Articles | Volume 21, issue 6
https://doi.org/10.5194/acp-21-4809-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-4809-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
29 Mar 2021
Research article |
| 29 Mar 2021
| 29 Mar 2021
A three-dimensional-model inversion of methyl chloroform to constrain the atmospheric oxidative capacity
Meteorology and Air Quality, Wageningen University and Research, Wageningen, the Netherlands
Stephen A. Montzka
Halocarbons and other Atmospheric Trace Species (HATS), NOAA Global Monitoring Laboratory, Boulder, CO, USA
Prabir K. Patra
Research Institute for Global Change, JAMSTEC, Yokohama, Japan
Center for Environmental Remote Sensing, Chiba University, Chiba, Japan
Maarten C. Krol
Meteorology and Air Quality, Wageningen University and Research, Wageningen, the Netherlands
Institute for Marine and Atmospheric Research, Utrecht University, Utrecht, the Netherlands
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Cited
14 citations as recorded by crossref.
- Order of magnitude wall time improvement of variational methane inversions by physical parallelization: a demonstration using TM5-4DVAR S. Pandey et al. 10.5194/gmd-15-4555-2022
- Methane emissions decreased in fossil fuel exploitation and sustainably increased in microbial source sectors during 1990–2020 N. Chandra et al. 10.1038/s43247-024-01286-x
- Temporary pause in the growth of atmospheric ethane and propane in 2015–2018 H. Angot et al. 10.5194/acp-21-15153-2021
- Reconciling the bottom-up and top-down estimates of the methane chemical sink using multiple observations Y. Zhao et al. 10.5194/acp-23-789-2023
- Decreasing seasonal cycle amplitude of methane in the northern high latitudes being driven by lower-latitude changes in emissions and transport E. Dowd et al. 10.5194/acp-23-7363-2023
- Radiocarbon monoxide indicates increasing atmospheric oxidizing capacity O. Morgenstern et al. 10.1038/s41467-024-55603-1
- Large and increasing methane emissions from eastern Amazonia derived from satellite data, 2010–2018 C. Wilson et al. 10.5194/acp-21-10643-2021
- Exploring the drivers of tropospheric hydroxyl radical trends in the Geophysical Fluid Dynamics Laboratory AM4.1 atmospheric chemistry–climate model G. Chua et al. 10.5194/acp-23-4955-2023
- Anthropogenic emission is the main contributor to the rise of atmospheric methane during 1993–2017 Z. Zhang et al. 10.1093/nsr/nwab200
- Technical note: Constraining the hydroxyl (OH) radical in the tropics with satellite observations of its drivers – first steps toward assessing the feasibility of a global observation strategy D. Anderson et al. 10.5194/acp-23-6319-2023
- Changes in tropospheric air quality related to the protection of stratospheric ozone in a changing climate S. Madronich et al. 10.1007/s43630-023-00369-6
- Estimation of the atmospheric hydroxyl radical oxidative capacity using multiple hydrofluorocarbons (HFCs) R. Thompson et al. 10.5194/acp-24-1415-2024
- Long‐Term Observations of Levoglucosan in Arctic Aerosols Reveal Its Biomass Burning Source and Implication on Radiative Forcing A. Chen et al. 10.1029/2022JD037597
- Effects of extreme meteorological conditions in 2018 on European methane emissions estimated using atmospheric inversions R. Thompson et al. 10.1098/rsta.2020.0443
14 citations as recorded by crossref.
- Order of magnitude wall time improvement of variational methane inversions by physical parallelization: a demonstration using TM5-4DVAR S. Pandey et al. 10.5194/gmd-15-4555-2022
- Methane emissions decreased in fossil fuel exploitation and sustainably increased in microbial source sectors during 1990–2020 N. Chandra et al. 10.1038/s43247-024-01286-x
- Temporary pause in the growth of atmospheric ethane and propane in 2015–2018 H. Angot et al. 10.5194/acp-21-15153-2021
- Reconciling the bottom-up and top-down estimates of the methane chemical sink using multiple observations Y. Zhao et al. 10.5194/acp-23-789-2023
- Decreasing seasonal cycle amplitude of methane in the northern high latitudes being driven by lower-latitude changes in emissions and transport E. Dowd et al. 10.5194/acp-23-7363-2023
- Radiocarbon monoxide indicates increasing atmospheric oxidizing capacity O. Morgenstern et al. 10.1038/s41467-024-55603-1
- Large and increasing methane emissions from eastern Amazonia derived from satellite data, 2010–2018 C. Wilson et al. 10.5194/acp-21-10643-2021
- Exploring the drivers of tropospheric hydroxyl radical trends in the Geophysical Fluid Dynamics Laboratory AM4.1 atmospheric chemistry–climate model G. Chua et al. 10.5194/acp-23-4955-2023
- Anthropogenic emission is the main contributor to the rise of atmospheric methane during 1993–2017 Z. Zhang et al. 10.1093/nsr/nwab200
- Technical note: Constraining the hydroxyl (OH) radical in the tropics with satellite observations of its drivers – first steps toward assessing the feasibility of a global observation strategy D. Anderson et al. 10.5194/acp-23-6319-2023
- Changes in tropospheric air quality related to the protection of stratospheric ozone in a changing climate S. Madronich et al. 10.1007/s43630-023-00369-6
- Estimation of the atmospheric hydroxyl radical oxidative capacity using multiple hydrofluorocarbons (HFCs) R. Thompson et al. 10.5194/acp-24-1415-2024
- Long‐Term Observations of Levoglucosan in Arctic Aerosols Reveal Its Biomass Burning Source and Implication on Radiative Forcing A. Chen et al. 10.1029/2022JD037597
- Effects of extreme meteorological conditions in 2018 on European methane emissions estimated using atmospheric inversions R. Thompson et al. 10.1098/rsta.2020.0443
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Short summary
Following up on previous box model studies, we employ a 3D transport model to estimate variations in the hydroxyl radical (OH) from observations of methyl chloroform (MCF). We derive small interannual OH variations that are consistent with variations in the El Niño–Southern Oscillation. We also find evidence for the release of MCF from oceans in atmospheric gradients of MCF. Both findings highlight the added value of a 3D transport model since box model studies did not identify these effects.
Following up on previous box model studies, we employ a 3D transport model to estimate...
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