Articles | Volume 21, issue 17
https://doi.org/10.5194/acp-21-12989-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-12989-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Sep 2021
Research article |
| 02 Sep 2021
| 02 Sep 2021
Optical properties of coated black carbon aggregates: numerical simulations, radiative forcing estimates, and size-resolved parameterization scheme
Baseerat Romshoo
CORRESPONDING AUTHOR
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Thomas Müller
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Sascha Pfeifer
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Jorge Saturno
PTB Physikalisch-Technische Bundesanstalt, 38116 Braunschweig,
Germany
Andreas Nowak
PTB Physikalisch-Technische Bundesanstalt, 38116 Braunschweig,
Germany
Krzysztof Ciupek
Environment Department, National Physical Laboratory (NPL),
Teddington, TW11 0LW, UK
Paul Quincey
Environment Department, National Physical Laboratory (NPL),
Teddington, TW11 0LW, UK
Alfred Wiedensohler
Leibniz Institute for Tropospheric Research, 04318 Leipzig, Germany
Viewed
Total article views: 4,255 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 15 Jan 2021)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,859 | 1,329 | 67 | 4,255 | 356 | 53 | 71 |
- HTML: 2,859
- PDF: 1,329
- XML: 67
- Total: 4,255
- Supplement: 356
- BibTeX: 53
- EndNote: 71
Total article views: 3,044 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 02 Sep 2021)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 2,181 | 806 | 57 | 3,044 | 181 | 50 | 62 |
- HTML: 2,181
- PDF: 806
- XML: 57
- Total: 3,044
- Supplement: 181
- BibTeX: 50
- EndNote: 62
Total article views: 1,211 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 15 Jan 2021)
| HTML | XML | Total | Supplement | BibTeX | EndNote | |
|---|---|---|---|---|---|---|
| 678 | 523 | 10 | 1,211 | 175 | 3 | 9 |
- HTML: 678
- PDF: 523
- XML: 10
- Total: 1,211
- Supplement: 175
- BibTeX: 3
- EndNote: 9
Viewed (geographical distribution)
Total article views: 4,255 (including HTML, PDF, and XML)
Thereof 4,255 with geography defined
and 0 with unknown origin.
Total article views: 3,044 (including HTML, PDF, and XML)
Thereof 3,044 with geography defined
and 0 with unknown origin.
Total article views: 1,211 (including HTML, PDF, and XML)
Thereof 1,211 with geography defined
and 0 with unknown origin.
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Country | # | Views | % |
|---|
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
| Total: | 0 |
| HTML: | 0 |
| PDF: | 0 |
| XML: | 0 |
- 1
1
Cited
28 citations as recorded by crossref.
- Relationship between light absorption properties of black carbon and aerosol origin at a background coastal site H. Li et al. 10.1016/j.scitotenv.2023.163863
- Improved representation of black carbon mixing structures suggests stronger direct radiative heating Y. Wang et al. 10.1016/j.oneear.2025.101311
- Carbonaceous Nanoparticle Air Pollution: Toxicity and Detection in Biological Samples I. Aslam & M. Roeffaers 10.3390/nano12223948
- Numerical investigation on the accuracy of size information of fractal soot aerosols retrieved by lidar: Optical property, morphology effect, and parameterization scheme J. Liu et al. 10.1016/j.jqsrt.2022.108435
- Measurements and calculations of enhanced side- and back-scattering of visible radiation by black carbon aggregates C. Haspel et al. 10.5194/acp-23-10091-2023
- Understanding the mechanism and importance of brown carbon bleaching across the visible spectrum in biomass burning plumes from the WE-CAN campaign Y. Shen et al. 10.5194/acp-24-12881-2024
