Articles | Volume 19, issue 5
https://doi.org/10.5194/acp-19-2861-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-2861-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
05 Mar 2019
Research article |
| 05 Mar 2019
| 05 Mar 2019
Unraveling the role of silicon in atmospheric aerosol secondary formation: a new conservative tracer for aerosol chemistry
Dawei Lu
State Key Laboratory of Environmental Chemistry and Ecotoxicology,
Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences,
Beijing 100085, China
Jihua Tan
College of Resources and Environment, University of Chinese Academy of
Sciences, Beijing 100049, China
Xuezhi Yang
State Key Laboratory of Environmental Chemistry and Ecotoxicology,
Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences,
Beijing 100085, China
College of Resources and Environment, University of Chinese Academy of
Sciences, Beijing 100049, China
Xu Sun
State Key Laboratory of Environmental Chemistry and Ecotoxicology,
Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences,
Beijing 100085, China
State Key Laboratory of Environmental Chemistry and Ecotoxicology,
Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences,
Beijing 100085, China
College of Resources and Environment, University of Chinese Academy of
Sciences, Beijing 100049, China
Institute of Environment and Health, Jianghan University, Wuhan
430056, China
Guibin Jiang
State Key Laboratory of Environmental Chemistry and Ecotoxicology,
Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences,
Beijing 100085, China
College of Resources and Environment, University of Chinese Academy of
Sciences, Beijing 100049, China
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- Performance evaluation of an online monitor based on X-ray fluorescence for detecting elemental concentrations in ambient particulate matter I. Trebs et al. 10.5194/amt-17-6791-2024
- Internal Exposure and Distribution of Airborne Fine Particles in the Human Body: Methodology, Current Understandings, and Research Needs W. Wang et al. 10.1021/acs.est.1c07051
- Phytolith particulate matter and its potential human and environmental effects W. Qader et al. 10.1016/j.envpol.2023.121541
- Elucidation of the Critical Role of Core Materials in PM2.5-Induced Cytotoxicity by Interrogating Silica- and Carbon-Based Model PM2.5 Particle Libraries G. Liu et al. 10.1021/acs.est.1c00001
- Two-Dimensional Silicon Fingerprints Reveal Dramatic Variations in the Sources of Particulate Matter in Beijing during 2013–2017 X. Yang et al. 10.1021/acs.est.0c00984
- Formation of Low-Volatile Products and Unexpected High Formaldehyde Yield from the Atmospheric Oxidation of Methylsiloxanes Z. Fu et al. 10.1021/acs.est.0c01090
- Unraveling the process of aerosols secondary formation and removal based on cosmogenic beryllium-7 and beryllium-10 X. Liu et al. 10.1016/j.scitotenv.2022.153293
- Revealing the Chemical Profiles of Airborne Particulate Matter Sources in Lake Baikal Area: A Combination of Three Techniques M. Semenov et al. 10.3390/su14106170
- PM2.5-bound silicon-containing secondary organic aerosols (Si-SOA) in Beijing ambient air J. Xu et al. 10.1016/j.chemosphere.2021.132377
- Volatile oxidation products and secondary organosiloxane aerosol from D5 + OH at varying OH exposures H. Kang et al. 10.5194/acp-23-14307-2023
- ToF‐SIMS analysis of chemical composition of atmospheric aerosols in Beijing F. Jia et al. 10.1002/sia.6710
- Separation and Tracing of Anthropogenic Magnetite Nanoparticles in the Urban Atmosphere Q. Zhang et al. 10.1021/acs.est.0c01841
- Recent advances in method development and application of multi-collector inductively coupled plasma mass spectrometry L. ZHANG et al. 10.3724/SP.J.1123.2020.07030
- Non-traditional stable isotopic analysis for source tracing of atmospheric particulate matter P. Zuo et al. 10.1016/j.trac.2022.116866
- Atmospheric Degradation of Cyclic Volatile Methyl Siloxanes: Radical Chemistry and Oxidation Products M. Alton & E. Browne 10.1021/acsenvironau.1c00043
16 citations as recorded by crossref.
- The interaction laws of atmospheric heavy metal ions and water-soluble organic compounds in PM2.5 based on the excitation-emission matrix fluorescence spectroscopy X. Wang et al. 10.1016/j.jhazmat.2020.123497
- Stable Iron Isotopic Signature Reveals Multiple Sources of Magnetic Particulate Matter in the 2021 Beijing Sandstorms P. Zuo et al. 10.1021/acs.estlett.2c00144
- Performance evaluation of an online monitor based on X-ray fluorescence for detecting elemental concentrations in ambient particulate matter I. Trebs et al. 10.5194/amt-17-6791-2024
- Internal Exposure and Distribution of Airborne Fine Particles in the Human Body: Methodology, Current Understandings, and Research Needs W. Wang et al. 10.1021/acs.est.1c07051
- Phytolith particulate matter and its potential human and environmental effects W. Qader et al. 10.1016/j.envpol.2023.121541
- Elucidation of the Critical Role of Core Materials in PM2.5-Induced Cytotoxicity by Interrogating Silica- and Carbon-Based Model PM2.5 Particle Libraries G. Liu et al. 10.1021/acs.est.1c00001
- Two-Dimensional Silicon Fingerprints Reveal Dramatic Variations in the Sources of Particulate Matter in Beijing during 2013–2017 X. Yang et al. 10.1021/acs.est.0c00984
- Formation of Low-Volatile Products and Unexpected High Formaldehyde Yield from the Atmospheric Oxidation of Methylsiloxanes Z. Fu et al. 10.1021/acs.est.0c01090
- Unraveling the process of aerosols secondary formation and removal based on cosmogenic beryllium-7 and beryllium-10 X. Liu et al. 10.1016/j.scitotenv.2022.153293
- Revealing the Chemical Profiles of Airborne Particulate Matter Sources in Lake Baikal Area: A Combination of Three Techniques M. Semenov et al. 10.3390/su14106170
- PM2.5-bound silicon-containing secondary organic aerosols (Si-SOA) in Beijing ambient air J. Xu et al. 10.1016/j.chemosphere.2021.132377
- Volatile oxidation products and secondary organosiloxane aerosol from D5 + OH at varying OH exposures H. Kang et al. 10.5194/acp-23-14307-2023
- ToF‐SIMS analysis of chemical composition of atmospheric aerosols in Beijing F. Jia et al. 10.1002/sia.6710
- Separation and Tracing of Anthropogenic Magnetite Nanoparticles in the Urban Atmosphere Q. Zhang et al. 10.1021/acs.est.0c01841
- Recent advances in method development and application of multi-collector inductively coupled plasma mass spectrometry L. ZHANG et al. 10.3724/SP.J.1123.2020.07030
- Non-traditional stable isotopic analysis for source tracing of atmospheric particulate matter P. Zuo et al. 10.1016/j.trac.2022.116866
Latest update: 14 Dec 2024
Short summary
We investigated for the first time the role of Si during secondary formation process of PM2.5. We show the noncorrelation of Si with the secondary aerosol (SA) formation in Beijing, which reveals a new conservative tracer for aerosol chemistry. The SA contribution can be estimated by using Si as a single tracer instead of commonly used multiple chemical tracers. The correlation analysis of SA with the Si isotopic composition of PM2.5 can also reveal the sources of the precursors of SA.
We investigated for the first time the role of Si during secondary formation process of PM2.5....
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