Articles | Volume 19, issue 3
https://doi.org/10.5194/acp-19-1587-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-1587-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Influence of cloud microphysical processes on black carbon wet removal, global distributions, and radiative forcing
Jiayu Xu
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
Jiachen Zhang
Department of Civil and Environmental Engineering, University of Southern California, Los Angeles, CA, USA
Junfeng Liu
CORRESPONDING AUTHOR
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
Kan Yi
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
Songlin Xiang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
Xiurong Hu
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
Yuqing Wang
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
Shu Tao
Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences, Peking University, Beijing, China
George Ban-Weiss
Department of Civil and Environmental Engineering, University of Southern California, Los Angeles, CA, USA
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Cited
16 citations as recorded by crossref.
- Coalescence Scavenging Drives Droplet Number Concentration in Southern Ocean Low Clouds L. Kang et al. 10.1029/2022GL097819
- Assessment of the combined radiative effects of black carbon in the atmosphere and snowpack in the Northern Hemisphere constrained by surface observations T. Shi et al. 10.1039/D2EA00005A
- Impacts of Simulated Contrail Processing and Organic Content Change on the Ice Nucleation of Soot Particles K. Gao & Z. Kanji 10.1029/2022GL099869
- Impacts of springtime biomass burning in Southeast Asia on atmospheric carbonaceous components over the Beibu Gulf in China: Insights from aircraft observations X. Yang et al. 10.1016/j.scitotenv.2022.159232
- Stage-resolved in-cloud scavenging of submicron and BC-containing particles: A case study Y. Yang et al. 10.1016/j.atmosenv.2020.117883
- Improving Below‐Cloud Scavenging Coefficients of Sulfate, Nitrate, and Ammonium in PM2.5 and Implications for Numerical Simulation and Air Pollution Control L. Yao et al. 10.1029/2023JD039487
- Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol Y. Yang et al. 10.3390/atmos10040175
- Improved Simulations of Global Black Carbon Distributions by Modifying Wet Scavenging Processes in Convective and Mixed‐Phase Clouds M. Liu & H. Matsui 10.1029/2020JD033890
- Spatiotemporal distribution and inter-media transfer of polycyclic aromatic hydrocarbons in Shanghai, China: Historical patterns and future trends T. Li et al. 10.1016/j.scitotenv.2024.173938
- Long-range aerosol transport and impacts on size-resolved aerosol composition in Metro Manila, Philippines R. Braun et al. 10.5194/acp-20-2387-2020
- Refractory black carbon aerosols in rainwater in the summer of 2019 in Beijing: Mass concentration, size distribution and wet scavenging ratio S. Lei et al. 10.1016/j.jes.2022.07.039
- Investigation of the wet removal rate of black carbon in East Asia: validation of a below- and in-cloud wet removal scheme in FLEXible PARTicle (FLEXPART) model v10.4 Y. Choi et al. 10.5194/acp-20-13655-2020
- A Review of Progress in Constraining Global Black Carbon Climate Effects J. Everett et al. 10.1007/s41748-022-00313-1
- Toward carbon neutrality: Projecting a desert-based photovoltaic power network circumnavigating the globe Y. Zhou et al. 10.1093/pnasnexus/pgad097
- Black Carbon Particles Physicochemical Real‐Time Data Set in a Cold City: Trends of Fall‐Winter BC Accumulation and COVID‐19 H. Li & P. Ariya 10.1029/2021JD035265
- Impacts of coal use phase-out in China on the atmospheric environment: (2) public health and global radiative forcing Y. Zhou et al. 10.1016/j.atmosenv.2023.120280
16 citations as recorded by crossref.
- Coalescence Scavenging Drives Droplet Number Concentration in Southern Ocean Low Clouds L. Kang et al. 10.1029/2022GL097819
- Assessment of the combined radiative effects of black carbon in the atmosphere and snowpack in the Northern Hemisphere constrained by surface observations T. Shi et al. 10.1039/D2EA00005A
- Impacts of Simulated Contrail Processing and Organic Content Change on the Ice Nucleation of Soot Particles K. Gao & Z. Kanji 10.1029/2022GL099869
- Impacts of springtime biomass burning in Southeast Asia on atmospheric carbonaceous components over the Beibu Gulf in China: Insights from aircraft observations X. Yang et al. 10.1016/j.scitotenv.2022.159232
- Stage-resolved in-cloud scavenging of submicron and BC-containing particles: A case study Y. Yang et al. 10.1016/j.atmosenv.2020.117883
- Improving Below‐Cloud Scavenging Coefficients of Sulfate, Nitrate, and Ammonium in PM2.5 and Implications for Numerical Simulation and Air Pollution Control L. Yao et al. 10.1029/2023JD039487
- Recent Advances in Quantifying Wet Scavenging Efficiency of Black Carbon Aerosol Y. Yang et al. 10.3390/atmos10040175
- Improved Simulations of Global Black Carbon Distributions by Modifying Wet Scavenging Processes in Convective and Mixed‐Phase Clouds M. Liu & H. Matsui 10.1029/2020JD033890
- Spatiotemporal distribution and inter-media transfer of polycyclic aromatic hydrocarbons in Shanghai, China: Historical patterns and future trends T. Li et al. 10.1016/j.scitotenv.2024.173938
- Long-range aerosol transport and impacts on size-resolved aerosol composition in Metro Manila, Philippines R. Braun et al. 10.5194/acp-20-2387-2020
- Refractory black carbon aerosols in rainwater in the summer of 2019 in Beijing: Mass concentration, size distribution and wet scavenging ratio S. Lei et al. 10.1016/j.jes.2022.07.039
- Investigation of the wet removal rate of black carbon in East Asia: validation of a below- and in-cloud wet removal scheme in FLEXible PARTicle (FLEXPART) model v10.4 Y. Choi et al. 10.5194/acp-20-13655-2020
- A Review of Progress in Constraining Global Black Carbon Climate Effects J. Everett et al. 10.1007/s41748-022-00313-1
- Toward carbon neutrality: Projecting a desert-based photovoltaic power network circumnavigating the globe Y. Zhou et al. 10.1093/pnasnexus/pgad097
- Black Carbon Particles Physicochemical Real‐Time Data Set in a Cold City: Trends of Fall‐Winter BC Accumulation and COVID‐19 H. Li & P. Ariya 10.1029/2021JD035265
- Impacts of coal use phase-out in China on the atmospheric environment: (2) public health and global radiative forcing Y. Zhou et al. 10.1016/j.atmosenv.2023.120280
Latest update: 23 Nov 2024
Short summary
In this study, we fully describe black carbon wet removal coupled with all cloud processes from a cloud microphysics scheme in a climate model and conduct sensitivity simulations that turn off each cloud process one at a time. We find that convective scavenging, aerosol activation, ice nucleation, evaporation of rain–snow, and below-cloud scavenging dominate wet deposition of BC. In addition, the range of direct radiative forcing derived from sensitivity simulations is large, 0.09–0.33 W m−2.
In this study, we fully describe black carbon wet removal coupled with all cloud processes from...
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