Articles | Volume 19, issue 9
https://doi.org/10.5194/acp-19-5973-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-5973-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Impact of anthropogenic and biogenic sources on the seasonal variation in the molecular composition of urban organic aerosols: a field and laboratory study using ultra-high-resolution mass spectrometry
Kaspar R. Daellenbach
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
now at: Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Ivan Kourtchev
Department of Chemistry, University of Cambridge, Cambridge, UK
Alexander L. Vogel
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
now at: Institute for Atmospheric and Environmental Sciences,
Goethe University, Frankfurt am Main, Germany
Emily A. Bruns
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
Jianhui Jiang
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
Tuukka Petäjä
Institute for Atmospheric and Earth System Research/Physics, Faculty
of Science, University of Helsinki, Helsinki, Finland
Jean-Luc Jaffrezo
Université Grenoble Alpes, CNRS, IRD, Grenoble INP, IGE, Grenoble,
France
Sebnem Aksoyoglu
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
Markus Kalberer
CORRESPONDING AUTHOR
Department of Chemistry, University of Cambridge, Cambridge, UK
Department of Environmental Sciences, University of Basel, Basel,
Switzerland
Urs Baltensperger
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
Imad El Haddad
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
André S. H. Prévôt
CORRESPONDING AUTHOR
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI),
5232 Villigen-PSI, Switzerland
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Latest update: 04 Nov 2024
Short summary
Here we present the molecular composition of the organic aerosol (OA) at an urban site in Central Europe (Zurich, Switzerland) and compare it to smog chamber wood smoke and ambient biogenic secondary OA (SOA) (Orbitrap analyses). Accordingly, we are able to explain the strong seasonality of the molecular composition by aged wood smoke and biogenic SOA during winter and summer. Our results could also explain the predominance of non-fossil organic carbon at European locations throughout the year.
Here we present the molecular composition of the organic aerosol (OA) at an urban site in...
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