Articles | Volume 19, issue 6
https://doi.org/10.5194/acp-19-4061-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-4061-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Apr 2019
Research article |
| 02 Apr 2019
| 02 Apr 2019
Insights into the O : C-dependent mechanisms controlling the evaporation of α-pinene secondary organic aerosol particles
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Andrew T. Lambe
Aerodyne Research Inc., Billerica, MA, USA
Arttu Ylisirniö
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Olli-Pekka Tikkanen
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Celia Faiola
Department of Ecology and Evolutionary Biology, University of California, Irvine, CA, USA
Eetu Kari
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Liqing Hao
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Olli Luoma
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Wei Huang
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Claudia Mohr
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Department of Environmental Science and Analytical Chemistry, Stockholm University, Stockholm, Sweden
Douglas R. Worsnop
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Aerodyne Research Inc., Billerica, MA, USA
Sergey A. Nizkorodov
Department of Chemistry, University of California, Irvine, CA, USA
Taina Yli-Juuti
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Siegfried Schobesberger
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Annele Virtanen
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
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Cited
20 citations as recorded by crossref.
- Evaluating Organic Aerosol Sources and Evolution with a Combined Molecular Composition and Volatility Framework Using the Filter Inlet for Gases and Aerosols (FIGAERO) J. Thornton et al. 10.1021/acs.accounts.0c00259
- Isothermal evaporation of α-pinene secondary organic aerosol particles formed under low NOx and high NOx conditions Z. Li et al. 10.5194/acp-23-203-2023
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. 10.1021/acsearthspacechem.0c00296
- Seasonal characteristics of organic aerosol chemical composition and volatility in Stuttgart, Germany W. Huang et al. 10.5194/acp-19-11687-2019
- Variation in chemical composition and volatility of oxygenated organic aerosol in different rural, urban, and mountain environments W. Huang et al. 10.5194/acp-24-2607-2024
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. 10.5194/acp-19-12515-2019
- Effect of Decreased Temperature on the Evaporation of α-Pinene Secondary Organic Aerosol Particles Z. Li et al. 10.1021/acsearthspacechem.9b00240
- Comparison of saturation vapor pressures of <i>α</i>-pinene + O<sub>3</sub> oxidation products derived from COSMO-RS computations and thermal desorption experiments N. Hyttinen et al. 10.5194/acp-22-1195-2022
- Direct mitigation of secondary organic aerosol particulate pollutants by multiphase photocatalysis L. Hao et al. 10.1016/j.scitotenv.2024.171323
- Bulk Organic Aerosol Analysis by Proton-Transfer-Reaction Mass Spectrometry: An Improved Methodology for the Determination of Total Organic Mass, O:C and H:C Elemental Ratios, and the Average Molecular Formula J. Leglise et al. 10.1021/acs.analchem.9b02949
- Diffusion Coefficients and Mixing Times of Organic Molecules in β-Caryophyllene Secondary Organic Aerosol (SOA) and Biomass Burning Organic Aerosol (BBOA) E. Evoy et al. 10.1021/acsearthspacechem.1c00317
- Partitioning of secondary organic aerosol onto nanoplastics leading to hygroscopic partially-engulfed particles K. Raincrow et al. 10.1039/D3EA00103B
- Comparing secondary organic aerosol (SOA) volatility distributions derived from isothermal SOA particle evaporation data and FIGAERO–CIMS measurements O. Tikkanen et al. 10.5194/acp-20-10441-2020
- Saturation vapor pressure characterization of selected low-volatility organic compounds using a residence time chamber Z. Li et al. 10.5194/acp-23-6863-2023
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. 10.1039/D0EA00020E
- Evolution of volatility and composition in sesquiterpene-mixed and <i>α</i>-pinene secondary organic aerosol particles during isothermal evaporation Z. Li et al. 10.5194/acp-21-18283-2021
- Composition and volatility of secondary organic aerosol (SOA) formed from oxidation of real tree emissions compared to simplified volatile organic compound (VOC) systems A. Ylisirniö et al. 10.5194/acp-20-5629-2020
- Exploring the composition and volatility of secondary organic aerosols in mixed anthropogenic and biogenic precursor systems A. Voliotis et al. 10.5194/acp-21-14251-2021
- Deconvolution of FIGAERO–CIMS thermal desorption profiles using positive matrix factorisation to identify chemical and physical processes during particle evaporation A. Buchholz et al. 10.5194/acp-20-7693-2020
20 citations as recorded by crossref.
