Articles | Volume 19, issue 3
https://doi.org/10.5194/acp-19-1971-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-1971-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Feb 2019
Research article |
| 13 Feb 2019
| 13 Feb 2019
A proxy for atmospheric daytime gaseous sulfuric acid concentration in urban Beijing
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Yueyun Fu
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Institute of Chemistry, Chinese Academy of Sciences, Beijing
100190, China
Yiliang Liu
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Gan Yang
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Yuwei Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Federico Bianchi
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Ying Zhou
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Rujing Yin
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Rima Baalbaki
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Olga Garmash
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Chenjuan Deng
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Weigang Wang
Institute of Chemistry, Chinese Academy of Sciences, Beijing
100190, China
Yongchun Liu
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Tuukka Petäjä
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Joint International Research Laboratory of Atmospheric and Earth
System Sciences (JirLATEST), School of Atmospheric Sciences, Nanjing
University, Nanjing 210023, China
Veli-Matti Kerminen
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Jingkun Jiang
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Markku Kulmala
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Institute of Atmospheric Sciences, Jiangwan Campus, Fudan
University, Shanghai 200438, China
Shanghai Institute of Pollution Control and Ecological Security,
Shanghai 200092, China
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Short summary
Gaseous sulfuric acid is one of the key precursors for atmospheric new particle formation processes, but its measurement remains challenging. This work develops an estimation method for the gaseous sulfuric acid concentration in an urban environment in China using multiple atmospheric variables that are easier to measure. The consideration of the heterogeneous formation of HONO and the subsequent photo-production of OH radicals improves the performance of the estimation method.
Gaseous sulfuric acid is one of the key precursors for atmospheric new particle formation...
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