Articles | Volume 19, issue 12
https://doi.org/10.5194/acp-19-8063-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-8063-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Jun 2019
Research article |
| 20 Jun 2019
| 20 Jun 2019
Significant source of secondary aerosol: formation from gasoline evaporative emissions in the presence of SO2 and NH3
Tianzeng Chen
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
Yongchun Liu
Beijing Advanced Innovation center for Soft Matter Science and
Engineering, Beijing University of Chemical Technology, Beijing 100029, China
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
Peng Zhang
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
Changgeng Liu
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
Jun Liu
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
University of Chinese Academy of Sciences, Beijing 100049, China
State Key Joint Laboratory of Environment Simulation and Pollution
Control, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China
University of Chinese Academy of Sciences, Beijing 100049, China
Center for Excellence in Regional Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
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46 citations as recorded by crossref.
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- Kinetics study of heterogeneous reactions of O3 and SO2 with sea salt single droplets using micro-FTIR spectroscopy: Potential for formation of sulfate aerosol in atmospheric environment X. He & Y. Zhang 10.1016/j.saa.2020.118219
- Review of Secondary Aerosol Formation and Its Contribution in Air Pollution Load of Delhi NCR M. Mishra et al. 10.1007/s11270-022-06047-0
- Measurement report: Effects of photochemical aging on the formation and evolution of summertime secondary aerosol in Beijing T. Chen et al. 10.5194/acp-21-1341-2021
- Assessing the influence of environmental conditions on secondary organic aerosol formation from a typical biomass burning compound X. Jiang et al. 10.1016/j.jes.2021.08.016
- NH3-promoted heterogeneous reaction of SO2 to sulfate on α-Fe2O3 particles with coexistence of NO2 under different relative humidities X. He et al. 10.1016/j.atmosenv.2021.118622
- Impacts of SO2, Relative Humidity, and Seed Acidity on Secondary Organic Aerosol Formation in the Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b02702
- Influence of Ammonia and Relative Humidity on the Formation and Composition of Secondary Brown Carbon from Oxidation of 1-Methylnaphthalene and Longifolene Y. Cui et al. 10.1021/acsearthspacechem.0c00353
- Dramatic decrease of secondary organic aerosol formation potential in Beijing: Important contribution from reduction of coal combustion emission J. Liu et al. 10.1016/j.scitotenv.2022.155045
- Impact of real-world traffic and super-emitters on vehicular emissions under inter-city driving conditions in Maharashtra, India S. Debbarma et al. 10.1016/j.apr.2024.102058
- A Comparison of the Evaporative Emissions Performance of Light-Duty Vehicles under US Tier 3 and China 6 Test Conditions D. Peng et al. 10.3390/atmos14071128
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
- Direct contribution of ammonia to <i>α</i>-pinene secondary organic aerosol formation L. Hao et al. 10.5194/acp-20-14393-2020
- Insights into the Peroxide-Bicyclic Intermediate Pathway of Aromatic Photooxidation: Experimental Yields and NOx-Dependency of Ring-Opening and Ring-Retaining Products S. He et al. 10.1021/acs.est.3c05304
- Insights into national distribution of NH3 concentrations in Republic of Korea: findings from passive sampler observations and implications for sources and management G. Yu et al. 10.1007/s10661-023-12288-1
- Synergetic effects of NH<sub>3</sub> and NO<sub><i>x</i></sub> on the production and optical absorption of secondary organic aerosol formation from toluene photooxidation S. Liu et al. 10.5194/acp-21-17759-2021
- A New Type of Quartz Smog Chamber: Design and Characterization W. Ma et al. 10.1021/acs.est.1c06341
- Synergistic generation mechanisms of SOA and ozone from the photochemical oxidation of 1,3,5-trimethylbenzene: Influence of precursors ratio, temperature and radiation intensity H. Zhang et al. 10.1016/j.atmosres.2023.106924
- Impacts of Mixed Gaseous and Particulate Pollutants on Secondary Particle Formation during Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b07650