- Evaluating Organic Aerosol Sources and Evolution with a Combined Molecular Composition and Volatility Framework Using the Filter Inlet for Gases and Aerosols (FIGAERO) J. Thornton et al. 10.1021/acs.accounts.0c00259
- Isothermal evaporation of α-pinene secondary organic aerosol particles formed under low NOx and high NOx conditions Z. Li et al. 10.5194/acp-23-203-2023
- Humidity-Dependent Viscosity of Secondary Organic Aerosol from Ozonolysis of β-Caryophyllene: Measurements, Predictions, and Implications A. Maclean et al. 10.1021/acsearthspacechem.0c00296
- Seasonal characteristics of organic aerosol chemical composition and volatility in Stuttgart, Germany W. Huang et al. 10.5194/acp-19-11687-2019
- Variation in chemical composition and volatility of oxygenated organic aerosol in different rural, urban, and mountain environments W. Huang et al. 10.5194/acp-24-2607-2024
- Radical chemistry in oxidation flow reactors for atmospheric chemistry research Z. Peng & J. Jimenez 10.1039/C9CS00766K
- Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors M. Song et al. 10.5194/acp-19-12515-2019
- Effect of Decreased Temperature on the Evaporation of α-Pinene Secondary Organic Aerosol Particles Z. Li et al. 10.1021/acsearthspacechem.9b00240
- Comparison of saturation vapor pressures of <i>α</i>-pinene + O<sub>3</sub> oxidation products derived from COSMO-RS computations and thermal desorption experiments N. Hyttinen et al. 10.5194/acp-22-1195-2022
- Direct mitigation of secondary organic aerosol particulate pollutants by multiphase photocatalysis L. Hao et al. 10.1016/j.scitotenv.2024.171323
- Bulk Organic Aerosol Analysis by Proton-Transfer-Reaction Mass Spectrometry: An Improved Methodology for the Determination of Total Organic Mass, O:C and H:C Elemental Ratios, and the Average Molecular Formula J. Leglise et al. 10.1021/acs.analchem.9b02949
- Diffusion Coefficients and Mixing Times of Organic Molecules in β-Caryophyllene Secondary Organic Aerosol (SOA) and Biomass Burning Organic Aerosol (BBOA) E. Evoy et al. 10.1021/acsearthspacechem.1c00317
- Partitioning of secondary organic aerosol onto nanoplastics leading to hygroscopic partially-engulfed particles K. Raincrow et al. 10.1039/D3EA00103B
- Comparing secondary organic aerosol (SOA) volatility distributions derived from isothermal SOA particle evaporation data and FIGAERO–CIMS measurements O. Tikkanen et al. 10.5194/acp-20-10441-2020
- Saturation vapor pressure characterization of selected low-volatility organic compounds using a residence time chamber Z. Li et al. 10.5194/acp-23-6863-2023
- Viscosity and liquid–liquid phase separation in healthy and stressed plant SOA N. Smith et al. 10.1039/D0EA00020E
- Evolution of volatility and composition in sesquiterpene-mixed and <i>α</i>-pinene secondary organic aerosol particles during isothermal evaporation Z. Li et al. 10.5194/acp-21-18283-2021
- Composition and volatility of secondary organic aerosol (SOA) formed from oxidation of real tree emissions compared to simplified volatile organic compound (VOC) systems A. Ylisirniö et al. 10.5194/acp-20-5629-2020
- Exploring the composition and volatility of secondary organic aerosols in mixed anthropogenic and biogenic precursor systems A. Voliotis et al. 10.5194/acp-21-14251-2021
- Deconvolution of FIGAERO–CIMS thermal desorption profiles using positive matrix factorisation to identify chemical and physical processes during particle evaporation A. Buchholz et al. 10.5194/acp-20-7693-2020
Latest update: 14 Dec 2024
Short summary
We studied the evaporation of α-pinene secondary organic aerosol particles in clean air to derive their volatility from the observed size changes. We found that the particles became more resilient to evaporation with increased oxidative age, possibly increasing their lifetime in the atmosphere. Also, increased relative humidity increased the particle evaporation. Mass spectrometry measurements of the particles at different stages of evaporation revealed some water-induced composition changes.
We studied the evaporation of α-pinene secondary organic aerosol particles in clean air to...
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