Articles | Volume 21, issue 17
https://doi.org/10.5194/acp-21-13483-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-13483-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds
Andreas Tilgner
Atmospheric Chemistry Department (ACD), Leibniz Institute for Tropospheric Research (TROPOS), Leipzig 04318, Germany
Thomas Schaefer
Atmospheric Chemistry Department (ACD), Leibniz Institute for Tropospheric Research (TROPOS), Leipzig 04318, Germany
Becky Alexander
Department of Atmospheric Science, University of Washington, Seattle, WA 98195, USA
Mary Barth
Atmospheric Chemistry Observation & Modeling Laboratory, National Center for Atmospheric Research, Boulder, CO 80307, USA
Jeffrey L. Collett Jr.
Department of Atmospheric Science, Colorado State University, Fort Collins, CO 80523, USA
Kathleen M. Fahey
Office of Research and Development, U.S. Environmental Protection Agency, Research Triangle Park, Durham, NC 27711, USA
Athanasios Nenes
School of Architecture, Civil and Environmental Engineering, École Polytechnique Fédérale de Lausanne, Lausanne 1015, Switzerland
Institute for Chemical Engineering Sciences, Foundation for Research and Technology Hellas, Patras 26504, Greece
Havala O. T. Pye
Office of Research and Development, U.S. Environmental Protection Agency, Research Triangle Park, Durham, NC 27711, USA
Atmospheric Chemistry Department (ACD), Leibniz Institute for Tropospheric Research (TROPOS), Leipzig 04318, Germany
Department of Chemical Engineering, Columbia University, New York, NY 10027, USA
Department of Earth and Environmental Sciences, Columbia University, New York, NY 10027, USA
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Feedbacks of acidity and atmospheric multiphase chemistry in deliquesced particles and clouds are crucial for the tropospheric composition, depositions, climate, and human health. This review synthesizes the current scientific knowledge on these feedbacks using both inorganic and organic aqueous-phase chemistry. Finally, this review outlines atmospheric implications and highlights the need for future investigations with respect to reducing emissions of key acid precursors in a changing world.
Feedbacks of acidity and atmospheric multiphase chemistry in deliquesced particles and clouds...
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