Articles | Volume 19, issue 23
https://doi.org/10.5194/acp-19-15007-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-15007-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
11 Dec 2019
Research article |
| 11 Dec 2019
| 11 Dec 2019
Secondary organic aerosol formation from OH-initiated oxidation of m-xylene: effects of relative humidity on yield and chemical composition
Qun Zhang
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
Department of Atmospheric Chemistry and Environmental Sciences,
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Yongfu Xu
CORRESPONDING AUTHOR
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
Department of Atmospheric Chemistry and Environmental Sciences,
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
Long Jia
State Key Laboratory of Atmospheric Boundary Layer Physics and
Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of
Sciences, Beijing 100029, China
Department of Atmospheric Chemistry and Environmental Sciences,
College of Earth Sciences, University of Chinese Academy of Sciences,
Beijing 100049, China
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- Functionality-based formation of secondary organic aerosol fromm-xylene photooxidation Y. Li et al. 10.5194/acp-22-9843-2022
- The formation mechanism of highly oxygenated organic molecules produced by toluene in the urban atmosphere Z. Dong et al. 10.1016/j.atmosenv.2022.119555
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
- Effects of NO2 and RH on secondary organic aerosol formation and light absorption from OH oxidation of ο-xylene S. Liu et al. 10.1016/j.chemosphere.2022.136541
- On-line study of the influence of seed particle acidity on ozonation reaction of pyrene S. Zhu et al. 10.1016/j.atmosenv.2021.118615
- Smog chamber study of the effects of NOx and NH3 on the formation of secondary organic aerosols and optical properties from photo-oxidation of toluene X. Qi et al. 10.1016/j.scitotenv.2020.138632
- Hydroxymethanesulfonate formation as a significant pathway of transformation of SO2 H. Zhang et al. 10.1016/j.atmosenv.2022.119474
- Evaluation of Secondary Organic Aerosol (SOA) Simulations for Seoul, Korea Y. Oak et al. 10.1029/2021MS002760
- Different chlorine and hydroxyl radical environments impact m-xylene oxidation products N. Bhattacharyya et al. 10.1039/D3EA00024A
- Oligomer formation from cross-reaction of Criegee intermediates in the styrene-isoprene-O3 mixed system S. Yu et al. 10.1016/j.chemosphere.2023.140811
- Variability in Aromatic Aerosol Yields under Very Low NOxConditions at Different HO2/RO2Regimes W. Peng et al. 10.1021/acs.est.1c04392
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- Molecular composition of secondary organic aerosol from styrene under different NO and humidity conditions S. Yu et al. 10.1016/j.atmosres.2021.105950
- Heterogeneous reaction of toluene/NO2/O3 on α-Fe2O3 nanoparticles: the impacts of O3, light illumination, and relative humidity on the formation of N-containing organic compounds (NOC) X. He et al. 10.1039/D2EN00426G
- Wall losses of oxygenated volatile organic compounds from oxidation of toluene: Effects of chamber volume and relative humidity S. Yu et al. 10.1016/j.jes.2021.09.026
- Molecular composition and sources of water-soluble organic aerosol in summer in Beijing Y. Qiu et al. 10.1016/j.chemosphere.2020.126850
- Atmospheric OH Oxidation Chemistry of Particulate Liquid Crystal Monomers: An Emerging Persistent Organic Pollutant in Air Q. Liu et al. 10.1021/acs.estlett.0c00447
- A core-shell box model for simulating viscosity dependent secondary organic aerosol (CSVA) and its application L. Jia & Y. Xu 10.1016/j.scitotenv.2021.147954
- The underappreciated role of monocarbonyl-dicarbonyl interconversion in secondary organic aerosol formation during photochemical oxidation of m-xylene J. Chen et al. 10.1016/j.scitotenv.2021.152575
- Effect of relative humidity on SOA formation from aromatic hydrocarbons: Implications from the evolution of gas- and particle-phase species T. Chen et al. 10.1016/j.scitotenv.2021.145015
- The role of functional groups in the understanding of secondary organic aerosol formation mechanism from α-pinene L. Jia & Y. Xu 10.1016/j.scitotenv.2020.139831
- Evaluation of reaction between SO2 and CH2OO in MCM mechanism against smog chamber data from ethylene ozonolysis H. Zhang et al. 10.1071/EN23029
28 citations as recorded by crossref.
