Articles | Volume 21, issue 18
https://doi.org/10.5194/acp-21-14275-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-14275-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
ACP Letters
| Highlight paper
| 
27 Sep 2021
ACP Letters | Highlight paper |
| 27 Sep 2021
| 27 Sep 2021
The driving factors of new particle formation and growth in the polluted boundary layer
Mao Xiao
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Christopher R. Hoyle
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Institute for Atmospheric and Climate Science, ETH Zurich, 8092
Zurich, Switzerland
Lubna Dada
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Dominik Stolzenburg
Faculty of Physics, University of Vienna, 1090 Vienna, Austria
Andreas Kürten
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Mingyi Wang
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Houssni Lamkaddam
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Olga Garmash
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Bernhard Mentler
Institute of Ion Physics and Applied Physics, University of Innsbruck,
6020 Innsbruck, Austria
Ugo Molteni
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Andrea Baccarini
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Mario Simon
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Xu-Cheng He
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Katrianne Lehtipalo
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Atmospheric Composition Research Unit, Finnish Meteorological Institute, 00560 Helsinki, Finland
Lauri R. Ahonen
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Rima Baalbaki
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Paulus S. Bauer
Faculty of Physics, University of Vienna, 1090 Vienna, Austria
Lisa Beck
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
David Bell
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Federico Bianchi
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Sophia Brilke
Faculty of Physics, University of Vienna, 1090 Vienna, Austria
Dexian Chen
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Randall Chiu
Department of Chemistry & CIRES, University of Colorado Boulder,
Boulder, CO 80309, USA
António Dias
CENTRA and FCUL, University of Lisbon, 1749-016 Lisbon, Portugal
Jonathan Duplissy
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Helsinki Institute of Physics, University of Helsinki, 00014
Helsinki, Finland
Henning Finkenzeller
Department of Chemistry & CIRES, University of Colorado Boulder,
Boulder, CO 80309, USA
Hamish Gordon
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Victoria Hofbauer
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Changhyuk Kim
Division of Chemistry and Chemical Engineering, California Institute
of Technology, Pasadena, CA 91125, USA
School of Civil and Environmental Engineering, Pusan National
University, 46241 Busan, Republic of Korea
Theodore K. Koenig
Department of Chemistry & CIRES, University of Colorado Boulder,
Boulder, CO 80309, USA
now at: College of Environmental Sciences and Engineering, Peking University, 100871 Beijing, China
Janne Lampilahti
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Chuan Ping Lee
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Department of Applied Physics, University of Eastern Finland, 70211
Kuopio, Finland
Huajun Mai
Division of Chemistry and Chemical Engineering, California Institute
of Technology, Pasadena, CA 91125, USA
Vladimir Makhmutov
Solar and Cosmic Ray Physics Laboratory, P.N. Lebedev Physical Institute of the Russian Academy of Sciences,
119991 Moscow, Russian Federation
Hanna E. Manninen
CERN, 1211 Geneva, Switzerland
Ruby Marten
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Serge Mathot
CERN, 1211 Geneva, Switzerland
Roy L. Mauldin
Department of Chemistry, Carnegie Mellon University, Pittsburgh, PA
15213, USA
Department of Oceanic and Atmospheric Sciences, University of
Colorado Boulder, Boulder, CO 80309, USA
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, China
Antti Onnela
CERN, 1211 Geneva, Switzerland
Eva Partoll
Institute of Ion Physics and Applied Physics, University of Innsbruck,
6020 Innsbruck, Austria
Tuukka Petäjä
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Joschka Pfeifer
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
CERN, 1211 Geneva, Switzerland
Veronika Pospisilova
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Lauriane L. J. Quéléver
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Matti Rissanen
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
now at: Aerosol Physics Laboratory, Physics Unit, Faculty of
Engineering and Natural Sciences, Tampere University, 33720 Tampere, Finland
Siegfried Schobesberger
Department of Applied Physics, University of Eastern Finland, 70211
Kuopio, Finland
Simone Schuchmann
CERN, 1211 Geneva, Switzerland
now at: Experimentelle Teilchen- und Astroteilchenphysik, Johannes Gutenberg University Mainz, 55128 Mainz, Germany
Yuri Stozhkov
Solar and Cosmic Ray Physics Laboratory, P.N. Lebedev Physical Institute of the Russian Academy of Sciences,
119991 Moscow, Russian Federation
Christian Tauber
Faculty of Physics, University of Vienna, 1090 Vienna, Austria
Yee Jun Tham
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
António Tomé
IDL-Universidade da Beira Interior, Covilhã, Portugal
Miguel Vazquez-Pufleau
Faculty of Physics, University of Vienna, 1090 Vienna, Austria
Andrea C. Wagner
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Department of Chemistry & CIRES, University of Colorado Boulder,
Boulder, CO 80309, USA
now at: Department of Chemistry & CIRES, University of
Colorado Boulder, Boulder, CO 80305, USA
Robert Wagner
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Yonghong Wang
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Lena Weitz
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Daniela Wimmer
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Faculty of Physics, University of Vienna, 1090 Vienna, Austria
Yusheng Wu
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Penglin Ye
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Aerodyne Research Inc., Billerica, MA 01821-3976, USA
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Qiaozhi Zha
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Xueqin Zhou
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Antonio Amorim
CENTRA and FCUL, University of Lisbon, 1749-016 Lisbon, Portugal
Ken Carslaw
School of Earth and Environment, University of Leeds, LS2 9JT Leeds, United Kingdom
Joachim Curtius
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
Armin Hansel
Institute of Ion Physics and Applied Physics, University of Innsbruck,
6020 Innsbruck, Austria
Rainer Volkamer
Department of Chemistry & CIRES, University of Colorado Boulder,
Boulder, CO 80309, USA
Department of Oceanic and Atmospheric Sciences, University of
Colorado Boulder, Boulder, CO 80309, USA
Paul M. Winkler
Faculty of Physics, University of Vienna, 1090 Vienna, Austria
Richard C. Flagan
Division of Chemistry and Chemical Engineering, California Institute
of Technology, Pasadena, CA 91125, USA
Markku Kulmala
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Helsinki Institute of Physics, University of Helsinki, 00014
Helsinki, Finland
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, China
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing, China
Douglas R. Worsnop
Institute for Atmospheric and Earth System Research (INAR)/Physics,
University of Helsinki, 00014 Helsinki, Finland
Aerodyne Research Inc., Billerica, MA 01821-3976, USA
Jasper Kirkby
Institute for Atmospheric and Environmental Sciences, Goethe
University Frankfurt, 60438 Frankfurt am Main, Germany
CERN, 1211 Geneva, Switzerland
Neil M. Donahue
Center for Atmospheric Particle Studies, Carnegie Mellon University,
Pittsburgh, PA 15213, USA
Urs Baltensperger
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
Josef Dommen
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, 5232
Villigen, Switzerland
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Latest update: 16 Mar 2025
Short summary
Experiments at CLOUD show that in polluted environments new particle formation (NPF) is largely driven by the formation of sulfuric acid–base clusters, stabilized by amines, high ammonia concentrations or lower temperatures. While oxidation products of aromatics can nucleate, they play a minor role in urban NPF. Our experiments span 4 orders of magnitude variation of observed NPF rates in ambient conditions. We provide a framework based on NPF and growth rates to interpret ambient observations.
Experiments at CLOUD show that in polluted environments new particle formation (NPF) is largely...
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