Articles | Volume 21, issue 14
https://doi.org/10.5194/acp-21-11437-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-21-11437-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
29 Jul 2021
Research article |
| 29 Jul 2021
| 29 Jul 2021
Atmospheric gaseous hydrochloric and hydrobromic acid in urban Beijing, China: detection, source identification and potential atmospheric impacts
Xiaolong Fan
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
Jing Cai
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Jian Zhao
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Yishuo Guo
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
Chang Li
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
Kaspar R. Dällenbach
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Feixue Zheng
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
Zhuohui Lin
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of
Sciences, Beijing 100085, China
Center for Excellence in Regional Atmospheric Environment,
Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021,
China
Yonghong Wang
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Lubna Dada
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Qiaozhi Zha
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Jenni Kontkanen
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Theo Kurtén
Department of Chemistry, University of Helsinki, Helsinki 00014, Finland
Siddhart Iyer
Aerosol Physics Laboratory, Physics Unit, Tampere University,
Tampere 33100, Finland
Joni T. Kujansuu
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Tuukka Petäjä
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Douglas R. Worsnop
Aerodyne Research Inc., Billerica, Massachusetts 01821, USA
Veli-Matti Kerminen
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Yongchun Liu
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
Federico Bianchi
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
School of Marine Sciences, Sun Yat-Sen University, Zhuhai 519082,
China
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Markku Kulmala
Aerosol and Haze Laboratory, Beijing Advanced Innovation Center for
Soft Matter Science and Engineering, Beijing University of Chemical
Technology, Beijing 100089, China
Institute for Atmospheric and Earth System Research (Physics), Faculty of Science, University of Helsinki, Helsinki 00560, Finland
Joint International Research Laboratory of Atmospheric and Earth
System Sciences (JirLATEST), Nanjing University, Nanjing 210023, China
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Cited
19 citations as recorded by crossref.
- Computational Investigation of Radical‐ and Catalyst‐Assisted Decomposition of CH2NO• to HCN S. Ghoshal & P. Sarkar 10.1002/cplu.202500295
- Halogen Emissions from Coal-Fired Power Plants in China: Evolutions, Driving Forces, and Future Trends Z. Fu et al. 10.1021/acs.est.4c12078
- Large presence of bromine and toxic metals in ambient fine particles from urban fires T. Li et al. 10.1016/j.atmosenv.2022.119554
- Characteristics, Origins, and Atmospheric Processes of Amines in Fine Aerosol Particles in Winter in China T. Liu et al. 10.1029/2023JD038974
- Elucidating the mechanisms of atmospheric new particle formation in the highly polluted Po Valley, Italy J. Cai et al. 10.5194/acp-24-2423-2024
- Changed mercury speciation in clouds driven by changing cloud water chemistry and impacts on photoreduction: Field evidence at Mt. Tai in eastern China J. Zhen et al. 10.1016/j.watres.2023.120402
- Midlatitude Ozone Depletion and Air Quality Impacts from Industrial Halogen Emissions in the Great Salt Lake Basin C. Womack et al. 10.1021/acs.est.2c05376
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
- Measurement report: Production and loss of atmospheric formaldehyde at a suburban site of Shanghai in summertime Y. Wu et al. 10.5194/acp-23-2997-2023
- Dust event identification and characterization with one-year online observations in Beijing F. Zheng et al. 10.1016/j.scitotenv.2024.177296
- Halogens Enhance Haze Pollution in China Q. Li et al. 10.1021/acs.est.1c01949
- Modeling the Global Impact of Chlorine Chemistry on Secondary Organic Aerosols X. Liu et al. 10.1021/acs.est.4c05037
- Study on the reactions of n-pentanal and n-hexanal with Br atoms: Kinetics, gas-phase products, and SOA formation C. Fan et al. 10.1016/j.atmosenv.2024.120869
- Observation based study on atmospheric oxidation capacity in Shanghai during late-autumn: Contribution from nitryl chloride S. Lou et al. 10.1016/j.atmosenv.2021.118902
- Widespread detection of chlorine oxyacids in the Arctic atmosphere Y. Tham et al. 10.1038/s41467-023-37387-y
- On the Chemical Pathways Influencing the Effective Global Warming Potential of Commercial Hydrofluoroolefin Gases G. Salierno 10.1002/cssc.202400280
- Isoprene–Chlorine Oxidation in the Presence of NOx and Implications for Urban Atmospheric Chemistry D. Wang et al. 10.1021/acs.est.1c07048
- Mechanisms of Reactions between HOI and HY (Y = Cl, Br, I) on a Water Nanodroplet Surface B. Tang & Z. Li 10.1021/acs.jpca.2c05414
- The semi-solid phase of atmospheric particles facilitates the formation of secondary brown carbon: Possible contribution of ionic strength to Maillard-like reactions J. Xie et al. 10.1016/j.atmosenv.2024.120991
19 citations as recorded by crossref.
