Articles | Volume 21, issue 9
https://doi.org/10.5194/acp-21-6999-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-21-6999-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
07 May 2021
Research article |
| 07 May 2021
| 07 May 2021
Water uptake of subpollen aerosol particles: hygroscopic growth, cloud condensation nuclei activation, and liquid–liquid phase separation
Eugene F. Mikhailov
CORRESPONDING AUTHOR
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
Department of Atmospheric Physics, Saint Petersburg State University, 7/9 Universitetskaya nab., St
Petersburg, 199034, Russia
Mira L. Pöhlker
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
Kathrin Reinmuth-Selzle
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
Sergey S. Vlasenko
Department of Atmospheric Physics, Saint Petersburg State University, 7/9 Universitetskaya nab., St
Petersburg, 199034, Russia
Ovid O. Krüger
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
Janine Fröhlich-Nowoisky
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
Christopher Pöhlker
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
Olga A. Ivanova
Department of Atmospheric Physics, Saint Petersburg State University, 7/9 Universitetskaya nab., St
Petersburg, 199034, Russia
Alexey A. Kiselev
Atmospheric Aerosol Research Department, Institute for Meteorology and
Climate Research, Karlsruhe Institute of Technology (KIT),
Hermann-von-Helmholtz Platz 1, 76344 Eggenstein-Leopoldshafen, Germany
Leslie A. Kremper
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
Ulrich Pöschl
Multiphase Chemistry and Biogeochemistry Departments, Max Planck
Institute for Chemistry, 55020 Mainz, Germany
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Cited
25 citations as recorded by crossref.
- Determination of the protein content of complex samples by aromatic amino acid analysis, liquid chromatography-UV absorbance, and colorimetry K. Reinmuth-Selzle et al. 10.1007/s00216-022-03910-1
- Identification and quantification of giant bioaerosol particles over the Amazon rainforest C. Barbosa et al. 10.1038/s41612-022-00294-y
- Vertical profile of aerosol characteristics including activation over a rain shadow region in India M. Varghese et al. 10.1016/j.atmosenv.2021.118653
- Water Solubility Distribution of Organic Matter Accounts for the Discrepancy in Hygroscopicity among Sub- and Supersaturated Humidity Regimes W. Lee et al. 10.1021/acs.est.2c04647
- Measurement report: Water diffusion in single suspended phase-separated aerosols Y. Tong et al. 10.5194/acp-24-2937-2024
- Bioaerosol nexus of air quality, climate system and human health F. Shen & M. Yao 10.1360/nso/20220050
- Water activity and surface tension of aqueous ammonium sulfate and D-glucose aerosol nanoparticles E. Mikhailov et al. 10.5194/acp-24-2971-2024
- Cloud condensation nuclei activation properties of Mediterranean pollen types considering organic chemical composition and surface tension effects A. Casans et al. 10.1016/j.atmosenv.2023.119961
- From trees to rain: enhancement of cloud glaciation and precipitation by pollen J. Kretzschmar et al. 10.1088/1748-9326/ad747a
- Respiratory aerosols and droplets in the transmission of infectious diseases M. Pöhlker et al. 10.1103/RevModPhys.95.045001
- Field Evaluation of an Automated Pollen Sensor C. Jiang et al. 10.3390/ijerph19116444
- Russian Studies on Clouds and Precipitation in 2019–2022 N. Bezrukova & A. Chernokulsky 10.31857/S0002351523070039
- Hygroscopic growth and CCN activity of secondary organic aerosol produced from dark ozonolysis of γ-terpinene H. Bouzidi et al. 10.1016/j.scitotenv.2022.153010
- Global organic and inorganic aerosol hygroscopicity and its effect on radiative forcing M. Pöhlker et al. 10.1038/s41467-023-41695-8
- Russian Studies on Clouds and Precipitation in 2019–2022 N. Bezrukova & A. Chernokulsky 10.1134/S0001433823150033
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al. 10.3389/fenvs.2023.1142941
- Detecting the pH-dependent liquid-liquid phase separation of single levitated aerosol microdroplets via laser tweezers-Raman spectroscopy Y. Tong et al. 10.3389/fphy.2022.969921
- Waste plastic-derived aerogel modified with graphene oxide for hygroscopic material and oil spill treatment P. Tu et al. 10.1016/j.molstruc.2023.135737
- Russian Investigations in the Field of Atmospheric Radiation in 2019–2022 Y. Timofeyev et al. 10.1134/S0001433823150124
- Liquid–Liquid Phase Separation in Single Suspended Aerosol Microdroplets Y. Tong & A. Ye 10.1021/acs.analchem.2c05605
- Russian Investigations in the Field of Amtospheric Radiation in 2019–2022 Y. Timofeyev et al. 10.31857/S000235152307012X
- Ice nucleation activity of airborne pollen: A short review of results from laboratory experiments P. Duan et al. 10.1016/j.atmosres.2023.106659
- Influence of acidity on liquid–liquid phase transitions of mixed secondary organic aerosol (SOA) proxy–inorganic aerosol droplets Y. Chen et al. 10.5194/acp-23-10255-2023
- Application of physisorption analyzer in measuring the hygroscopicity of atmospheric aerosols Y. Hu et al. 10.1051/e3sconf/202453603021
- Sensitivities to biological aerosol particle properties and ageing processes: potential implications for aerosol–cloud interactions and optical properties M. Zhang et al. 10.5194/acp-21-3699-2021
24 citations as recorded by crossref.
