Articles | Volume 21, issue 1
https://doi.org/10.5194/acp-21-255-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-255-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
14 Jan 2021
Research article |
| 14 Jan 2021
| 14 Jan 2021
Atmospheric evolution of emissions from a boreal forest fire: the formation of highly functionalized oxygen-, nitrogen-, and sulfur-containing organic compounds
Jenna C. Ditto
Department of Chemical and Environmental Engineering, Yale
University, New Haven, CT 06511, USA
Department of Chemical and Environmental Engineering, Yale
University, New Haven, CT 06511, USA
Tori N. Hass-Mitchell
Department of Chemical and Environmental Engineering, Yale
University, New Haven, CT 06511, USA
Samar G. Moussa
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
Katherine Hayden
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
Shao-Meng Li
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
John Liggio
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
Amy Leithead
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
Patrick Lee
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
Michael J. Wheeler
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
Jeremy J. B. Wentzell
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario M3H 5T4, Canada
Drew R. Gentner
CORRESPONDING AUTHOR
Department of Chemical and Environmental Engineering, Yale
University, New Haven, CT 06511, USA
Solutions for Energy, Air, Climate and Health (SEARCH), School of the Environment, Yale University, New Haven, CT 06511, USA
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Cited
21 citations as recorded by crossref.
- Research on the Setting of Australian Mountain Fire Emergency Center Based on K-Means Algorithm C. Tang et al. 10.1155/2021/5783713
- Reconciling the total carbon budget for boreal forest wildfire emissions using airborne observations K. Hayden et al. 10.5194/acp-22-12493-2022
- Biomass burning nitrogen dioxide emissions derived from space with TROPOMI: methodology and validation D. Griffin et al. 10.5194/amt-14-7929-2021
- The Impact of Coronavirus Disease of 2019 (COVID-19) Lockdown Restrictions on the Criteria Pollutants P. Verma et al. 10.3390/pr11010296
- Insights into the different mixing states and formation processes of amine-containing single particles in Guangzhou, China Q. Zhong et al. 10.1016/j.scitotenv.2022.157440
- Analysis of reduced and oxidized nitrogen-containing organic compounds at a coastal site in summer and winter J. Ditto et al. 10.5194/acp-22-3045-2022
- Mass spectrometric analysis of unprecedented high levels of carbonaceous aerosol particles long-range transported from wildfires in the Siberian Arctic E. Schneider et al. 10.5194/acp-24-553-2024
- Catastrophic Pm2.5 Emissions from Siberian Forest Fires: Impacting Factors Analysis A. Romanov et al. 10.2139/ssrn.4045859
- Sulfate Formation by Photosensitization in Mixed Incense Burning–Sodium Chloride Particles: Effects of RH, Light Intensity, and Aerosol Aging R. Tang et al. 10.1021/acs.est.3c02225
- Total organic carbon measurements reveal major gaps in petrochemical emissions reporting M. He et al. 10.1126/science.adj6233
- Evolution of nucleophilic high molecular-weight organic compounds in ambient aerosols: a case study C. He et al. 10.5194/acp-24-1627-2024
- The state of wildfire and bushfire science: Temporal trends, research divisions and knowledge gaps M. Haghani et al. 10.1016/j.ssci.2022.105797
- Nontarget Tandem High-Resolution Mass Spectrometry Analysis of Functionalized Organic Compounds in Atmospherically Relevant Samples Y. Wan et al. 10.1021/acs.estlett.2c00788
- Quantification of Methane Emissions from Cold Heavy Oil Production with Sand Extraction in Alberta and Saskatchewan, Canada T. Han et al. 10.1021/acs.est.4c02333
- A newly developed Lagrangian chemical transport scheme: Part 1. Simulation of a boreal forest fire plume Y. Liu et al. 10.1016/j.scitotenv.2023.163232
- Appearance of Recalcitrant Dissolved Black Carbon and Dissolved Organic Sulfur in River Waters Following Wildfire Events Y. Xu et al. 10.1021/acs.est.4c00492
- Observations and Modeling of NOx Photochemistry and Fate in Fresh Wildfire Plumes Q. Peng et al. 10.1021/acsearthspacechem.1c00086
- Oxidized and Unsaturated: Key Organic Aerosol Traits Associated with Cellular Reactive Oxygen Species Production in the Southeastern United States F. Liu et al. 10.1021/acs.est.3c03641
- Molecular Characterization of Water-Soluble Aerosol Particle Extracts by Ultrahigh-Resolution Mass Spectrometry: Observation of Industrial Emissions and an Atmospherically Aged Wildfire Plume at Lake Baikal E. Schneider et al. 10.1021/acsearthspacechem.2c00017
- Catastrophic PM2.5 emissions from Siberian forest fires: Impacting factors analysis A. Romanov et al. 10.1016/j.envpol.2022.119324
- Effects of Organic Matrices on Nucleophilic Aqueous Aerosol Chemistry: Yields and Mechanistic Insight for Brown Carbon Formation from Glyoxal and Ammonia G. Drozd et al. 10.1021/acsearthspacechem.2c00068
21 citations as recorded by crossref.