- Smog Chamber Study on the Role of NOxin SOA and O3Formation from Aromatic Hydrocarbons T. Chen et al. 10.1021/acs.est.2c04022
- Effects of OH radical and SO2 concentrations on photochemical reactions of mixed anthropogenic organic gases J. Li et al. 10.5194/acp-22-10489-2022
- Comprehensive study about the heterogeneous conversion of NH3on nanoscale TiO2particles: insight into the mechanism and atmospheric implications Q. Ma et al. 10.1039/D2EN00966H
- Effects of NH3 on secondary aerosol formation from toluene/NOx photo-oxidation in different O3 formation regimes Z. Bao et al. 10.1016/j.atmosenv.2021.118603
- A large-scale outdoor atmospheric simulation smog chamber for studying atmospheric photochemical processes: Characterization and preliminary application J. Li et al. 10.1016/j.jes.2020.09.015
- Anthropogenic–Biogenic Interactions at Night: Enhanced Formation of Secondary Aerosols and Particulate Nitrogen- and Sulfur-Containing Organics from β-Pinene Oxidation L. Xu et al. 10.1021/acs.est.0c07879
- Enhanced secondary organic aerosol formation from the photo-oxidation of mixed anthropogenic volatile organic compounds J. Li et al. 10.5194/acp-21-7773-2021
- A new smog chamber system for atmospheric multiphase chemistry study: design and characterization T. Zong et al. 10.5194/amt-16-3679-2023
- Effect of NOx on secondary organic aerosol formation from the photochemical transformation of allyl acetate S. Wang et al. 10.1016/j.atmosenv.2021.118426
- Hydroxyl, hydroperoxyl free radicals determination methods in atmosphere and troposphere G. Wang et al. 10.1016/j.jes.2020.06.038
- SO<sub>2</sub> and NH<sub>3</sub> emissions enhance organosulfur compounds and fine particle formation from the photooxidation of a typical aromatic hydrocarbon Z. Yang et al. 10.5194/acp-21-7963-2021
- Synergistic Effects of SO2 and NH3 Coexistence on SOA Formation from Gasoline Evaporative Emissions T. Chen et al. 10.1021/acs.est.3c01921
- Application of smog chambers in atmospheric process studies B. Chu et al. 10.1093/nsr/nwab103
- NOx enhances secondary organic aerosol formation from nighttime γ-terpinene ozonolysis L. Xu et al. 10.1016/j.atmosenv.2020.117375
- Increased primary and secondary H<sub>2</sub>SO<sub>4</sub> showing the opposing roles in secondary organic aerosol formation from ethyl methacrylate ozonolysis P. Zhang et al. 10.5194/acp-21-7099-2021
- Source apportionment of ambient PM2.5 in Ho Chi Minh City, Vietnam N. Tran et al. 10.1007/s44273-023-00024-7
- Applications of environmental mass spectrometry in atmospheric haze chemistry T. Chen et al. 10.1016/j.trac.2024.117614
- Secondary Organic Aerosol Formation Potential from Vehicular Non-tailpipe Emissions under Real-World Driving Conditions J. Zhang et al. 10.1021/acs.est.3c06475
- Chemical characterization of submicron aerosol in summertime Beijing: A case study in southern suburbs in 2018 T. Chen et al. 10.1016/j.chemosphere.2020.125918
- Effect of relative humidity on SOA formation from aromatic hydrocarbons: Implications from the evolution of gas- and particle-phase species T. Chen et al. 10.1016/j.scitotenv.2021.145015
- NH3 Weakens the Enhancing Effect of SO2 on Biogenic Secondary Organic Aerosol Formation L. Du et al. 10.1021/acs.estlett.2c00959
- Monitoring gaseous pollutants using passive sampling in the Philadelphia region B. Terry & K. Shakya 10.1080/10962247.2023.2279733
- Particulate emissions from L-Category vehicles towards Euro 5 A. Kontses et al. 10.1016/j.envres.2019.109071
- Quantifying traffic, biomass burning and secondary source contributions to atmospheric particle number concentrations at urban and suburban sites J. Casquero-Vera et al. 10.1016/j.scitotenv.2021.145282
- Indoor Particulate Matter in Urban Households: Sources, Pathways, Characteristics, Health Effects, and Exposure Mitigation L. Zhang et al. 10.3390/ijerph182111055
- Effects of NO and SO2 on the secondary organic aerosol formation from the photooxidation of 1,3,5-trimethylbenzene: A new source of organosulfates Z. Yang et al. 10.1016/j.envpol.2020.114742
- Secondary organic aerosol formation from mixed volatile organic compounds: Effect of RO2 chemistry and precursor concentration T. Chen et al. 10.1038/s41612-022-00321-y
46 citations as recorded by crossref.