- Determination of the protein content of complex samples by aromatic amino acid analysis, liquid chromatography-UV absorbance, and colorimetry K. Reinmuth-Selzle et al. 10.1007/s00216-022-03910-1
- Identification and quantification of giant bioaerosol particles over the Amazon rainforest C. Barbosa et al. 10.1038/s41612-022-00294-y
- Vertical profile of aerosol characteristics including activation over a rain shadow region in India M. Varghese et al. 10.1016/j.atmosenv.2021.118653
- Water Solubility Distribution of Organic Matter Accounts for the Discrepancy in Hygroscopicity among Sub- and Supersaturated Humidity Regimes W. Lee et al. 10.1021/acs.est.2c04647
- Measurement report: Water diffusion in single suspended phase-separated aerosols Y. Tong et al. 10.5194/acp-24-2937-2024
- Bioaerosol nexus of air quality, climate system and human health F. Shen & M. Yao 10.1360/nso/20220050
- Water activity and surface tension of aqueous ammonium sulfate and D-glucose aerosol nanoparticles E. Mikhailov et al. 10.5194/acp-24-2971-2024
- Cloud condensation nuclei activation properties of Mediterranean pollen types considering organic chemical composition and surface tension effects A. Casans et al. 10.1016/j.atmosenv.2023.119961
- From trees to rain: enhancement of cloud glaciation and precipitation by pollen J. Kretzschmar et al. 10.1088/1748-9326/ad747a
- Respiratory aerosols and droplets in the transmission of infectious diseases M. Pöhlker et al. 10.1103/RevModPhys.95.045001
- Field Evaluation of an Automated Pollen Sensor C. Jiang et al. 10.3390/ijerph19116444
- Russian Studies on Clouds and Precipitation in 2019–2022 N. Bezrukova & A. Chernokulsky 10.31857/S0002351523070039
- Hygroscopic growth and CCN activity of secondary organic aerosol produced from dark ozonolysis of γ-terpinene H. Bouzidi et al. 10.1016/j.scitotenv.2022.153010
- Global organic and inorganic aerosol hygroscopicity and its effect on radiative forcing M. Pöhlker et al. 10.1038/s41467-023-41695-8
- Russian Studies on Clouds and Precipitation in 2019–2022 N. Bezrukova & A. Chernokulsky 10.1134/S0001433823150033
- Morphology and phase state of PM2.5 in urban and coastal-rural areas during summer S. Gaikwad et al. 10.3389/fenvs.2023.1142941
- Detecting the pH-dependent liquid-liquid phase separation of single levitated aerosol microdroplets via laser tweezers-Raman spectroscopy Y. Tong et al. 10.3389/fphy.2022.969921
- Waste plastic-derived aerogel modified with graphene oxide for hygroscopic material and oil spill treatment P. Tu et al. 10.1016/j.molstruc.2023.135737
- Russian Investigations in the Field of Atmospheric Radiation in 2019–2022 Y. Timofeyev et al. 10.1134/S0001433823150124
- Liquid–Liquid Phase Separation in Single Suspended Aerosol Microdroplets Y. Tong & A. Ye 10.1021/acs.analchem.2c05605
- Russian Investigations in the Field of Amtospheric Radiation in 2019–2022 Y. Timofeyev et al. 10.31857/S000235152307012X
- Ice nucleation activity of airborne pollen: A short review of results from laboratory experiments P. Duan et al. 10.1016/j.atmosres.2023.106659
- Influence of acidity on liquid–liquid phase transitions of mixed secondary organic aerosol (SOA) proxy–inorganic aerosol droplets Y. Chen et al. 10.5194/acp-23-10255-2023
- Application of physisorption analyzer in measuring the hygroscopicity of atmospheric aerosols Y. Hu et al. 10.1051/e3sconf/202453603021
Latest update: 03 Nov 2024
Short summary
Subpollen particles are a relatively new subset of atmospheric aerosol particles. When pollen grains rupture, they release cytoplasmic fragments known as subpollen particles (SPPs). We found that SPPs, containing a broad spectrum of biopolymers and hydrocarbons, exhibit abnormally high water uptake. This effect may influence the life cycle of SPPs and the related direct and indirect impacts on radiation budget as well as reinforce their allergic potential.
Subpollen particles are a relatively new subset of atmospheric aerosol particles. When pollen...
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