Articles | Volume 20, issue 8
https://doi.org/10.5194/acp-20-4607-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-4607-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
21 Apr 2020
Research article |
| 21 Apr 2020
| 21 Apr 2020
Characterization of organic aerosol across the global remote troposphere: a comparison of ATom measurements and global chemistry models
Alma Hodzic
CORRESPONDING AUTHOR
National Center for Atmospheric Research, Boulder, CO, USA
Pedro Campuzano-Jost
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Huisheng Bian
NASA Goddard Space Flight Center, Greenbelt, MD, USA
Mian Chin
NASA Goddard Space Flight Center, Greenbelt, MD, USA
Peter R. Colarco
NASA Goddard Space Flight Center, Greenbelt, MD, USA
Douglas A. Day
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Karl D. Froyd
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO, USA
Bernd Heinold
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Duseong S. Jo
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Joseph M. Katich
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO, USA
John K. Kodros
Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
Benjamin A. Nault
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Jeffrey R. Pierce
Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO, USA
Jacob Schacht
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Gregory P. Schill
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO, USA
Jason C. Schroder
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Joshua P. Schwarz
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO, USA
Donna T. Sueper
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
Ina Tegen
Leibniz Institute for Tropospheric Research, Leipzig, Germany
Simone Tilmes
National Center for Atmospheric Research, Boulder, CO, USA
Kostas Tsigaridis
Center for Climate Systems Research, Columbia University, New York, NY, USA
NASA Goddard Institute for Space Studies, New York, NY, USA
Pengfei Yu
NOAA Earth System Research Laboratory (ESRL), Chemical Sciences Division, Boulder, CO, USA
Institute for Environmental and Climate Research, Jinan University, Guangzhou, Guangdong, China
Jose L. Jimenez
Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado, Boulder, CO, USA
Department of Chemistry, University of Colorado, Boulder, CO, USA
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- Secondary aerosol formation during the dark oxidation of residential biomass burning emissions J. Kodros et al. 10.1039/D2EA00031H
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- Isoprene–Chlorine Oxidation in the Presence of NOx and Implications for Urban Atmospheric Chemistry D. Wang et al. 10.1021/acs.est.1c07048
59 citations as recorded by crossref.
- A Scheme for Representing Aromatic Secondary Organic Aerosols in Chemical Transport Models: Application to Source Attribution of Organic Aerosols Over South Korea During the KORUS‐AQ Campaign J. Brewer et al. 10.1029/2022JD037257
- Large contribution to secondary organic aerosol from isoprene cloud chemistry H. Lamkaddam et al. 10.1126/sciadv.abe2952
- Impact of the Atmospheric Photochemical Evolution of the Organic Component of Biomass Burning Aerosol on Its Radiative Forcing Efficiency: A Box Model Analysis T. Zhuravleva et al. 10.3390/atmos12121555
- Probing autoxidation of oleic acid at air-water interface: A neglected and significant pathway for secondary organic aerosols formation J. He et al. 10.1016/j.envres.2022.113232
- Secondary aerosol formation during the dark oxidation of residential biomass burning emissions J. Kodros et al. 10.1039/D2EA00031H
- Effects of volatility, viscosity, and non-ideality on particle–particle mixing timescales of secondary organic aerosols M. Schervish et al. 10.1080/02786826.2023.2256827
- Nitrogen oxides in the free troposphere: implications for tropospheric oxidants and the interpretation of satellite NO2 measurements V. Shah et al. 10.5194/acp-23-1227-2023
- Investigation of factors controlling PM2.5 variability across the South Korean Peninsula during KORUS-AQ C. Jordan et al. 10.1525/elementa.424
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- Aerosol pH indicator and organosulfate detectability from aerosol mass spectrometry measurements M. Schueneman et al. 10.5194/amt-14-2237-2021
- Marine biogenic emissions of benzene and toluene and their contribution to secondary organic aerosols over the polar oceans C. Wohl et al. 10.1126/sciadv.add9031
- Vertical Distribution of Alkanes in Atmospheric Aerosol in the Russian Arctic in September 2020 V. Arshinova et al. 10.1134/S1024856021060312
- Chemical transport models often underestimate inorganic aerosol acidity in remote regions of the atmosphere B. Nault et al. 10.1038/s43247-021-00164-0
- Evaluation of Biogenic Organic Aerosols in the Amazon Rainforest Using WRF‐Chem With MOSAIC J. Mao et al. 10.1029/2021JD034913
- Contribution of Organic Nitrates to Organic Aerosol over South Korea during KORUS-AQ H. Kenagy et al. 10.1021/acs.est.1c05521