- Combined Smog Chamber/Oxidation Flow Reactor Study on Aging of Secondary Organic Aerosol from Photooxidation of Aromatic Hydrocarbons T. Chen et al. 10.1021/acs.est.3c04089
- Kinetics study of heterogeneous reactions of O3 and SO2 with sea salt single droplets using micro-FTIR spectroscopy: Potential for formation of sulfate aerosol in atmospheric environment X. He & Y. Zhang 10.1016/j.saa.2020.118219
- Review of Secondary Aerosol Formation and Its Contribution in Air Pollution Load of Delhi NCR M. Mishra et al. 10.1007/s11270-022-06047-0
- Measurement report: Effects of photochemical aging on the formation and evolution of summertime secondary aerosol in Beijing T. Chen et al. 10.5194/acp-21-1341-2021
- Assessing the influence of environmental conditions on secondary organic aerosol formation from a typical biomass burning compound X. Jiang et al. 10.1016/j.jes.2021.08.016
- NH3-promoted heterogeneous reaction of SO2 to sulfate on α-Fe2O3 particles with coexistence of NO2 under different relative humidities X. He et al. 10.1016/j.atmosenv.2021.118622
- Impacts of SO2, Relative Humidity, and Seed Acidity on Secondary Organic Aerosol Formation in the Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b02702
- Influence of Ammonia and Relative Humidity on the Formation and Composition of Secondary Brown Carbon from Oxidation of 1-Methylnaphthalene and Longifolene Y. Cui et al. 10.1021/acsearthspacechem.0c00353
- Dramatic decrease of secondary organic aerosol formation potential in Beijing: Important contribution from reduction of coal combustion emission J. Liu et al. 10.1016/j.scitotenv.2022.155045
- Impact of real-world traffic and super-emitters on vehicular emissions under inter-city driving conditions in Maharashtra, India S. Debbarma et al. 10.1016/j.apr.2024.102058
- A Comparison of the Evaporative Emissions Performance of Light-Duty Vehicles under US Tier 3 and China 6 Test Conditions D. Peng et al. 10.3390/atmos14071128
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
- Direct contribution of ammonia to <i>α</i>-pinene secondary organic aerosol formation L. Hao et al. 10.5194/acp-20-14393-2020
- Insights into the Peroxide-Bicyclic Intermediate Pathway of Aromatic Photooxidation: Experimental Yields and NOx-Dependency of Ring-Opening and Ring-Retaining Products S. He et al. 10.1021/acs.est.3c05304
- Insights into national distribution of NH3 concentrations in Republic of Korea: findings from passive sampler observations and implications for sources and management G. Yu et al. 10.1007/s10661-023-12288-1
- Synergetic effects of NH<sub>3</sub> and NO<sub><i>x</i></sub> on the production and optical absorption of secondary organic aerosol formation from toluene photooxidation S. Liu et al. 10.5194/acp-21-17759-2021
- A New Type of Quartz Smog Chamber: Design and Characterization W. Ma et al. 10.1021/acs.est.1c06341
- Synergistic generation mechanisms of SOA and ozone from the photochemical oxidation of 1,3,5-trimethylbenzene: Influence of precursors ratio, temperature and radiation intensity H. Zhang et al. 10.1016/j.atmosres.2023.106924
- Impacts of Mixed Gaseous and Particulate Pollutants on Secondary Particle Formation during Ozonolysis of Butyl Vinyl Ether P. Zhang et al. 10.1021/acs.est.9b07650
- Smog Chamber Study on the Role of NOxin SOA and O3Formation from Aromatic Hydrocarbons T. Chen et al. 10.1021/acs.est.2c04022
- Effects of OH radical and SO2 concentrations on photochemical reactions of mixed anthropogenic organic gases J. Li et al. 10.5194/acp-22-10489-2022
- Comprehensive study about the heterogeneous conversion of NH3on nanoscale TiO2particles: insight into the mechanism and atmospheric implications Q. Ma et al. 10.1039/D2EN00966H
- Effects of NH3 on secondary aerosol formation from toluene/NOx photo-oxidation in different O3 formation regimes Z. Bao et al. 10.1016/j.atmosenv.2021.118603
- A large-scale outdoor atmospheric simulation smog chamber for studying atmospheric photochemical processes: Characterization and preliminary application J. Li et al. 10.1016/j.jes.2020.09.015