- Significant contribution of fractal morphology to aerosol light absorption in polluted environments dominated by black carbon (BC) B. Romshoo et al. 10.1038/s41612-024-00634-0
- Siberian Arctic black carbon: gas flaring and wildfire impact O. Popovicheva et al. 10.5194/acp-22-5983-2022
- Fresh organic and soot particles from crop straw burning: Morphology, composition and size distribution Y. Li et al. 10.1002/gj.4861
- Constraining the particle-scale diversity of black carbon light absorption using a unified framework P. Beeler & R. Chakrabarty 10.5194/acp-22-14825-2022
- Particle size amplification of black carbon by scattering measurement due to morphology diversity Y. Wu et al. 10.1088/1748-9326/acaede
- Assessing direct radiative effect of aging black carbon using an advanced aerosol optics module AI-NAOS and the climate model CAM6 X. Wang et al. 10.1038/s41612-025-01080-2
- Ambient aerosol properties in the remote atmosphere from global-scale in situ measurements C. Brock et al. 10.5194/acp-21-15023-2021
- Improving the predictions of black carbon (BC) optical properties at various aging stages using a machine-learning-based approach B. Romshoo et al. 10.5194/acp-24-8821-2024
- Black carbon in contrasting environments in India: Temporal variability, source apportionment and radiative forcing B. Romshoo et al. 10.1016/j.atmosenv.2023.119734
- Validation of cantilever-enhanced photoacoustic particle-size-resolved light absorption measurement using nigrosin reference particles and Mie modelling J. Kuula et al. 10.5194/ar-3-1-2025
- Analysis of Aerosol Characteristics through Stereoscopic Observation of the West Sea during the 2019 YES-AQ Campaign M. Jeong et al. 10.5572/KOSAE.2022.38.6.823
- Black carbon, organic carbon, and mineral dust in South American tropical glaciers: A review S. Gilardoni et al. 10.1016/j.gloplacha.2022.103837
- Challenges and policy implications of long-term changes in mass absorption cross-section derived from equivalent black carbon and elemental carbon measurements in London and south-east England in 2014–2019 K. Ciupek et al. 10.1039/D1EM00200G
- Quantifying the effects of the microphysical hygroscopic restructuring of soot on ensemble optical properties and satellite aerosol optical depth retrievals K. Chang et al. 10.1016/j.scitotenv.2024.177821
- Photochemical Aging Induces Changes in the Effective Densities, Morphologies, and Optical Properties of Combustion Aerosol Particles J. Leskinen et al. 10.1021/acs.est.2c04151
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Importance of size representation and morphology in modelling optical properties of black carbon: comparison between laboratory measurements and model simulations B. Romshoo et al. 10.5194/amt-15-6965-2022
- Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts W. Li et al. 10.1038/s41612-024-00610-8
- Comparison of scanning aerosol lidar and in situ measurements of aerosol physical properties and boundary layer heights H. Zhang et al. 10.5194/ar-2-135-2024
- Seasonal, Weekly, and Diurnal Black Carbon in Moscow Megacity Background under Impact of Urban and Regional Sources O. Popovicheva et al. 10.3390/atmos13040563
- Contribution of brown carbon to light absorption in emissions of European residential biomass combustion appliances S. Basnet et al. 10.5194/acp-24-3197-2024
- Using convolutional neural networks to predict the optical properties of coated black carbon Z. Qin et al. 10.1016/j.jqsrt.2024.109326
28 citations as recorded by crossref.
