Articles | Volume 19, issue 24
https://doi.org/10.5194/acp-19-15651-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-15651-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
20 Dec 2019
Research article |
| 20 Dec 2019
| 20 Dec 2019
Potential dual effect of anthropogenic emissions on the formation of biogenic secondary organic aerosol (BSOA)
Eetu Kari
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
currently at: Neste Oyj, Porvoo, Finland
Liqing Hao
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Arttu Ylisirniö
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Angela Buchholz
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Ari Leskinen
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Finnish Meteorological Institute, Kuopio, Finland
Pasi Yli-Pirilä
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, Finland
Ilpo Nuutinen
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, Finland
currently at: Savonia University of Applied Sciences, Kuopio, Finland
Kari Kuuspalo
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, Finland
currently at: Savonia University of Applied Sciences, Kuopio, Finland
Jorma Jokiniemi
Department of Environmental and Biological Sciences, University of
Eastern Finland, Kuopio, Finland
Celia L. Faiola
Department of Ecology and Evolutionary Biology, University of
California, Irvine, Irvine, CA, USA
Department of Chemistry, University of California, Irvine, Irvine, CA, USA
Siegfried Schobesberger
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
Annele Virtanen
CORRESPONDING AUTHOR
Department of Applied Physics, University of Eastern Finland, Kuopio, Finland
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22 citations as recorded by crossref.
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- Pathogenic Mechanisms of Secondary Organic Aerosols T. Déméautis et al. https://doi.org/10.1021/acs.chemrestox.1c00353
- Mass spectrometry-based Aerosolomics: a new approach to resolve sources, composition, and partitioning of secondary organic aerosol M. Thoma et al. https://doi.org/10.5194/amt-15-7137-2022
- Effects of driving conditions on aerosol formation from photooxidation of gasoline vehicles exhaust in Hong Kong H. Poon et al. https://doi.org/10.1016/j.atmosenv.2023.120089
- Effects of relative humidity on atmospheric organosulfur species derived from photooxidation and nocturnal chemistry in a forest environment L. Li et al. https://doi.org/10.1016/j.envpol.2024.125253
- Comparison of dimension reduction techniques in the analysis of mass spectrometry data S. Isokääntä et al. https://doi.org/10.5194/amt-13-2995-2020
- Tower-based profiles of wintertime secondary organic aerosols in the urban boundary layer over Guangzhou Y. Li et al. https://doi.org/10.1016/j.scitotenv.2024.175326
- Direct contribution of ammonia to α-pinene secondary organic aerosol formation L. Hao et al. https://doi.org/10.5194/acp-20-14393-2020
- A Closure Study of Secondary Organic Aerosol Estimation at an Urban Site of Yangtze River Delta, China Z. Wan et al. https://doi.org/10.3390/atmos13101679
- Effects of driving conditions on secondary aerosol formation from a GDI vehicle using an oxidation flow reactor N. Kuittinen et al. https://doi.org/10.1016/j.envpol.2021.117069
- Interaction between marine and terrestrial biogenic volatile organic compounds: Non-linear effect on secondary organic aerosol formation X. Chen et al. https://doi.org/10.1016/j.atmosenv.2024.120868
- Measurement report: New particle formation events observed during the COALA-2020 campaign J. Ramirez-Gamboa et al. https://doi.org/10.5194/acp-25-9937-2025
- Tracer-based characterization of source variations of PM2.5 and organic carbon in Shanghai influenced by the COVID-19 lockdown S. Zhu et al. https://doi.org/10.1039/D0FD00091D
- Suppression of anthropogenic secondary organic aerosol formation by isoprene K. Li et al. https://doi.org/10.1038/s41612-022-00233-x
- Source apportionment and secondary organic aerosol formation potential of VOCs in urban and suburban areas of South Korea K. Kim et al. https://doi.org/10.1016/j.apr.2026.102964
- Secondary organic aerosol formed by Euro 5 gasoline vehicle emissions: chemical composition and gas-to-particle phase partitioning E. Kostenidou et al. https://doi.org/10.5194/acp-24-2705-2024
- Enhanced secondary organic aerosol formation from the photo-oxidation of mixed anthropogenic volatile organic compounds J. Li et al. https://doi.org/10.5194/acp-21-7773-2021
- Measurement report: Effects of anthropogenic emissions and environmental factors on the formation of biogenic secondary organic aerosol (BSOA) in a coastal city of southeastern China Y. Hong et al. https://doi.org/10.5194/acp-22-7827-2022
- Monoterpene Photooxidation in a Continuous-Flow Chamber: SOA Yields and Impacts of Oxidants, NOx, and VOC Precursors J. Liu et al. https://doi.org/10.1021/acs.est.2c02630
- Evaluation of the chemical composition of gas- and particle-phase products of aromatic oxidation A. Mehra et al. https://doi.org/10.5194/acp-20-9783-2020
- Novel Findings on Molecular SOA Fingerprint Lists: Implications for Interaction of Multiprecursor Oxidation W. Zhu et al. https://doi.org/10.1021/acs.estlett.4c00585
- Synergistic formation of secondary organic aerosols at an urban-forested interface: The role of anthropogenic oxidants in biogenic precursor oxidation S. Kwon et al. https://doi.org/10.1016/j.envpol.2026.128556
22 citations as recorded by crossref.
