Articles | Volume 19, issue 24
https://doi.org/10.5194/acp-19-15545-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-15545-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Impact of isolated atmospheric aging processes on the cloud condensation nuclei activation of soot particles
Institute for Atmospheric and Climate Science, ETH Zurich, Zurich,
8092, Switzerland
Prem Lobo
Institute for Atmospheric and Climate Science, ETH Zurich, Zurich,
8092, Switzerland
Center of Excellence for Aerospace Particulate Emissions Reduction
Research, Missouri University of Science and Technology, Rolla, Missouri
65401, USA
now at: Metrology Research Centre, National Research Council Canada, Ottawa, Ontario K1A 0R6, Canada
David Neubauer
Institute for Atmospheric and Climate Science, ETH Zurich, Zurich,
8092, Switzerland
Ulrike Lohmann
Institute for Atmospheric and Climate Science, ETH Zurich, Zurich,
8092, Switzerland
Saskia Drossaart van Dusseldorp
Institute for Atmospheric and Climate Science, ETH Zurich, Zurich,
8092, Switzerland
Evelyn Mühlhofer
Institute for Atmospheric and Climate Science, ETH Zurich, Zurich,
8092, Switzerland
Institute for Atmospheric and Climate Science, ETH Zurich, Zurich,
8092, Switzerland
now at: Environmental and Health Protection Service, City of Zurich, Zurich, 8003, Switzerland
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Cited
13 citations as recorded by crossref.
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Addressing Complexity in Global Aerosol Climate Model Cloud Microphysics U. Proske et al. 10.1029/2022MS003571
- Assessing the potential for simplification in global climate model cloud microphysics U. Proske et al. 10.5194/acp-22-4737-2022
- Influence of the dry aerosol particle size distribution and morphology on the cloud condensation nuclei activation. An experimental and theoretical investigation J. Wu et al. 10.5194/acp-20-4209-2020
- Future warming exacerbated by aged-soot effect on cloud formation U. Lohmann et al. 10.1038/s41561-020-0631-0
- Observation of Structural Changes during Oxidation of Black and Brown Soot Using Raman Spectroscopy K. Le et al. 10.3390/c10020038
- Insights into chemical aging of urban aerosols over Delhi, India K. Pandey et al. 10.1016/j.aeaoa.2024.100296
- On the correlation between hygroscopic properties and chemical composition of cloud condensation nuclei obtained from the chemical aging of soot particles with O3 and SO2 J. Wu et al. 10.1016/j.scitotenv.2023.167745
- Aqueous aging of secondary organic aerosol coating onto black carbon: Insights from simultaneous L-ToF-AMS and SP-AMS measurements at an urban site in southern China L. Cao et al. 10.1016/j.jclepro.2021.129888
- Efficient droplet activation of ambient black carbon particles in a suburban environment P. Tian et al. 10.5194/acp-24-5149-2024
- Ozone Concentration versus Temperature: Atmospheric Aging of Soot Particles F. Friebel & A. Mensah 10.1021/acs.langmuir.9b02372
- Modelling Complex Refractive Indices of Sub-micron Pure and Polluted Dust based on Compositional Sensitive Analysis . Sarla et al. 10.1007/s12647-022-00547-4
- A Review of Progress in Constraining Global Black Carbon Climate Effects J. Everett et al. 10.1007/s41748-022-00313-1
10 citations as recorded by crossref.
- Variability in morphology of soot particles during non-cloud and in-cloud processes Y. Wang et al. 10.1016/j.atmosenv.2024.120489
- Addressing Complexity in Global Aerosol Climate Model Cloud Microphysics U. Proske et al. 10.1029/2022MS003571
- Assessing the potential for simplification in global climate model cloud microphysics U. Proske et al. 10.5194/acp-22-4737-2022
- Influence of the dry aerosol particle size distribution and morphology on the cloud condensation nuclei activation. An experimental and theoretical investigation J. Wu et al. 10.5194/acp-20-4209-2020
- Future warming exacerbated by aged-soot effect on cloud formation U. Lohmann et al. 10.1038/s41561-020-0631-0
- Observation of Structural Changes during Oxidation of Black and Brown Soot Using Raman Spectroscopy K. Le et al. 10.3390/c10020038
- Insights into chemical aging of urban aerosols over Delhi, India K. Pandey et al. 10.1016/j.aeaoa.2024.100296
- On the correlation between hygroscopic properties and chemical composition of cloud condensation nuclei obtained from the chemical aging of soot particles with O3 and SO2 J. Wu et al. 10.1016/j.scitotenv.2023.167745
- Aqueous aging of secondary organic aerosol coating onto black carbon: Insights from simultaneous L-ToF-AMS and SP-AMS measurements at an urban site in southern China L. Cao et al. 10.1016/j.jclepro.2021.129888
- Efficient droplet activation of ambient black carbon particles in a suburban environment P. Tian et al. 10.5194/acp-24-5149-2024
3 citations as recorded by crossref.
- Ozone Concentration versus Temperature: Atmospheric Aging of Soot Particles F. Friebel & A. Mensah 10.1021/acs.langmuir.9b02372
- Modelling Complex Refractive Indices of Sub-micron Pure and Polluted Dust based on Compositional Sensitive Analysis . Sarla et al. 10.1007/s12647-022-00547-4
- A Review of Progress in Constraining Global Black Carbon Climate Effects J. Everett et al. 10.1007/s41748-022-00313-1
Latest update: 14 Dec 2024
Short summary
We investigated the change in cloud droplet activity of size-selected soot particles after being exposed to atmospheric levels of ozone over the course of 12 h. For this, we operated a 3 m3 aerosol chamber in continuous-flow mode. The results were fed into a climate model (ECHAM-HAM). We found that the oxidation of soot particles with ozone is a significant source of cloud condensation nuclei in the atmosphere.
We investigated the change in cloud droplet activity of size-selected soot particles after being...
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