- Computational Investigation of Radical‐ and Catalyst‐Assisted Decomposition of CH2NO• to HCN S. Ghoshal & P. Sarkar 10.1002/cplu.202500295
- Halogen Emissions from Coal-Fired Power Plants in China: Evolutions, Driving Forces, and Future Trends Z. Fu et al. 10.1021/acs.est.4c12078
- Large presence of bromine and toxic metals in ambient fine particles from urban fires T. Li et al. 10.1016/j.atmosenv.2022.119554
- Characteristics, Origins, and Atmospheric Processes of Amines in Fine Aerosol Particles in Winter in China T. Liu et al. 10.1029/2023JD038974
- Elucidating the mechanisms of atmospheric new particle formation in the highly polluted Po Valley, Italy J. Cai et al. 10.5194/acp-24-2423-2024
- Changed mercury speciation in clouds driven by changing cloud water chemistry and impacts on photoreduction: Field evidence at Mt. Tai in eastern China J. Zhen et al. 10.1016/j.watres.2023.120402
- Midlatitude Ozone Depletion and Air Quality Impacts from Industrial Halogen Emissions in the Great Salt Lake Basin C. Womack et al. 10.1021/acs.est.2c05376
- Characterization of offline analysis of particulate matter with FIGAERO-CIMS J. Cai et al. 10.5194/amt-16-1147-2023
- Measurement report: Production and loss of atmospheric formaldehyde at a suburban site of Shanghai in summertime Y. Wu et al. 10.5194/acp-23-2997-2023
- Dust event identification and characterization with one-year online observations in Beijing F. Zheng et al. 10.1016/j.scitotenv.2024.177296
- Halogens Enhance Haze Pollution in China Q. Li et al. 10.1021/acs.est.1c01949
- Modeling the Global Impact of Chlorine Chemistry on Secondary Organic Aerosols X. Liu et al. 10.1021/acs.est.4c05037
- Study on the reactions of n-pentanal and n-hexanal with Br atoms: Kinetics, gas-phase products, and SOA formation C. Fan et al. 10.1016/j.atmosenv.2024.120869
- Observation based study on atmospheric oxidation capacity in Shanghai during late-autumn: Contribution from nitryl chloride S. Lou et al. 10.1016/j.atmosenv.2021.118902
- Widespread detection of chlorine oxyacids in the Arctic atmosphere Y. Tham et al. 10.1038/s41467-023-37387-y
- On the Chemical Pathways Influencing the Effective Global Warming Potential of Commercial Hydrofluoroolefin Gases G. Salierno 10.1002/cssc.202400280
- Isoprene–Chlorine Oxidation in the Presence of NOx and Implications for Urban Atmospheric Chemistry D. Wang et al. 10.1021/acs.est.1c07048
- Mechanisms of Reactions between HOI and HY (Y = Cl, Br, I) on a Water Nanodroplet Surface B. Tang & Z. Li 10.1021/acs.jpca.2c05414
- The semi-solid phase of atmospheric particles facilitates the formation of secondary brown carbon: Possible contribution of ionic strength to Maillard-like reactions J. Xie et al. 10.1016/j.atmosenv.2024.120991
Latest update: 13 Jul 2025
Short summary
We observed significant concentrations of gaseous HBr and HCl throughout the winter and springtime in urban Beijing, China. Our results indicate that gaseous HCl and HBr are most likely originated from anthropogenic emissions such as burning activities, and the gas–aerosol partitioning may play a crucial role in contributing to the gaseous HCl and HBr. These observations suggest that there is an important recycling pathway of halogen species in inland megacities.
We observed significant concentrations of gaseous HBr and HCl throughout the winter and...
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