- Anthropogenic–Biogenic Interactions at Night: Enhanced Formation of Secondary Aerosols and Particulate Nitrogen- and Sulfur-Containing Organics from β-Pinene Oxidation L. Xu et al. 10.1021/acs.est.0c07879
- Enhanced secondary organic aerosol formation from the photo-oxidation of mixed anthropogenic volatile organic compounds J. Li et al. 10.5194/acp-21-7773-2021
- A new smog chamber system for atmospheric multiphase chemistry study: design and characterization T. Zong et al. 10.5194/amt-16-3679-2023
- Effect of NOx on secondary organic aerosol formation from the photochemical transformation of allyl acetate S. Wang et al. 10.1016/j.atmosenv.2021.118426
- Hydroxyl, hydroperoxyl free radicals determination methods in atmosphere and troposphere G. Wang et al. 10.1016/j.jes.2020.06.038
- SO<sub>2</sub> and NH<sub>3</sub> emissions enhance organosulfur compounds and fine particle formation from the photooxidation of a typical aromatic hydrocarbon Z. Yang et al. 10.5194/acp-21-7963-2021
- Synergistic Effects of SO2 and NH3 Coexistence on SOA Formation from Gasoline Evaporative Emissions T. Chen et al. 10.1021/acs.est.3c01921
- Application of smog chambers in atmospheric process studies B. Chu et al. 10.1093/nsr/nwab103
- NOx enhances secondary organic aerosol formation from nighttime γ-terpinene ozonolysis L. Xu et al. 10.1016/j.atmosenv.2020.117375
- Increased primary and secondary H<sub>2</sub>SO<sub>4</sub> showing the opposing roles in secondary organic aerosol formation from ethyl methacrylate ozonolysis P. Zhang et al. 10.5194/acp-21-7099-2021
- Source apportionment of ambient PM2.5 in Ho Chi Minh City, Vietnam N. Tran et al. 10.1007/s44273-023-00024-7
- Applications of environmental mass spectrometry in atmospheric haze chemistry T. Chen et al. 10.1016/j.trac.2024.117614
- Secondary Organic Aerosol Formation Potential from Vehicular Non-tailpipe Emissions under Real-World Driving Conditions J. Zhang et al. 10.1021/acs.est.3c06475
- Chemical characterization of submicron aerosol in summertime Beijing: A case study in southern suburbs in 2018 T. Chen et al. 10.1016/j.chemosphere.2020.125918
- Effect of relative humidity on SOA formation from aromatic hydrocarbons: Implications from the evolution of gas- and particle-phase species T. Chen et al. 10.1016/j.scitotenv.2021.145015
- NH3 Weakens the Enhancing Effect of SO2 on Biogenic Secondary Organic Aerosol Formation L. Du et al. 10.1021/acs.estlett.2c00959
- Monitoring gaseous pollutants using passive sampling in the Philadelphia region B. Terry & K. Shakya 10.1080/10962247.2023.2279733
- Particulate emissions from L-Category vehicles towards Euro 5 A. Kontses et al. 10.1016/j.envres.2019.109071
- Quantifying traffic, biomass burning and secondary source contributions to atmospheric particle number concentrations at urban and suburban sites J. Casquero-Vera et al. 10.1016/j.scitotenv.2021.145282
- Indoor Particulate Matter in Urban Households: Sources, Pathways, Characteristics, Health Effects, and Exposure Mitigation L. Zhang et al. 10.3390/ijerph182111055
- Effects of NO and SO2 on the secondary organic aerosol formation from the photooxidation of 1,3,5-trimethylbenzene: A new source of organosulfates Z. Yang et al. 10.1016/j.envpol.2020.114742
- Secondary organic aerosol formation from mixed volatile organic compounds: Effect of RO2 chemistry and precursor concentration T. Chen et al. 10.1038/s41612-022-00321-y
Latest update: 17 Apr 2024
Short summary
Effects of SO2 and NH3 on SA formation from unburned gasoline vapor were investigated in a 30 m3 smog chamber. With the increase in SO2 and NH3 concentrations, formation of SA and each of its chemical species was promoted. Meanwhile, NPF and particle size growth were also significantly enhanced. This work indicates that gasoline evaporation emissions will be a significant source of SA and sulfur- and nitrogen-containing organics, especially in the presence of high concentrations of SO2 and NH3.
Effects of SO2 and NH3 on SA formation from unburned gasoline vapor were investigated in a 30 m3...
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