- Influence of Ammonia and Relative Humidity on the Formation and Composition of Secondary Brown Carbon from Oxidation of 1-Methylnaphthalene and Longifolene Y. Cui et al. 10.1021/acsearthspacechem.0c00353
- Particle-Bound Highly Oxidized Organic Molecules Derived from Aromatic Hydrocarbons in an Urban Atmosphere M. Zhu et al. 10.1021/acs.estlett.2c00841
- Air pollution from unconventional oil and gas development in the Eagle Ford Shale K. McPherson et al. 10.1016/j.atmosenv.2024.120812
- Effects of Relative Humidity and Photoaging on the Formation, Composition, and Aging of Ethylbenzene SOA: Insights from Chamber Experiments on Chlorine Radical-Initiated Oxidation of Ethylbenzene L. Jahn et al. 10.1021/acsearthspacechem.3c00279
- A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system T. Pan et al. 10.5194/amt-17-4915-2024
- Functionality-based formation of secondary organic aerosol fromm-xylene photooxidation Y. Li et al. 10.5194/acp-22-9843-2022
- The formation mechanism of highly oxygenated organic molecules produced by toluene in the urban atmosphere Z. Dong et al. 10.1016/j.atmosenv.2022.119555
- Review of Smog Chamber Research Trends J. Kim et al. 10.5572/KOSAE.2023.39.5.866
- Effects of NO2 and RH on secondary organic aerosol formation and light absorption from OH oxidation of ο-xylene S. Liu et al. 10.1016/j.chemosphere.2022.136541
- On-line study of the influence of seed particle acidity on ozonation reaction of pyrene S. Zhu et al. 10.1016/j.atmosenv.2021.118615
- Smog chamber study of the effects of NOx and NH3 on the formation of secondary organic aerosols and optical properties from photo-oxidation of toluene X. Qi et al. 10.1016/j.scitotenv.2020.138632
- Hydroxymethanesulfonate formation as a significant pathway of transformation of SO2 H. Zhang et al. 10.1016/j.atmosenv.2022.119474
- Evaluation of Secondary Organic Aerosol (SOA) Simulations for Seoul, Korea Y. Oak et al. 10.1029/2021MS002760
- Different chlorine and hydroxyl radical environments impact m-xylene oxidation products N. Bhattacharyya et al. 10.1039/D3EA00024A
- Oligomer formation from cross-reaction of Criegee intermediates in the styrene-isoprene-O3 mixed system S. Yu et al. 10.1016/j.chemosphere.2023.140811
- Variability in Aromatic Aerosol Yields under Very Low NOxConditions at Different HO2/RO2Regimes W. Peng et al. 10.1021/acs.est.1c04392
- Secondary organic aerosol formation from monocyclic aromatic hydrocarbons: insights from laboratory studies Z. Yang et al. 10.1039/D1EM00409C
- Effect of NOx and RH on the secondary organic aerosol formation from toluene photooxidation S. Liu et al. 10.1016/j.jes.2021.06.017
- Molecular composition of secondary organic aerosol from styrene under different NO and humidity conditions S. Yu et al. 10.1016/j.atmosres.2021.105950
- Heterogeneous reaction of toluene/NO2/O3 on α-Fe2O3 nanoparticles: the impacts of O3, light illumination, and relative humidity on the formation of N-containing organic compounds (NOC) X. He et al. 10.1039/D2EN00426G
- Wall losses of oxygenated volatile organic compounds from oxidation of toluene: Effects of chamber volume and relative humidity S. Yu et al. 10.1016/j.jes.2021.09.026
- Molecular composition and sources of water-soluble organic aerosol in summer in Beijing Y. Qiu et al. 10.1016/j.chemosphere.2020.126850
- Atmospheric OH Oxidation Chemistry of Particulate Liquid Crystal Monomers: An Emerging Persistent Organic Pollutant in Air Q. Liu et al. 10.1021/acs.estlett.0c00447
- A core-shell box model for simulating viscosity dependent secondary organic aerosol (CSVA) and its application L. Jia & Y. Xu 10.1016/j.scitotenv.2021.147954
- The underappreciated role of monocarbonyl-dicarbonyl interconversion in secondary organic aerosol formation during photochemical oxidation of m-xylene J. Chen et al. 10.1016/j.scitotenv.2021.152575
- Effect of relative humidity on SOA formation from aromatic hydrocarbons: Implications from the evolution of gas- and particle-phase species T. Chen et al. 10.1016/j.scitotenv.2021.145015
- The role of functional groups in the understanding of secondary organic aerosol formation mechanism from α-pinene L. Jia & Y. Xu 10.1016/j.scitotenv.2020.139831
- Evaluation of reaction between SO2 and CH2OO in MCM mechanism against smog chamber data from ethylene ozonolysis H. Zhang et al. 10.1071/EN23029
Latest update: 19 Nov 2024
Short summary
The negative effects of relative humidity (RH) on secondary organic aerosol (SOA) formation from m-xylene under low NOx conditions were observed. The mechanisms of the RH effects of SOA yields have been sufficiently discussed. The decrease of SOA formation at high RH may be mainly attributed to the suppression of oligomers and the further particle-phase reaction of highly oxygenated organic molecules. The faster wall loss of SOA precursors at higher RH may also influence the SOA yield.
The negative effects of relative humidity (RH) on secondary organic aerosol (SOA) formation from...
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