Articles | Volume 21, issue 14
https://doi.org/10.5194/acp-21-11303-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-11303-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
28 Jul 2021
Research article |
| 28 Jul 2021
| 28 Jul 2021
Phase state of secondary organic aerosol in chamber photo-oxidation of mixed precursors
Centre for Atmospheric Science, Department of Earth and Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
Aristeidis Voliotis
Centre for Atmospheric Science, Department of Earth and Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
Yunqi Shao
Centre for Atmospheric Science, Department of Earth and Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
Taomou Zong
State Key Joint Laboratory of Environmental Simulation and Pollution Control, International Joint Laboratory for Regional Pollution Control, Ministry of Education (IJRC), College of Environmental Sciences and
Engineering, Peking University, Beijing 100871, China
Xiangxinyue Meng
State Key Joint Laboratory of Environmental Simulation and Pollution Control, International Joint Laboratory for Regional Pollution Control, Ministry of Education (IJRC), College of Environmental Sciences and
Engineering, Peking University, Beijing 100871, China
Centre for Atmospheric Science, Department of Earth and Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
Dawei Hu
Centre for Atmospheric Science, Department of Earth and Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
Ying Chen
Lancaster Environment Centre, Lancaster University, Lancaster LA1 4YQ, UK
currently at: Exeter Climate Systems, University of Exeter, Exeter
EX4 4QE, UK
Zhijun Wu
State Key Joint Laboratory of Environmental Simulation and Pollution Control, International Joint Laboratory for Regional Pollution Control, Ministry of Education (IJRC), College of Environmental Sciences and
Engineering, Peking University, Beijing 100871, China
International Joint Laboratory for Regional Pollution Control, 52425 Jülich, Germany, and Beijing 100871, China
Collaborative Innovation Center of Atmospheric Environment and
Equipment Technology, Nanjing University of Information Science and Technology, Nanjing 210044, China
M. Rami Alfarra
Centre for Atmospheric Science, Department of Earth and Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
National Centre for Atmospheric Science, School of Earth and
Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
Qatar Environment and Energy Research Institute, Hamad Bin Khalifa University, Doha, Qatar
Gordon McFiggans
CORRESPONDING AUTHOR
Centre for Atmospheric Science, Department of Earth and Environmental Sciences, The University of Manchester, Manchester M13 9PL, UK
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Cited
11 citations as recorded by crossref.
- Chamber investigation of the formation and transformation of secondary organic aerosol in mixtures of biogenic and anthropogenic volatile organic compounds A. Voliotis et al. 10.5194/acp-22-14147-2022
- Heterogeneous Nucleation Drives Particle Size Segregation in Sequential Ozone and Nitrate Radical Oxidation of Catechol L. Garofalo et al. 10.1021/acs.est.1c02984
- Glass Transition Temperatures of Organic Mixtures from Isoprene Epoxydiol-Derived Secondary Organic Aerosol B. Chen et al. 10.1021/acs.jpca.2c08936
- Characterisation of the Manchester Aerosol Chamber facility Y. Shao et al. 10.5194/amt-15-539-2022
- Relative Humidity Modulates the Physicochemical Processing of Secondary Brown Carbon Formation from Nighttime Oxidation of Furan and Pyrrole K. Chen et al. 10.1021/acsestair.4c00025
- On the evolution of sub- and super-saturated water uptake of secondary organic aerosol in chamber experiments from mixed precursors Y. Wang et al. 10.5194/acp-22-4149-2022
- Aerosolized algal bloom toxins are not inert E. Vejerano et al. 10.1039/D4EA00078A
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al. 10.1016/j.scitotenv.2024.177298
- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
- Secondary organic aerosol formation from monocyclic aromatic hydrocarbons: insights from laboratory studies Z. Yang et al. 10.1039/D1EM00409C
- Bibliometric analysis of photocatalytic oxidation of volatile organic compounds from 1998 to 2023 X. Zhu et al. 10.3389/fenvs.2024.1482766
11 citations as recorded by crossref.
- Chamber investigation of the formation and transformation of secondary organic aerosol in mixtures of biogenic and anthropogenic volatile organic compounds A. Voliotis et al. 10.5194/acp-22-14147-2022
- Heterogeneous Nucleation Drives Particle Size Segregation in Sequential Ozone and Nitrate Radical Oxidation of Catechol L. Garofalo et al. 10.1021/acs.est.1c02984
- Glass Transition Temperatures of Organic Mixtures from Isoprene Epoxydiol-Derived Secondary Organic Aerosol B. Chen et al. 10.1021/acs.jpca.2c08936
- Characterisation of the Manchester Aerosol Chamber facility Y. Shao et al. 10.5194/amt-15-539-2022
- Relative Humidity Modulates the Physicochemical Processing of Secondary Brown Carbon Formation from Nighttime Oxidation of Furan and Pyrrole K. Chen et al. 10.1021/acsestair.4c00025
- On the evolution of sub- and super-saturated water uptake of secondary organic aerosol in chamber experiments from mixed precursors Y. Wang et al. 10.5194/acp-22-4149-2022
- Aerosolized algal bloom toxins are not inert E. Vejerano et al. 10.1039/D4EA00078A
- Hydrogel network formation triggers atypical hygroscopic behavior in atmospheric aerosols F. Dong et al. 10.1016/j.scitotenv.2024.177298
- Organic Coating Reduces Hygroscopic Growth of Phase-Separated Aerosol Particles W. Li et al. 10.1021/acs.est.1c05901
- Secondary organic aerosol formation from monocyclic aromatic hydrocarbons: insights from laboratory studies Z. Yang et al. 10.1039/D1EM00409C
- Bibliometric analysis of photocatalytic oxidation of volatile organic compounds from 1998 to 2023 X. Zhu et al. 10.3389/fenvs.2024.1482766
Latest update: 22 Nov 2024
Short summary
Aerosol phase behaviour plays a profound role in atmospheric physicochemical processes. We designed dedicated chamber experiments to study the phase state of secondary organic aerosol from biogenic and anthropogenic mixed precursors. Our results highlight the key role of the organic–inorganic ratio and relative humidity in phase state, but the sources and organic composition are less important. The result provides solid laboratory evidence for understanding aerosol phase in a complex atmosphere.
Aerosol phase behaviour plays a profound role in atmospheric physicochemical processes. We...
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