Articles | Volume 20, issue 6
https://doi.org/10.5194/acp-20-3793-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-3793-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Summertime and wintertime atmospheric processes of secondary aerosol in Beijing
Jing Duan
State Key Laboratory of Loess and Quaternary Geology, Key
Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an 710061, China
CAS Center for Excellence in Quaternary Science and Global Change,
Chinese Academy of Sciences, Xi'an 710061, China
University of Chinese Academy of Sciences, Beijing 100049, China
Ru-Jin Huang
CORRESPONDING AUTHOR
State Key Laboratory of Loess and Quaternary Geology, Key
Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an 710061, China
CAS Center for Excellence in Quaternary Science and Global Change,
Chinese Academy of Sciences, Xi'an 710061, China
Yongjie Li
Department of Civil and Environmental Engineering, Faculty of Science
and Technology, University of Macau, Taipa, Macau 999078, China
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Yan Zheng
State Key Joint Laboratory of Environmental Simulation and Pollution
Control, College of Environmental Sciences and Engineering, Peking
University, Beijing 100871, China
Yang Chen
Chongqing Institute of Green and Intelligent Technology, Chinese
Academy of Sciences, Chongqing 400714, China
Chunshui Lin
State Key Laboratory of Loess and Quaternary Geology, Key
Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an 710061, China
CAS Center for Excellence in Quaternary Science and Global Change,
Chinese Academy of Sciences, Xi'an 710061, China
Haiyan Ni
State Key Laboratory of Loess and Quaternary Geology, Key
Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an 710061, China
CAS Center for Excellence in Quaternary Science and Global Change,
Chinese Academy of Sciences, Xi'an 710061, China
Meng Wang
State Key Laboratory of Loess and Quaternary Geology, Key
Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an 710061, China
CAS Center for Excellence in Quaternary Science and Global Change,
Chinese Academy of Sciences, Xi'an 710061, China
Jurgita Ovadnevaite
School of Physics and Centre for Climate and Air Pollution Studies,
Ryan Institute, National University of Ireland Galway, University Road,
Galway, H91CF50, Ireland
Darius Ceburnis
School of Physics and Centre for Climate and Air Pollution Studies,
Ryan Institute, National University of Ireland Galway, University Road,
Galway, H91CF50, Ireland
Chunying Chen
CAS Key Laboratory for Biological Effects of Nanomaterials and
Nanosafety, National Centre for Nanoscience and Technology, Beijing 100191,
China
Douglas R. Worsnop
Aerodyne Research, Inc., Billerica, MA, USA
Thorsten Hoffmann
Institute of Inorganic and Analytical Chemistry, Johannes Gutenberg
University Mainz, Duesbergweg 10–14, 55128 Mainz, Germany
Colin O'Dowd
School of Physics and Centre for Climate and Air Pollution Studies,
Ryan Institute, National University of Ireland Galway, University Road,
Galway, H91CF50, Ireland
Junji Cao
State Key Laboratory of Loess and Quaternary Geology, Key
Laboratory of Aerosol Chemistry and Physics, Institute of Earth
Environment, Chinese Academy of Sciences, Xi'an 710061, China
CAS Center for Excellence in Quaternary Science and Global Change,
Chinese Academy of Sciences, Xi'an 710061, China
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67 citations as recorded by crossref.
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67 citations as recorded by crossref.
- Contrasting the characteristics, sources, and evolution of organic aerosols between summer and winter in a megacity of China J. Liu et al. 10.1016/j.scitotenv.2023.162937
- Response of warm season secondary pollutants to emissions and meteorology in the North China Plain region during 2018–2022 Y. Gao et al. 10.1016/j.aosl.2024.100495
- Comparative observation of aerosol vertical profiles in urban and suburban areas: Impacts of local and regional transport J. Zhu et al. 10.1016/j.scitotenv.2021.150363
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- The characterization of ambient levoglucosan in Beijing during summertime: Dynamic variation and source contributions under strong cooking influences J. Wang et al. 10.1016/j.jes.2024.08.029
- Impact of meteorological condition changes on air quality and particulate chemical composition during the COVID-19 lockdown J. Ding et al. 10.1016/j.jes.2021.02.022
- Understanding the Driving Forces of Summer PM1 Composition in Seoul, Korea, with Explainable Machine Learning Q. Hu et al. 10.1021/acsestair.3c00116
- Aqueous‐Phase Secondary Processes and Meteorological Change Promote the Brown Carbon Formation and Transformation During Haze Events H. Jiang et al. 10.1029/2023JD038735
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- Significant changes in autumn and winter aerosol composition and sources in Beijing from 2012 to 2018: Effects of clean air actions J. Li et al. 10.1016/j.envpol.2020.115855
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- Impact of aging on the sources, volatility, and viscosity of organic aerosols in Chinese outflows T. Feng et al. 10.5194/acp-23-611-2023
- Understanding secondary particles in a regional site of Yangtze River Delta: Insights from mass spectrometric measurement W. Zhu et al. 10.1016/j.scitotenv.2024.172994
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- Chemical characteristics and formation mechanism of secondary inorganic aerosols: The decisive role of aerosol acidity and meteorological conditions Y. Ting et al. 10.1016/j.envpol.2024.124472
- Chemical components of PM2.5 in different seasons in Harbin, China Q. Yu et al. 10.1016/j.partic.2022.08.002
