous-Phase Sulfate Radical (SO4•–) Oxidation of Some Atmospherically Relevant Organic Compounds L. Tran et al. 10.1021/acs.jpca.2c04964
- Molecular characteristics, sources, and formation pathways of organosulfur compounds in ambient aerosol in Guangzhou, South China H. Jiang et al. 10.5194/acp-22-6919-2022
Latest update: 17 Apr 2025
Short summary
Organosulfates are important constituents in tropospheric aerosol particles, but their hygroscopic properties and cloud condensation nuclei activities are not well understood. In our work, three complementary techniques were employed to investigate the interactions of 11 organosulfates with water vapor under sub- and supersaturated conditions.
Organosulfates are important constituents in tropospheric aerosol particles, but their...
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