- Research on the Setting of Australian Mountain Fire Emergency Center Based on K-Means Algorithm C. Tang et al. 10.1155/2021/5783713
- Reconciling the total carbon budget for boreal forest wildfire emissions using airborne observations K. Hayden et al. 10.5194/acp-22-12493-2022
- Biomass burning nitrogen dioxide emissions derived from space with TROPOMI: methodology and validation D. Griffin et al. 10.5194/amt-14-7929-2021
- The Impact of Coronavirus Disease of 2019 (COVID-19) Lockdown Restrictions on the Criteria Pollutants P. Verma et al. 10.3390/pr11010296
- Insights into the different mixing states and formation processes of amine-containing single particles in Guangzhou, China Q. Zhong et al. 10.1016/j.scitotenv.2022.157440
- Analysis of reduced and oxidized nitrogen-containing organic compounds at a coastal site in summer and winter J. Ditto et al. 10.5194/acp-22-3045-2022
- Mass spectrometric analysis of unprecedented high levels of carbonaceous aerosol particles long-range transported from wildfires in the Siberian Arctic E. Schneider et al. 10.5194/acp-24-553-2024
- Catastrophic Pm2.5 Emissions from Siberian Forest Fires: Impacting Factors Analysis A. Romanov et al. 10.2139/ssrn.4045859
- Sulfate Formation by Photosensitization in Mixed Incense Burning–Sodium Chloride Particles: Effects of RH, Light Intensity, and Aerosol Aging R. Tang et al. 10.1021/acs.est.3c02225
- Total organic carbon measurements reveal major gaps in petrochemical emissions reporting M. He et al. 10.1126/science.adj6233
- Evolution of nucleophilic high molecular-weight organic compounds in ambient aerosols: a case study C. He et al. 10.5194/acp-24-1627-2024
- The state of wildfire and bushfire science: Temporal trends, research divisions and knowledge gaps M. Haghani et al. 10.1016/j.ssci.2022.105797
- Nontarget Tandem High-Resolution Mass Spectrometry Analysis of Functionalized Organic Compounds in Atmospherically Relevant Samples Y. Wan et al. 10.1021/acs.estlett.2c00788
- Quantification of Methane Emissions from Cold Heavy Oil Production with Sand Extraction in Alberta and Saskatchewan, Canada T. Han et al. 10.1021/acs.est.4c02333
- A newly developed Lagrangian chemical transport scheme: Part 1. Simulation of a boreal forest fire plume Y. Liu et al. 10.1016/j.scitotenv.2023.163232
- Appearance of Recalcitrant Dissolved Black Carbon and Dissolved Organic Sulfur in River Waters Following Wildfire Events Y. Xu et al. 10.1021/acs.est.4c00492
- Observations and Modeling of NOx Photochemistry and Fate in Fresh Wildfire Plumes Q. Peng et al. 10.1021/acsearthspacechem.1c00086
- Oxidized and Unsaturated: Key Organic Aerosol Traits Associated with Cellular Reactive Oxygen Species Production in the Southeastern United States F. Liu et al. 10.1021/acs.est.3c03641
- Molecular Characterization of Water-Soluble Aerosol Particle Extracts by Ultrahigh-Resolution Mass Spectrometry: Observation of Industrial Emissions and an Atmospherically Aged Wildfire Plume at Lake Baikal E. Schneider et al. 10.1021/acsearthspacechem.2c00017
- Catastrophic PM2.5 emissions from Siberian forest fires: Impacting factors analysis A. Romanov et al. 10.1016/j.envpol.2022.119324
- Effects of Organic Matrices on Nucleophilic Aqueous Aerosol Chemistry: Yields and Mechanistic Insight for Brown Carbon Formation from Glyoxal and Ammonia G. Drozd et al. 10.1021/acsearthspacechem.2c00068
Latest update: 20 Nov 2024
Short summary
Forest fires are an important source of reactive organic gases and aerosols to the atmosphere. We analyzed organic aerosols collected from an aircraft above a boreal forest fire and reported an increasing contribution from compounds containing oxygen, nitrogen, and sulfur as the plume aged, with sulfide and ring-bound nitrogen functionality. Our results demonstrated chemistry that is important in biomass burning but also in urban/developing regions with high local nitrogen and sulfur emissions.
Forest fires are an important source of reactive organic gases and aerosols to the atmosphere....
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