- Relationship between light absorption properties of black carbon and aerosol origin at a background coastal site H. Li et al. 10.1016/j.scitotenv.2023.163863
- Improved representation of black carbon mixing structures suggests stronger direct radiative heating Y. Wang et al. 10.1016/j.oneear.2025.101311
- Carbonaceous Nanoparticle Air Pollution: Toxicity and Detection in Biological Samples I. Aslam & M. Roeffaers 10.3390/nano12223948
- Numerical investigation on the accuracy of size information of fractal soot aerosols retrieved by lidar: Optical property, morphology effect, and parameterization scheme J. Liu et al. 10.1016/j.jqsrt.2022.108435
- Measurements and calculations of enhanced side- and back-scattering of visible radiation by black carbon aggregates C. Haspel et al. 10.5194/acp-23-10091-2023
- Understanding the mechanism and importance of brown carbon bleaching across the visible spectrum in biomass burning plumes from the WE-CAN campaign Y. Shen et al. 10.5194/acp-24-12881-2024
- Significant contribution of fractal morphology to aerosol light absorption in polluted environments dominated by black carbon (BC) B. Romshoo et al. 10.1038/s41612-024-00634-0
- Siberian Arctic black carbon: gas flaring and wildfire impact O. Popovicheva et al. 10.5194/acp-22-5983-2022
- Fresh organic and soot particles from crop straw burning: Morphology, composition and size distribution Y. Li et al. 10.1002/gj.4861
- Constraining the particle-scale diversity of black carbon light absorption using a unified framework P. Beeler & R. Chakrabarty 10.5194/acp-22-14825-2022
- Particle size amplification of black carbon by scattering measurement due to morphology diversity Y. Wu et al. 10.1088/1748-9326/acaede
- Assessing direct radiative effect of aging black carbon using an advanced aerosol optics module AI-NAOS and the climate model CAM6 X. Wang et al. 10.1038/s41612-025-01080-2
- Ambient aerosol properties in the remote atmosphere from global-scale in situ measurements C. Brock et al. 10.5194/acp-21-15023-2021
- Improving the predictions of black carbon (BC) optical properties at various aging stages using a machine-learning-based approach B. Romshoo et al. 10.5194/acp-24-8821-2024
- Black carbon in contrasting environments in India: Temporal variability, source apportionment and radiative forcing B. Romshoo et al. 10.1016/j.atmosenv.2023.119734
- Validation of cantilever-enhanced photoacoustic particle-size-resolved light absorption measurement using nigrosin reference particles and Mie modelling J. Kuula et al. 10.5194/ar-3-1-2025
- Analysis of Aerosol Characteristics through Stereoscopic Observation of the West Sea during the 2019 YES-AQ Campaign M. Jeong et al. 10.5572/KOSAE.2022.38.6.823
- Black carbon, organic carbon, and mineral dust in South American tropical glaciers: A review S. Gilardoni et al. 10.1016/j.gloplacha.2022.103837
- Challenges and policy implications of long-term changes in mass absorption cross-section derived from equivalent black carbon and elemental carbon measurements in London and south-east England in 2014–2019 K. Ciupek et al. 10.1039/D1EM00200G
- Quantifying the effects of the microphysical hygroscopic restructuring of soot on ensemble optical properties and satellite aerosol optical depth retrievals K. Chang et al. 10.1016/j.scitotenv.2024.177821
- Photochemical Aging Induces Changes in the Effective Densities, Morphologies, and Optical Properties of Combustion Aerosol Particles J. Leskinen et al. 10.1021/acs.est.2c04151
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Importance of size representation and morphology in modelling optical properties of black carbon: comparison between laboratory measurements and model simulations B. Romshoo et al. 10.5194/amt-15-6965-2022
- Microphysical properties of atmospheric soot and organic particles: measurements, modeling, and impacts W. Li et al. 10.1038/s41612-024-00610-8
- Comparison of scanning aerosol lidar and in situ measurements of aerosol physical properties and boundary layer heights H. Zhang et al. 10.5194/ar-2-135-2024
- Seasonal, Weekly, and Diurnal Black Carbon in Moscow Megacity Background under Impact of Urban and Regional Sources O. Popovicheva et al. 10.3390/atmos13040563
- Contribution of brown carbon to light absorption in emissions of European residential biomass combustion appliances S. Basnet et al. 10.5194/acp-24-3197-2024
- Using convolutional neural networks to predict the optical properties of coated black carbon Z. Qin et al. 10.1016/j.jqsrt.2024.109326
Latest update: 27 May 2025
Short summary
Modifications in the optical properties of black carbon (BC) due to ageing are presented and quantified in this study using a state-of-the-art description scheme of BC fractal aggregates. It is shown that the relative change in BC radiative forcing can be larger than 50 % as a function of changing fractal dimension and organic content. A comprehensive parameterization scheme for coated BC optical properties is developed with applications for modelling, ambient, and laboratory-based BC studies.
Modifications in the optical properties of black carbon (BC) due to ageing are presented and...
Altmetrics
Final-revised paper
Preprint