Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics
ACP
Articles | Volume 21, issue 3
Articles | Volume 21, issue 3
https://doi.org/10.5194/acp-21-1987-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-1987-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
Articles | Volume 21, issue 3
Measurement report
 | 
10 Feb 2021
Measurement report |  | 10 Feb 2021

Measurement report: Sulfuric acid nucleation and experimental conditions in a photolytic flow reactor

David R. Hanson, Seakh Menheer, Michael Wentzel, and Joan Kunz

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Short summary
We report experimental measurements of particle formation in a flow reactor that extend the results from this experiment to a total of more than 270 runs over a time period of ~3 years. This has allowed us to detect a general increase in the cleanliness of the system and improve our knowledge of its chemistry. In-house simulations allowed us to construct phenomenological free energies of molecular clusters of sulfuric acid and ammonia that are appropriate for application to the atmosphere.
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