- Secondary Organic Aerosol Mass Yields from NO3 Oxidation of α-Pinene and Δ-Carene: Effect of RO2 Radical Fate D. Day et al. 10.1021/acs.jpca.2c04419
- Altitude Aerosol Measurements in Central France: Seasonality, Sources and Free‐Troposphere/Boundary Layer Segregation A. Farah et al. 10.1029/2019EA001018
- The Role of Cloud Processing for the Ice Nucleating Ability of Organic Aerosol and Coal Fly Ash Particles K. Kilchhofer et al. 10.1029/2020JD033338
- The importance of size ranges in aerosol instrument intercomparisons: a case study for the Atmospheric Tomography Mission H. Guo et al. 10.5194/amt-14-3631-2021
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- Highly oxidized organic aerosols in Beijing: Possible contribution of aqueous-phase chemistry Z. Feng et al. 10.1016/j.atmosenv.2022.118971
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- Remote Aerosol Simulated During the Atmospheric Tomography (ATom) Campaign and Implications for Aerosol Lifetime C. Gao et al. 10.1029/2022JD036524
- Global Health and Climate Effects of Organic Aerosols from Different Sources D. Jo et al. 10.1021/acs.est.3c02823
- Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign S. Das et al. 10.5194/acp-24-4421-2024
- Accounting for Cloud Nucleation Activation Mechanism of Secondary Organic Matter from α-Pinene Oxidation Using Experimentally Retrieved Water Solubility Distributions W. Lee et al. 10.1021/acs.est.3c03039
- Benchmarking GOCART-2G in the Goddard Earth Observing System (GEOS) A. Collow et al. 10.5194/gmd-17-1443-2024
- An attribution of the low single-scattering albedo of biomass burning aerosol over the southeastern Atlantic A. Dobracki et al. 10.5194/acp-23-4775-2023
- Changes in sources and formation mechanisms of carbonaceous aerosols driven by short-term air pollution controls in Megacity Xi'an, China Z. Zhang et al. 10.1016/j.atmosenv.2024.120369
- Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vaporization techniques A. Hünig et al. 10.5194/amt-15-2889-2022
- Estimating Submicron Aerosol Mixing State at the Global Scale With Machine Learning and Earth System Modeling Z. Zheng et al. 10.1029/2020EA001500
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- Constraints on global aerosol number concentration, SO<sub>2</sub> and condensation sink in UKESM1 using ATom measurements A. Ranjithkumar et al. 10.5194/acp-21-4979-2021
- Contribution of Speciated Monoterpenes to Secondary Aerosol in the Eastern North Atlantic D. Kilgour et al. 10.1021/acsestair.3c00112
- Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations H. Bian et al. 10.5194/acp-24-1717-2024
- Future changes in isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) under the Shared Socioeconomic Pathways: the importance of physicochemical dependency D. Jo et al. 10.5194/acp-21-3395-2021
- Evolution of OH reactivity in NO-free volatile organic compound photooxidation investigated by the fully explicit GECKO-A model Z. Peng et al. 10.5194/acp-21-14649-2021
- On the differences in the vertical distribution of modeled aerosol optical depth over the southeastern Atlantic I. Chang et al. 10.5194/acp-23-4283-2023
- Fine Ash‐Bearing Particles as a Major Aerosol Component in Biomass Burning Smoke K. Adachi et al. 10.1029/2021JD035657
- Study of secondary organic aerosol formation and aging using ambient air in an oxidation flow reactor during high pollution events over Delhi V. Goel et al. 10.1016/j.envres.2024.118542
- Impact of stratospheric air and surface emissions on tropospheric nitrous oxide during ATom Y. Gonzalez et al. 10.5194/acp-21-11113-2021
- Evaluating the Impact of Chemical Complexity and Horizontal Resolution on Tropospheric Ozone Over the Conterminous US With a Global Variable Resolution Chemistry Model R. Schwantes et al. 10.1029/2021MS002889
- Review of Brown Carbon Aerosols in China: Pollution Level, Optical Properties, and Emissions Q. Wang et al. 10.1029/2021JD035473
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- Oxidation Flow Reactor Results in a Chinese Megacity Emphasize the Important Contribution of S/IVOCs to Ambient SOA Formation W. Hu et al. 10.1021/acs.est.1c03155
- Impacts of marine organic emissions on low-level stratiform clouds – a large eddy simulator study M. Prank et al. 10.5194/acp-22-10971-2022
Latest update: 13 Dec 2024
Short summary
Organic aerosol (OA) is a key source of uncertainty in aerosol climate effects. We present the first pole-to-pole OA characterization during the NASA Atmospheric Tomography aircraft mission. OA has a strong seasonal and zonal variability, with the highest levels in summer and over fire-influenced regions and the lowest ones in the southern high latitudes. We show that global models predict the OA distribution well but not the relative contribution of OA emissions vs. chemical production.
Organic aerosol (OA) is a key source of uncertainty in aerosol climate effects. We present the...
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