Articles | Volume 19, issue 3
https://doi.org/10.5194/acp-19-1971-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-1971-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
A proxy for atmospheric daytime gaseous sulfuric acid concentration in urban Beijing
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Yueyun Fu
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Institute of Chemistry, Chinese Academy of Sciences, Beijing
100190, China
Yiliang Liu
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Gan Yang
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Yuwei Wang
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Federico Bianchi
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Ying Zhou
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Rujing Yin
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Rima Baalbaki
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Olga Garmash
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Chenjuan Deng
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Weigang Wang
Institute of Chemistry, Chinese Academy of Sciences, Beijing
100190, China
Yongchun Liu
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Tuukka Petäjä
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Joint International Research Laboratory of Atmospheric and Earth
System Sciences (JirLATEST), School of Atmospheric Sciences, Nanjing
University, Nanjing 210023, China
Veli-Matti Kerminen
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Jingkun Jiang
State Key Joint Laboratory of Environment Simulation and Pollution
Control, School of Environment, Tsinghua University, Beijing 100084, China
Markku Kulmala
Institute for Atmospheric and Earth System Research/Physics,
Faculty of Science, University of Helsinki, 00014 Helsinki, Finland
Aerosol and Haze Laboratory, Advanced Innovation Center for Soft
Matter Science and Engineering, Beijing University of Chemical Technology,
Beijing 100029, China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP), Department of Environmental Science &
Engineering,
Jiangwan Campus, Fudan University, Shanghai 200438, China
Institute of Atmospheric Sciences, Jiangwan Campus, Fudan
University, Shanghai 200438, China
Shanghai Institute of Pollution Control and Ecological Security,
Shanghai 200092, China
Viewed
Total article views: 3,647 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 29 Nov 2018)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
2,485 | 1,090 | 72 | 3,647 | 581 | 65 | 111 |
- HTML: 2,485
- PDF: 1,090
- XML: 72
- Total: 3,647
- Supplement: 581
- BibTeX: 65
- EndNote: 111
Total article views: 2,955 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 13 Feb 2019)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
2,055 | 841 | 59 | 2,955 | 434 | 60 | 102 |
- HTML: 2,055
- PDF: 841
- XML: 59
- Total: 2,955
- Supplement: 434
- BibTeX: 60
- EndNote: 102
Total article views: 692 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 29 Nov 2018)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
430 | 249 | 13 | 692 | 147 | 5 | 9 |
- HTML: 430
- PDF: 249
- XML: 13
- Total: 692
- Supplement: 147
- BibTeX: 5
- EndNote: 9
Viewed (geographical distribution)
Total article views: 3,647 (including HTML, PDF, and XML)
Thereof 3,492 with geography defined
and 155 with unknown origin.
Total article views: 2,955 (including HTML, PDF, and XML)
Thereof 2,851 with geography defined
and 104 with unknown origin.
Total article views: 692 (including HTML, PDF, and XML)
Thereof 641 with geography defined
and 51 with unknown origin.
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Cited
45 citations as recorded by crossref.
- Observation of sub-3nm particles and new particle formation at an urban location in India M. Sebastian et al. 10.1016/j.atmosenv.2021.118460
- Measurement report: Size distributions of urban aerosols down to 1 nm from long-term measurements C. Deng et al. 10.5194/acp-22-13569-2022
- Characterization of dust-related new particle formation events based on long-term measurement in the North China Plain X. Shen et al. 10.5194/acp-23-8241-2023
- Survival probabilities of atmospheric particles: comparison based on theory, cluster population simulations, and observations in Beijing S. Tuovinen et al. 10.5194/acp-22-15071-2022
- The biogeochemistry of marine dimethylsulfide F. Hopkins et al. 10.1038/s43017-023-00428-7
- The impact of the atmospheric turbulence-development tendency on new particle formation: a common finding on three continents H. Wu et al. 10.1093/nsr/nwaa157
- Substantially positive contributions of new particle formation to cloud condensation nuclei under low supersaturation in China based on numerical model improvements C. Zhang et al. 10.5194/acp-23-10713-2023
- Investigation of several proxies to estimate sulfuric acid concentration under volcanic plume conditions C. Rose et al. 10.5194/acp-21-4541-2021
- The important roles of surface tension and growth rate in the contribution of new particle formation (NPF) to cloud condensation nuclei (CCN) number concentration: evidence from field measurements in southern China M. Cai et al. 10.5194/acp-21-8575-2021
- Variations in Source Contributions of Particle Number Concentration Under Long-Term Emission Control in Winter of Urban Beijing D. Shang et al. 10.2139/ssrn.3975615