- Control of particulate nitrate air pollution in China S. Zhai et al. 10.1038/s41561-021-00726-z
- Influence of ozone pollution on the mixing state and formation of oxygenated organics containing single particles S. Liu et al. 10.1016/j.scitotenv.2024.171880
- Characteristics, sources of volatile organic compounds, and their contributions to secondary air pollution during different periods in Beijing, China S. Liang et al. 10.1016/j.scitotenv.2022.159831
- Chemical composition, sources and evolution of wintertime inorganic and organic aerosols in urban Shanghai, China Y. Qian et al. 10.3389/fenvs.2023.1199652
- Ozone and SOA formation potential based on photochemical loss of VOCs during the Beijing summer J. Zhan et al. 10.1016/j.envpol.2021.117444
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- Aerosol acidity and its impact on sulfate and nitrate of PM2.5 in southern city of Beijing-Tianjin-Hebei region Z. Wei & N. Tahrin 10.1016/j.apr.2023.101997
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- Insight into wet scavenging effects on sulfur and nitrogen containing organic compounds in urban Beijing C. Zhang et al. 10.1038/s41612-024-00756-5
- The formation and evolution of secondary organic aerosol during summer in Xi'an: Aqueous phase processing in fog-rain days J. Duan et al. 10.1016/j.scitotenv.2020.144077
- Quantification of solid fuel combustion and aqueous chemistry contributions to secondary organic aerosol during wintertime haze events in Beijing Y. Tong et al. 10.5194/acp-21-9859-2021
- Chemical composition of NR-PM1 in a coastal city of Southeast China: Temporal variations and formation pathways Y. Chen et al. 10.1016/j.atmosenv.2022.119243
- Spatial variability of air pollutants in a megacity characterized by mobile measurements R. Khuzestani et al. 10.5194/acp-22-7389-2022
- Seasonal variations in the highly time-resolved aerosol composition, sources and chemical processes of background submicron particles in the North China Plain J. Li et al. 10.5194/acp-21-4521-2021
- Bayesian inference-based estimation of hourly primary and secondary organic carbon in suburban Hong Kong: multi-temporal-scale variations and evolution characteristics during PM2.5 episodes S. Wang et al. 10.5194/acp-24-5803-2024
- The effect of local pollution and transport dust on near surface aerosol properties over a semi-arid station from ground and satellite observations B. Akkiraju et al. 10.1007/s11869-023-01462-6
- Mapping the seamless hourly surface visibility in China: a real-time retrieval framework using a machine-learning-based stacked ensemble model X. Zhang et al. 10.1038/s41612-024-00617-1
- Weakened Gas-to-Particle Partitioning of Oxygenated Organic Molecules in Liquified Aerosol Particles W. Ma et al. 10.1021/acs.estlett.2c00556
- A novel prediction framework for estimating high spatial resolution near-ground PM2.5 and O3 concentrations at street-level in urban areas J. Xu et al. 10.1016/j.buildenv.2024.112141
- Secondary Formation of Submicron and Supermicron Organic and Inorganic Aerosols in a Highly Polluted Urban Area Y. Zheng et al. 10.1029/2022JD037865
- Exploring the driving factors of haze events in Beijing during Chinese New Year holidays in 2020 and 2021 under the influence of COVID-19 pandemic L. Luo et al. 10.1016/j.scitotenv.2022.160172
- Estimating the transboundary budget of sulfate aerosols in Northeast Asia with NASA MERRA aerosol reanalysis data D. Kwon et al. 10.1016/j.apr.2023.101981
- Significant Reductions in Secondary Aerosols after the Three-Year Action Plan in Beijing Summer Y. Li et al. 10.1021/acs.est.3c02417
- Measurements of traffic-dominated pollutant emissions in a Chinese megacity F. Squires et al. 10.5194/acp-20-8737-2020
- Seasonal source identification and formation processes of marine particulate water soluble organic nitrogen over an offshore island in the East China Sea M. Tian et al. 10.1016/j.scitotenv.2022.160895
- Substantial contribution of transported emissions to organic aerosol in Beijing K. Daellenbach et al. 10.1038/s41561-024-01493-3
- Mass spectral characterization of secondary organic aerosol from urban cooking and vehicular sources W. Zhu et al. 10.5194/acp-21-15065-2021
- Insights into aqueous-phase and photochemical formation of secondary organic aerosol in the winter of Beijing Y. Xiao et al. 10.1016/j.atmosenv.2021.118535
- Temperature-Dependent Composition of Summertime PM2.5 in Observations and Model Predictions across the Eastern U.S. P. Vannucci et al. 10.1021/acsearthspacechem.3c00333
- The seasonal variation of Asian dust, anthropogenic PM, and their sources in Dushanbe, Tajikistan K. Fomba et al. 10.1016/j.atmosenv.2024.120667
- Characteristics, primary sources and secondary formation of water-soluble organic aerosols in downtown Beijing Q. Yu et al. 10.5194/acp-21-1775-2021
- Measurement report: On the contribution of long-distance transport to the secondary aerosol formation and aging H. Zhong et al. 10.5194/acp-22-9513-2022
Latest update: 12 Nov 2024
Short summary
We characterized secondary aerosol formation in Beijing. Our results showed that relative humidity (RH) and Ox have opposite effects on sulfate and nitrate formation in summer and winter. The wintertime more-oxidized OOA (MO-OOA) showed a good correlation with aerosol liquid water content (ALWC). Meanwhile, the dependence of less-oxidized OOA (LO-OOA) and the mass ratio of LO-OOA to MO-OOA in Ox both degraded when RH > 60 %, suggesting that RH or ALWC may also affect LO-OOA formation.
We characterized secondary aerosol formation in Beijing. Our results showed that relative...
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