Articles | Volume 21, issue 6
https://doi.org/10.5194/acp-21-4541-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-4541-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Mar 2021
Research article |
| 24 Mar 2021
| 24 Mar 2021
Investigation of several proxies to estimate sulfuric acid concentration under volcanic plume conditions
Clémence Rose
CORRESPONDING AUTHOR
Université Clermont Auvergne, CNRS, Laboratoire de Météorologie Physique (LaMP), 63000 Clermont-Ferrand, France
Matti P. Rissanen
Aerosol Physics Laboratory, Physics Unit, Tampere University, Tampere, Finland
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Siddharth Iyer
Aerosol Physics Laboratory, Physics Unit, Tampere University, Tampere, Finland
Jonathan Duplissy
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Helsinki Institute of Physics, University of Helsinki, Helsinki, Finland
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
John B. Nowak
Chemistry and Dynamics Branch, NASA Langley Research Center, Hampton, VA 23681, USA
Aurélie Colomb
Université Clermont Auvergne, CNRS, Laboratoire de Météorologie Physique (LaMP), 63000 Clermont-Ferrand, France
Régis Dupuy
Université Clermont Auvergne, CNRS, Laboratoire de Météorologie Physique (LaMP), 63000 Clermont-Ferrand, France
Xu-Cheng He
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Janne Lampilahti
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Yee Jun Tham
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Daniela Wimmer
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Jean-Marc Metzger
Observatoire des Sciences de l'Univers de La Réunion, UMS 3365 (CNRS, Université de La Réunion, Météo-France), 97744 Saint-Denis, Réunion, France
Pierre Tulet
LACy, Laboratoire de l'Atmosphère et des Cyclones, UMR8105 (CNRS, Université de La Réunion, Météo-France), 97744 Saint-Denis, Réunion, France
Jérôme Brioude
LACy, Laboratoire de l'Atmosphère et des Cyclones, UMR8105 (CNRS, Université de La Réunion, Météo-France), 97744 Saint-Denis, Réunion, France
Céline Planche
Université Clermont Auvergne, CNRS, Laboratoire de Météorologie Physique (LaMP), 63000 Clermont-Ferrand, France
Markku Kulmala
Institute for Atmospheric and Earth System Research (INAR)/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Karine Sellegri
Université Clermont Auvergne, CNRS, Laboratoire de Météorologie Physique (LaMP), 63000 Clermont-Ferrand, France
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Cited
6 citations as recorded by crossref.
- Direct Measurements of Covalently Bonded Sulfuric Anhydrides from Gas-Phase Reactions of SO3 with Acids under Ambient Conditions A. Kumar et al. 10.1021/jacs.4c04531
- Measurement report: Insights into the chemical composition and origin of molecular clusters and potential precursor molecules present in the free troposphere over the southern Indian Ocean: observations from the Maïdo Observatory (2150 m a.s.l., Réunion) R. Salignat et al. 10.5194/acp-24-3785-2024
- Titanium Dioxide Promotes New Particle Formation: A Smog Chamber Study H. Zhang et al. 10.1021/acs.est.2c06946
- Observed in-plume gaseous elemental mercury depletion suggests significant mercury scavenging by volcanic aerosols A. Koenig et al. 10.1039/D3EA00063J
- Data‐Driven Compound Identification in Atmospheric Mass Spectrometry H. Sandström et al. 10.1002/advs.202306235
- Stratospheric air intrusions promote global-scale new particle formation J. Zhang et al. 10.1126/science.adn2961
6 citations as recorded by crossref.
- Direct Measurements of Covalently Bonded Sulfuric Anhydrides from Gas-Phase Reactions of SO3 with Acids under Ambient Conditions A. Kumar et al. 10.1021/jacs.4c04531
- Measurement report: Insights into the chemical composition and origin of molecular clusters and potential precursor molecules present in the free troposphere over the southern Indian Ocean: observations from the Maïdo Observatory (2150 m a.s.l., Réunion) R. Salignat et al. 10.5194/acp-24-3785-2024
- Titanium Dioxide Promotes New Particle Formation: A Smog Chamber Study H. Zhang et al. 10.1021/acs.est.2c06946
- Observed in-plume gaseous elemental mercury depletion suggests significant mercury scavenging by volcanic aerosols A. Koenig et al. 10.1039/D3EA00063J
- Data‐Driven Compound Identification in Atmospheric Mass Spectrometry H. Sandström et al. 10.1002/advs.202306235
- Stratospheric air intrusions promote global-scale new particle formation J. Zhang et al. 10.1126/science.adn2961
Latest update: 04 Feb 2025
Short summary
Sulfuric acid (H2SO4) is commonly accepted as a key precursor for atmospheric new particle formation. However, direct measurements of [H2SO4] remain challenging, motivating the development of proxies. Using data collected in two different volcanic plumes, we show, under these specific conditions, the good performance of a proxy from the literature and also highlight the benefit of the newly developed proxies for the prediction of the highest [H2SO4] values.
Sulfuric acid (H2SO4) is commonly accepted as a key precursor for atmospheric new particle...
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