- Key characteristics of new particle formation events occurring simultaneously in the Yangtze River Delta and northeast rural sites in China S. Liu et al. 10.1016/j.atmosenv.2024.120406
- Formation of condensable organic vapors from anthropogenic and biogenic volatile organic compounds (VOCs) is strongly perturbed by NO<sub><i>x</i></sub> in eastern China Y. Liu et al. 10.5194/acp-21-14789-2021
- Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 2: Modeling chemical drivers and 3-D new particle formation occurrence M. Chu et al. 10.5194/acp-24-6769-2024
- Unexpected quenching effect on new particle formation from the atmospheric reaction of methanol with SO 3 L. Liu et al. 10.1073/pnas.1915459116
- Variation of size-segregated particle number concentrations in wintertime Beijing Y. Zhou et al. 10.5194/acp-20-1201-2020
- Chemistry of new particle formation and growth events during wintertime in suburban area of Beijing: Insights from highly polluted atmosphere S. Yang et al. 10.1016/j.atmosres.2021.105553
- Sources and sinks driving sulfuric acid concentrations in contrasting environments: implications on proxy calculations L. Dada et al. 10.5194/acp-20-11747-2020
- Contribution of New Particle Formation to Cloud Condensation Nuclei Activity and its Controlling Factors in a Mountain Region of Inland China M. Cai et al. 10.1029/2020JD034302
- Investigating three patterns of new particles growing to the size of cloud condensation nuclei in Beijing's urban atmosphere L. Ma et al. 10.5194/acp-21-183-2021
- Reduction of anthropogenic emissions enhanced atmospheric new particle formation: Observational evidence during the Beijing 2022 Winter Olympics W. Zhu et al. 10.1016/j.atmosenv.2023.120094
- High contribution of new particle formation to ultrafine particles in four seasons in an urban atmosphere in south China L. Tao et al. 10.1016/j.scitotenv.2023.164202
- Formation of nighttime sulfuric acid from the ozonolysis of alkenes in Beijing Y. Guo et al. 10.5194/acp-21-5499-2021
- Measurement report: New particle formation characteristics at an urban and a mountain station in northern China Y. Zhou et al. 10.5194/acp-21-17885-2021
- Sulfuric acid in the Amazon basin: measurements and evaluation of existing sulfuric acid proxies D. Myers et al. 10.5194/acp-22-10061-2022
- Measurement Report: Wintertime new particle formation in the rural area of the North China Plain – influencing factors and possible formation mechanism J. Hong et al. 10.5194/acp-23-5699-2023
- Particle growth with photochemical age from new particle formation to haze in the winter of Beijing, China B. Chu et al. 10.1016/j.scitotenv.2020.142207
- Formation and growth of sub-3 nm particles in megacities: impact of background aerosols C. Deng et al. 10.1039/D0FD00083C
- Machine Learning Reveals the Parameters Affecting the Gaseous Sulfuric Acid Distribution in a Coastal City: Model Construction and Interpretation C. Yang et al. 10.1021/acs.estlett.3c00170
- Seasonal Characteristics of New Particle Formation and Growth in Urban Beijing C. Deng et al. 10.1021/acs.est.0c00808
- Titanium Dioxide Promotes New Particle Formation: A Smog Chamber Study H. Zhang et al. 10.1021/acs.est.2c06946
- Spatial Inhomogeneity of New Particle Formation in the Urban and Mountainous Atmospheres of the North China Plain during the 2022 Winter Olympics D. Shang et al. 10.3390/atmos14091395
- Towards understanding the characteristics of new particle formation in the Eastern Mediterranean R. Baalbaki et al. 10.5194/acp-21-9223-2021
- Enhancement of nanoparticle formation and growth during the COVID-19 lockdown period in urban Beijing X. Shen et al. 10.5194/acp-21-7039-2021
- The effectiveness of the coagulation sink of 3–10 nm atmospheric particles R. Cai et al. 10.5194/acp-22-11529-2022
- Acid–Base Clusters during Atmospheric New Particle Formation in Urban Beijing R. Yin et al. 10.1021/acs.est.1c02701
- Estimation of sulfuric acid concentration using ambient ion composition and concentration data obtained with atmospheric pressure interface time-of-flight ion mass spectrometer L. Beck et al. 10.5194/amt-15-1957-2022
- New Particle Formation Occurrence in the Urban Atmosphere of Beijing During 2013–2020 D. Shang et al. 10.1029/2022JD038334
- Overview: Recent advances in the understanding of the northern Eurasian environments and of the urban air quality in China – a Pan-Eurasian Experiment (PEEX) programme perspective H. Lappalainen et al. 10.5194/acp-22-4413-2022
- Aerosol number concentrations and new particle formation events over a polluted megacity during the COVID-19 lockdown S. Yadav et al. 10.1016/j.atmosenv.2021.118526
- Variations in source contributions of particle number concentration under long-term emission control in winter of urban Beijing D. Shang et al. 10.1016/j.envpol.2022.119072
- Particle number size distributions and formation and growth rates of different new particle formation types of a megacity in China L. Dai et al. 10.1016/j.jes.2022.07.029
- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
- Iodine oxoacids and their roles in sub-3 nm particle growth in polluted urban environments Y. Zhang et al. 10.5194/acp-24-1873-2024
- Responses of gaseous sulfuric acid and particulate sulfate to reduced SO2 concentration: A perspective from long-term measurements in Beijing X. Li et al. 10.1016/j.scitotenv.2020.137700
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
45 citations as recorded by crossref.