- Modeling the Effects of Dimerization and Bulk Diffusion on the Evaporative Behavior of Secondary Organic Aerosol Formed from α-Pinene and 1,3,5-Trimethylbenzene Y. Morino et al. https://doi.org/10.1021/acsearthspacechem.0c00106
- Pathogenic Mechanisms of Secondary Organic Aerosols T. Déméautis et al. https://doi.org/10.1021/acs.chemrestox.1c00353
- Mass spectrometry-based Aerosolomics: a new approach to resolve sources, composition, and partitioning of secondary organic aerosol M. Thoma et al. https://doi.org/10.5194/amt-15-7137-2022
- Effects of driving conditions on aerosol formation from photooxidation of gasoline vehicles exhaust in Hong Kong H. Poon et al. https://doi.org/10.1016/j.atmosenv.2023.120089
- Effects of relative humidity on atmospheric organosulfur species derived from photooxidation and nocturnal chemistry in a forest environment L. Li et al. https://doi.org/10.1016/j.envpol.2024.125253
- Comparison of dimension reduction techniques in the analysis of mass spectrometry data S. Isokääntä et al. https://doi.org/10.5194/amt-13-2995-2020
- Tower-based profiles of wintertime secondary organic aerosols in the urban boundary layer over Guangzhou Y. Li et al. https://doi.org/10.1016/j.scitotenv.2024.175326
- Direct contribution of ammonia to α-pinene secondary organic aerosol formation L. Hao et al. https://doi.org/10.5194/acp-20-14393-2020
- A Closure Study of Secondary Organic Aerosol Estimation at an Urban Site of Yangtze River Delta, China Z. Wan et al. https://doi.org/10.3390/atmos13101679
- Effects of driving conditions on secondary aerosol formation from a GDI vehicle using an oxidation flow reactor N. Kuittinen et al. https://doi.org/10.1016/j.envpol.2021.117069
- Interaction between marine and terrestrial biogenic volatile organic compounds: Non-linear effect on secondary organic aerosol formation X. Chen et al. https://doi.org/10.1016/j.atmosenv.2024.120868
- Measurement report: New particle formation events observed during the COALA-2020 campaign J. Ramirez-Gamboa et al. https://doi.org/10.5194/acp-25-9937-2025
- Tracer-based characterization of source variations of PM2.5 and organic carbon in Shanghai influenced by the COVID-19 lockdown S. Zhu et al. https://doi.org/10.1039/D0FD00091D
- Suppression of anthropogenic secondary organic aerosol formation by isoprene K. Li et al. https://doi.org/10.1038/s41612-022-00233-x
- Source apportionment and secondary organic aerosol formation potential of VOCs in urban and suburban areas of South Korea K. Kim et al. https://doi.org/10.1016/j.apr.2026.102964
- Secondary organic aerosol formed by Euro 5 gasoline vehicle emissions: chemical composition and gas-to-particle phase partitioning E. Kostenidou et al. https://doi.org/10.5194/acp-24-2705-2024
- Enhanced secondary organic aerosol formation from the photo-oxidation of mixed anthropogenic volatile organic compounds J. Li et al. https://doi.org/10.5194/acp-21-7773-2021
- Measurement report: Effects of anthropogenic emissions and environmental factors on the formation of biogenic secondary organic aerosol (BSOA) in a coastal city of southeastern China Y. Hong et al. https://doi.org/10.5194/acp-22-7827-2022
- Monoterpene Photooxidation in a Continuous-Flow Chamber: SOA Yields and Impacts of Oxidants, NOx, and VOC Precursors J. Liu et al. https://doi.org/10.1021/acs.est.2c02630
- Evaluation of the chemical composition of gas- and particle-phase products of aromatic oxidation A. Mehra et al. https://doi.org/10.5194/acp-20-9783-2020
- Novel Findings on Molecular SOA Fingerprint Lists: Implications for Interaction of Multiprecursor Oxidation W. Zhu et al. https://doi.org/10.1021/acs.estlett.4c00585
- Synergistic formation of secondary organic aerosols at an urban-forested interface: The role of anthropogenic oxidants in biogenic precursor oxidation S. Kwon et al. https://doi.org/10.1016/j.envpol.2026.128556
Saved (final revised paper)
Latest update: 21 Jun 2026
Short summary
We present, for the first time, the dual effect of GDI-vehicle exhaust on α-pinene SOA mass yield suppression. The first effect is a well-known NOx effect, but the second effect is more complex. Our results imply that this second effect is related to change of reaction pathways of α-pinene in the presence of GDI exhaust. The presence of vehicle exhaust caused more than 50 % suppression in α-pinene SOA mass yield compared to the α-pinene SOA mass yield measured in the absence of GDI emissions.
We present, for the first time, the dual effect of GDI-vehicle exhaust on α-pinene SOA mass...
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