Articles | Volume 21, issue 17
https://doi.org/10.5194/acp-21-13713-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-13713-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
14 Sep 2021
Research article |
| 14 Sep 2021
| 14 Sep 2021
A comprehensive observation-based multiphase chemical model analysis of sulfur dioxide oxidations in both summer and winter
Huan Song
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Huabin Dong
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Shule Li
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Shiyi Chen
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Zhijun Wu
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Mei Zheng
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Limin Zeng
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
Yuanhang Zhang
State Key Joint Laboratory or Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing, China
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Total article views: 2,072 (including HTML, PDF, and XML)
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Total article views: 790 (including HTML, PDF, and XML)
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Cited
14 citations as recorded by crossref.
- Key Factors Determining the Formation of Sulfate Aerosols Through Multiphase Chemistry—A Kinetic Modeling Study Based on Beijing Conditions T. Wang et al. 10.1029/2022JD038382
- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Factors affecting recent PM2.5 concentrations in China and South Korea from 2016 to 2020 Y. Cha et al. 10.1016/j.scitotenv.2023.163524
- Reduced Aerosol Uptake of Hydroperoxyl Radical May Increase the Sensitivity of Ozone Production to Volatile Organic Compounds H. Song et al. 10.1021/acs.estlett.1c00893
- Modeling particulate nitrate in China: Current findings and future directions X. Xie et al. 10.1016/j.envint.2022.107369
- Technical Note: A technique to convert NO2 to NO2− with S(IV) and its application to measuring nitrate photolysis A. Lieberman et al. 10.5194/acp-24-4411-2024
- Investigation of a haze-to-dust and dust swing process at a coastal city in northern China part II: A study on the solubility of iron and manganese across aerosol sources and secondary processes M. Sun et al. 10.1016/j.atmosenv.2024.120532
- Box Model Applications for Secondary Inorganic Aerosol: A Review Focused on Nitrate Formation S. Park 10.5572/KOSAE.2024.40.1.1
- Critical Roles of Surface-Enhanced Heterogeneous Oxidation of SO2 in Haze Chemistry: Review of Extended Pathways for Complex Air Pollution Z. Zhang et al. 10.1007/s40726-023-00287-2
- Assessment of Secondary Sulfate Aqueous-Phase Formation Pathways in the Tropical Island City of Haikou: A Chemical Kinetic Perspective C. Wang et al. 10.3390/toxics12020105
- Trace Metals Reveal Significant Contribution of Coal Combustion to Winter Haze Pollution in Northern China H. Shen et al. 10.1021/acsestair.4c00050
- High fraction of soluble trace metals in fine particles under heavy haze in central China M. Liu et al. 10.1016/j.scitotenv.2022.156771
- The important role of nitrate in iron and manganese dissolution and sulfate formation in fine particles at a coastal site in Northern China X. Gao et al. 10.1016/j.scitotenv.2024.170318
- A critical review of sulfate aerosol formation mechanisms during winter polluted periods C. Ye et al. 10.1016/j.jes.2022.07.011
14 citations as recorded by crossref.
- Key Factors Determining the Formation of Sulfate Aerosols Through Multiphase Chemistry—A Kinetic Modeling Study Based on Beijing Conditions T. Wang et al. 10.1029/2022JD038382
- Significant formation of sulfate aerosols contributed by the heterogeneous drivers of dust surface T. Wang et al. 10.5194/acp-22-13467-2022
- Factors affecting recent PM2.5 concentrations in China and South Korea from 2016 to 2020 Y. Cha et al. 10.1016/j.scitotenv.2023.163524
- Reduced Aerosol Uptake of Hydroperoxyl Radical May Increase the Sensitivity of Ozone Production to Volatile Organic Compounds H. Song et al. 10.1021/acs.estlett.1c00893
- Modeling particulate nitrate in China: Current findings and future directions X. Xie et al. 10.1016/j.envint.2022.107369
- Technical Note: A technique to convert NO2 to NO2− with S(IV) and its application to measuring nitrate photolysis A. Lieberman et al. 10.5194/acp-24-4411-2024
- Investigation of a haze-to-dust and dust swing process at a coastal city in northern China part II: A study on the solubility of iron and manganese across aerosol sources and secondary processes M. Sun et al. 10.1016/j.atmosenv.2024.120532
- Box Model Applications for Secondary Inorganic Aerosol: A Review Focused on Nitrate Formation S. Park 10.5572/KOSAE.2024.40.1.1
- Critical Roles of Surface-Enhanced Heterogeneous Oxidation of SO2 in Haze Chemistry: Review of Extended Pathways for Complex Air Pollution Z. Zhang et al. 10.1007/s40726-023-00287-2
- Assessment of Secondary Sulfate Aqueous-Phase Formation Pathways in the Tropical Island City of Haikou: A Chemical Kinetic Perspective C. Wang et al. 10.3390/toxics12020105
- Trace Metals Reveal Significant Contribution of Coal Combustion to Winter Haze Pollution in Northern China H. Shen et al. 10.1021/acsestair.4c00050
- High fraction of soluble trace metals in fine particles under heavy haze in central China M. Liu et al. 10.1016/j.scitotenv.2022.156771
- The important role of nitrate in iron and manganese dissolution and sulfate formation in fine particles at a coastal site in Northern China X. Gao et al. 10.1016/j.scitotenv.2024.170318
- A critical review of sulfate aerosol formation mechanisms during winter polluted periods C. Ye et al. 10.1016/j.jes.2022.07.011
Latest update: 13 Dec 2024
Short summary
Secondary sulfate aerosols are an important component of fine particles in severe air pollution events. We calculated the sulfate formation rates via a state-of-the-art multiphase model constrained to the observed values. We showed that transition metals in urban aerosols contribute significantly to sulfate formation during haze periods and thus play an important role in mitigation strategies and public health measures in megacities worldwide.
Secondary sulfate aerosols are an important component of fine particles in severe air pollution...
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