- Observation of sub-3nm particles and new particle formation at an urban location in India M. Sebastian et al. 10.1016/j.atmosenv.2021.118460
- Measurement report: Size distributions of urban aerosols down to 1 nm from long-term measurements C. Deng et al. 10.5194/acp-22-13569-2022
- Characterization of dust-related new particle formation events based on long-term measurement in the North China Plain X. Shen et al. 10.5194/acp-23-8241-2023
- Survival probabilities of atmospheric particles: comparison based on theory, cluster population simulations, and observations in Beijing S. Tuovinen et al. 10.5194/acp-22-15071-2022
- The biogeochemistry of marine dimethylsulfide F. Hopkins et al. 10.1038/s43017-023-00428-7
- The impact of the atmospheric turbulence-development tendency on new particle formation: a common finding on three continents H. Wu et al. 10.1093/nsr/nwaa157
- Substantially positive contributions of new particle formation to cloud condensation nuclei under low supersaturation in China based on numerical model improvements C. Zhang et al. 10.5194/acp-23-10713-2023
- Investigation of several proxies to estimate sulfuric acid concentration under volcanic plume conditions C. Rose et al. 10.5194/acp-21-4541-2021
- The important roles of surface tension and growth rate in the contribution of new particle formation (NPF) to cloud condensation nuclei (CCN) number concentration: evidence from field measurements in southern China M. Cai et al. 10.5194/acp-21-8575-2021
- Variations in Source Contributions of Particle Number Concentration Under Long-Term Emission Control in Winter of Urban Beijing D. Shang et al. 10.2139/ssrn.3975615
- Key characteristics of new particle formation events occurring simultaneously in the Yangtze River Delta and northeast rural sites in China S. Liu et al. 10.1016/j.atmosenv.2024.120406
- Formation of condensable organic vapors from anthropogenic and biogenic volatile organic compounds (VOCs) is strongly perturbed by NO<sub><i>x</i></sub> in eastern China Y. Liu et al. 10.5194/acp-21-14789-2021
- Investigating the contribution of grown new particles to cloud condensation nuclei with largely varying preexisting particles – Part 2: Modeling chemical drivers and 3-D new particle formation occurrence M. Chu et al. 10.5194/acp-24-6769-2024
- Unexpected quenching effect on new particle formation from the atmospheric reaction of methanol with SO 3 L. Liu et al. 10.1073/pnas.1915459116
- Variation of size-segregated particle number concentrations in wintertime Beijing Y. Zhou et al. 10.5194/acp-20-1201-2020
- Chemistry of new particle formation and growth events during wintertime in suburban area of Beijing: Insights from highly polluted atmosphere S. Yang et al. 10.1016/j.atmosres.2021.105553
- Sources and sinks driving sulfuric acid concentrations in contrasting environments: implications on proxy calculations L. Dada et al. 10.5194/acp-20-11747-2020
- Contribution of New Particle Formation to Cloud Condensation Nuclei Activity and its Controlling Factors in a Mountain Region of Inland China M. Cai et al. 10.1029/2020JD034302
- Investigating three patterns of new particles growing to the size of cloud condensation nuclei in Beijing's urban atmosphere L. Ma et al. 10.5194/acp-21-183-2021
- Reduction of anthropogenic emissions enhanced atmospheric new particle formation: Observational evidence during the Beijing 2022 Winter Olympics W. Zhu et al. 10.1016/j.atmosenv.2023.120094
- High contribution of new particle formation to ultrafine particles in four seasons in an urban atmosphere in south China L. Tao et al. 10.1016/j.scitotenv.2023.164202
- Formation of nighttime sulfuric acid from the ozonolysis of alkenes in Beijing Y. Guo et al. 10.5194/acp-21-5499-2021
- Measurement report: New particle formation characteristics at an urban and a mountain station in northern China Y. Zhou et al. 10.5194/acp-21-17885-2021
