Articles | Volume 21, issue 17
https://doi.org/10.5194/acp-21-12809-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-12809-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
31 Aug 2021
Research article |
| 31 Aug 2021
| 31 Aug 2021
Source-specific light absorption by carbonaceous components in the complex aerosol matrix from yearly filter-based measurements
Vaios Moschos
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
Martin Gysel-Beer
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
Robin L. Modini
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
Joel C. Corbin
Metrology Research Centre, National Research Council Canada, Ottawa,
ON K1A 0R6, Canada
Dario Massabò
Department of Physics, University of
Genoa, Genoa, 16146, Italy
National Institute for Nuclear Physics (INFN), University of Genoa, Genoa, 16146, Italy
Camilla Costa
Department of Chemistry and Industrial Chemistry, University of Genoa, Genoa, 16146, Italy
Silvia G. Danelli
National Institute for Nuclear Physics (INFN), University of Genoa, Genoa, 16146, Italy
Athanasia Vlachou
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
Kaspar R. Daellenbach
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
Sönke Szidat
Department of Chemistry, Biochemistry and Pharmaceutical Sciences, University of Bern, Bern, 3012, Switzerland
Oeschger Centre for Climate Change Research, University of Bern, Bern, 3012, Switzerland
Paolo Prati
Department of Physics, University of
Genoa, Genoa, 16146, Italy
National Institute for Nuclear Physics (INFN), University of Genoa, Genoa, 16146, Italy
André S. H. Prévôt
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute,
Villigen, 5232, Switzerland
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Cited
14 citations as recorded by crossref.
- Elucidating the present-day chemical composition, seasonality and source regions of climate-relevant aerosols across the Arctic land surface V. Moschos et al. 10.1088/1748-9326/ac444b
- Combined influences of sources and atmospheric bleaching on light absorption of water-soluble brown carbon aerosols W. Fang et al. 10.1038/s41612-023-00438-8
- Potential underestimation of ambient brown carbon absorption based on the methanol extraction method and its impacts on source analysis Z. Xu et al. 10.5194/acp-22-13739-2022
- Particle size amplification of black carbon by scattering measurement due to morphology diversity Y. Wu et al. 10.1088/1748-9326/acaede
- Primary nature of brown carbon absorption in a frigid atmosphere with strong haze chemistry Y. Cheng et al. 10.1016/j.envres.2021.112324
- Characterization of soot produced by the mini inverted soot generator with an atmospheric simulation chamber V. Vernocchi et al. 10.5194/amt-15-2159-2022
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- Morphological and optical properties of carbonaceous aerosol particles from ship emissions and biomass burning during a summer cruise measurement in the South China Sea C. Sun et al. 10.5194/acp-24-3043-2024
- An optimised organic carbon ∕ elemental carbon (OC ∕ EC) fraction separation method for radiocarbon source apportionment applied to low-loaded Arctic aerosol filters M. Rauber et al. 10.5194/amt-16-825-2023
- Equal abundance of summertime natural and wintertime anthropogenic Arctic organic aerosols V. Moschos et al. 10.1038/s41561-021-00891-1
- Recommendations for reporting equivalent black carbon (eBC) mass concentrations based on long-term pan-European in-situ observations M. Savadkoohi et al. 10.1016/j.envint.2024.108553
- More water-soluble brown carbon after the residential “coal-to-gas” conversion measure in urban Beijing W. Yuan et al. 10.1038/s41612-023-00355-w
- Chromophores and chemical composition of brown carbon characterized at an urban kerbside by excitation–emission spectroscopy and mass spectrometry F. Jiang et al. 10.5194/acp-22-14971-2022
- Information content and aerosol property retrieval potential for different types of in situ polar nephelometer data A. Moallemi et al. 10.5194/amt-15-5619-2022
14 citations as recorded by crossref.
- Elucidating the present-day chemical composition, seasonality and source regions of climate-relevant aerosols across the Arctic land surface V. Moschos et al. 10.1088/1748-9326/ac444b
- Combined influences of sources and atmospheric bleaching on light absorption of water-soluble brown carbon aerosols W. Fang et al. 10.1038/s41612-023-00438-8
- Potential underestimation of ambient brown carbon absorption based on the methanol extraction method and its impacts on source analysis Z. Xu et al. 10.5194/acp-22-13739-2022
- Particle size amplification of black carbon by scattering measurement due to morphology diversity Y. Wu et al. 10.1088/1748-9326/acaede
- Primary nature of brown carbon absorption in a frigid atmosphere with strong haze chemistry Y. Cheng et al. 10.1016/j.envres.2021.112324
- Characterization of soot produced by the mini inverted soot generator with an atmospheric simulation chamber V. Vernocchi et al. 10.5194/amt-15-2159-2022
- Quantifying the Light-Absorption Properties and Molecular Composition of Brown Carbon Aerosol from Sub-Saharan African Biomass Combustion V. Moschos et al. 10.1021/acs.est.3c09378
- Morphological and optical properties of carbonaceous aerosol particles from ship emissions and biomass burning during a summer cruise measurement in the South China Sea C. Sun et al. 10.5194/acp-24-3043-2024
- An optimised organic carbon ∕ elemental carbon (OC ∕ EC) fraction separation method for radiocarbon source apportionment applied to low-loaded Arctic aerosol filters M. Rauber et al. 10.5194/amt-16-825-2023
- Equal abundance of summertime natural and wintertime anthropogenic Arctic organic aerosols V. Moschos et al. 10.1038/s41561-021-00891-1
- Recommendations for reporting equivalent black carbon (eBC) mass concentrations based on long-term pan-European in-situ observations M. Savadkoohi et al. 10.1016/j.envint.2024.108553
- More water-soluble brown carbon after the residential “coal-to-gas” conversion measure in urban Beijing W. Yuan et al. 10.1038/s41612-023-00355-w
- Chromophores and chemical composition of brown carbon characterized at an urban kerbside by excitation–emission spectroscopy and mass spectrometry F. Jiang et al. 10.5194/acp-22-14971-2022
- Information content and aerosol property retrieval potential for different types of in situ polar nephelometer data A. Moallemi et al. 10.5194/amt-15-5619-2022
Latest update: 26 Apr 2024
Short summary
This study provides a holistic approach to studying the spectrally resolved light absorption by atmospheric brown carbon (BrC) and black carbon using long time series of daily samples from filter-based measurements. The obtained results provide (1) a better understanding of the aerosol absorption profile and its dependence on BrC and on lensing from less absorbing coatings and (2) an estimation of the most important absorbers at typical European locations.
This study provides a holistic approach to studying the spectrally resolved light absorption by...
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