Articles | Volume 20, issue 1
https://doi.org/10.5194/acp-20-1-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-1-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Traffic-originated nanocluster emission exceeds H2SO4-driven photochemical new particle formation in an urban area
Aerosol Physics Laboratory, Physics Unit, Tampere University, 33014 Tampere, Finland
Heino Kuuluvainen
Aerosol Physics Laboratory, Physics Unit, Tampere University, 33014 Tampere, Finland
Minna Aurela
Atmospheric Composition Research, Finnish Meteorological Institute, 00101 Helsinki, Finland
Joni Kalliokoski
Aerosol Physics Laboratory, Physics Unit, Tampere University, 33014 Tampere, Finland
Niina Kuittinen
Aerosol Physics Laboratory, Physics Unit, Tampere University, 33014 Tampere, Finland
Mia Isotalo
Aerosol Physics Laboratory, Physics Unit, Tampere University, 33014 Tampere, Finland
Hilkka J. Timonen
Atmospheric Composition Research, Finnish Meteorological Institute, 00101 Helsinki, Finland
Jarkko V. Niemi
Helsinki Region Environmental Services Authority (HSY), 00066 HSY, Helsinki, Finland
Topi Rönkkö
Aerosol Physics Laboratory, Physics Unit, Tampere University, 33014 Tampere, Finland
Miikka Dal Maso
Aerosol Physics Laboratory, Physics Unit, Tampere University, 33014 Tampere, Finland
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- What is the spatiotemporal pattern of benzene concentration spread over susceptible area surrounding the Hartman Park community, Houston, Texas? A. Asri et al. 10.1016/j.jhazmat.2024.134666
- Engine preheating under real-world subfreezing conditions provides less than expected benefits to vehicle fuel economy and emission reduction for light-duty vehicles M. Olin et al. 10.1016/j.apenergy.2023.121805
- Road Traffic Emissions Lead to Much Enhanced New Particle Formation through Increased Growth Rates J. Brean et al. 10.1021/acs.est.3c10526
- Emerging Investigator Series: COVID-19 lockdown effects on aerosol particle size distributions in northern Italy J. Shen et al. 10.1039/D1EA00016K
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- Measurement report: The influence of traffic and new particle formation on the size distribution of 1–800 nm particles in Helsinki – a street canyon and an urban background station comparison M. Okuljar et al. 10.5194/acp-21-9931-2021
- Unprecedented Ambient Sulfur Trioxide (SO3) Detection: Possible Formation Mechanism and Atmospheric Implications L. Yao et al. 10.1021/acs.estlett.0c00615
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- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
- CFD modeling the diffusional losses of nanocluster-sized particles and condensing vapors in 90° bends of circular tubes M. Olin & M. Dal Maso 10.1016/j.jaerosci.2020.105618
- Thermodynamical framework for effective mitigation of high aerosol loading in the Indo-Gangetic Plain during winter P. Acharja et al. 10.1038/s41598-023-40657-w
- Molecular insights into new particle formation in Barcelona, Spain J. Brean et al. 10.5194/acp-20-10029-2020
- A phenomenology of new particle formation (NPF) at 13 European sites D. Bousiotis et al. 10.5194/acp-21-11905-2021
- Sub-23 nm Particles Dominate Non-Volatile Particle Number Emissions of Road Traffic H. Lintusaari et al. 10.1021/acs.est.3c03221
- The effect of meteorological conditions and atmospheric composition in the occurrence and development of new particle formation (NPF) events in Europe D. Bousiotis et al. 10.5194/acp-21-3345-2021
- Seasonality of the particle number concentration and size distribution: a global analysis retrieved from the network of Global Atmosphere Watch (GAW) near-surface observatories C. Rose et al. 10.5194/acp-21-17185-2021
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- High Concentration of Atmospheric Sub‐3 nm Particles in Polluted Environment of Eastern China: New Particle Formation and Traffic Emission L. Chen et al. 10.1029/2023JD039669
- Brownian coagulation of particles in the gasoline engine exhaust system: Experimental measurement and Monte Carlo simulation H. Liu et al. 10.1016/j.fuel.2021.121340
- An evaluation of new particle formation events in Helsinki during a Baltic Sea cyanobacterial summer bloom R. Thakur et al. 10.5194/acp-22-6365-2022
- Analysis of aerosol particle number size distribution and source attribution at three megacities in China D. Zhang et al. 10.1016/j.atmosenv.2022.119114
- Effect of industrial alkene ozonolysis on atmospheric H2SO4 formation X. Wang et al. 10.1016/j.jes.2023.11.012
- Contribution of traffic-originated nanoparticle emissions to regional and local aerosol levels M. Olin et al. 10.5194/acp-22-1131-2022
- Particle number size distribution and new particle formation in Xiamen, the coastal city of Southeast China in wintertime J. Wang et al. 10.1016/j.scitotenv.2022.154208
- Description and evaluation of the community aerosol dynamics model MAFOR v2.0 M. Karl et al. 10.5194/gmd-15-3969-2022
- Nanocluster aerosol formation via ozone chemistry on worn clothing: Influence of environmental parameters S. Yang & D. Licina 10.1016/j.buildenv.2024.111474
- Measurement report: Atmospheric new particle formation in a coastal agricultural site explained with binPMF analysis of nitrate CI-APi-TOF spectra M. Olin et al. 10.5194/acp-22-8097-2022
Latest update: 20 Nov 2024
Short summary
Photochemically formed sulfuric acid is generally considered the main source for new particle formation in the atmosphere. Contrary to current understanding, our measurements of nanoclusters and gaseous sulfuric acid performed in an urban area imply that traffic contributes to sulfuric acid concentration and that even for the smallest particles, the traffic-emitted fraction mostly exceeds the photochemistry-driven regional new particle formation.
Photochemically formed sulfuric acid is generally considered the main source for new particle...
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