- Sulfuric acid in the Amazon basin: measurements and evaluation of existing sulfuric acid proxies D. Myers et al. 10.5194/acp-22-10061-2022
- Measurement Report: Wintertime new particle formation in the rural area of the North China Plain – influencing factors and possible formation mechanism J. Hong et al. 10.5194/acp-23-5699-2023
- Particle growth with photochemical age from new particle formation to haze in the winter of Beijing, China B. Chu et al. 10.1016/j.scitotenv.2020.142207
- Formation and growth of sub-3 nm particles in megacities: impact of background aerosols C. Deng et al. 10.1039/D0FD00083C
- Machine Learning Reveals the Parameters Affecting the Gaseous Sulfuric Acid Distribution in a Coastal City: Model Construction and Interpretation C. Yang et al. 10.1021/acs.estlett.3c00170
- Seasonal Characteristics of New Particle Formation and Growth in Urban Beijing C. Deng et al. 10.1021/acs.est.0c00808
- Titanium Dioxide Promotes New Particle Formation: A Smog Chamber Study H. Zhang et al. 10.1021/acs.est.2c06946
- Spatial Inhomogeneity of New Particle Formation in the Urban and Mountainous Atmospheres of the North China Plain during the 2022 Winter Olympics D. Shang et al. 10.3390/atmos14091395
- Towards understanding the characteristics of new particle formation in the Eastern Mediterranean R. Baalbaki et al. 10.5194/acp-21-9223-2021
- Enhancement of nanoparticle formation and growth during the COVID-19 lockdown period in urban Beijing X. Shen et al. 10.5194/acp-21-7039-2021
- The effectiveness of the coagulation sink of 3–10 nm atmospheric particles R. Cai et al. 10.5194/acp-22-11529-2022
- Acid–Base Clusters during Atmospheric New Particle Formation in Urban Beijing R. Yin et al. 10.1021/acs.est.1c02701
- Estimation of sulfuric acid concentration using ambient ion composition and concentration data obtained with atmospheric pressure interface time-of-flight ion mass spectrometer L. Beck et al. 10.5194/amt-15-1957-2022
- New Particle Formation Occurrence in the Urban Atmosphere of Beijing During 2013–2020 D. Shang et al. 10.1029/2022JD038334
- Overview: Recent advances in the understanding of the northern Eurasian environments and of the urban air quality in China – a Pan-Eurasian Experiment (PEEX) programme perspective H. Lappalainen et al. 10.5194/acp-22-4413-2022
- Aerosol number concentrations and new particle formation events over a polluted megacity during the COVID-19 lockdown S. Yadav et al. 10.1016/j.atmosenv.2021.118526
- Variations in source contributions of particle number concentration under long-term emission control in winter of urban Beijing D. Shang et al. 10.1016/j.envpol.2022.119072
- Particle number size distributions and formation and growth rates of different new particle formation types of a megacity in China L. Dai et al. 10.1016/j.jes.2022.07.029
- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
- Iodine oxoacids and their roles in sub-3 nm particle growth in polluted urban environments Y. Zhang et al. 10.5194/acp-24-1873-2024
- Responses of gaseous sulfuric acid and particulate sulfate to reduced SO2 concentration: A perspective from long-term measurements in Beijing X. Li et al. 10.1016/j.scitotenv.2020.137700
- Atmospheric nanoparticle growth D. Stolzenburg et al. 10.1103/RevModPhys.95.045002
Latest update: 02 Oct 2024
Short summary
Gaseous sulfuric acid is one of the key precursors for atmospheric new particle formation processes, but its measurement remains challenging. This work develops an estimation method for the gaseous sulfuric acid concentration in an urban environment in China using multiple atmospheric variables that are easier to measure. The consideration of the heterogeneous formation of HONO and the subsequent photo-production of OH radicals improves the performance of the estimation method.
Gaseous sulfuric acid is one of the key precursors for atmospheric new particle formation...
Altmetrics
Final-revised paper
Preprint