Articles | Volume 19, issue 22
https://doi.org/10.5194/acp-19-13945-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-13945-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Molecular characterization of polar organic aerosol constituents in off-road engine emissions using Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS): implications for source apportionment
Min Cui
College of Environmental Science and Engineering, Tongji University, Shanghai 200092, P.R. China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, P.R. China
Cheng Li
Institute for Environmental and Climate Research, Jinan University, Guangzhou, 511443, P.R. China
Shanghai Key Laboratory of Atmospheric Particle Pollution and
Prevention (LAP3), Department of Environmental Science and Engineering,
Fudan University, Shanghai 200433, P.R. China
College of Environmental Science and Engineering, Tongji University, Shanghai 200092, P.R. China
Fan Zhang
College of Environmental Science and Engineering, Tongji University, Shanghai 200092, P.R. China
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, P.R. China
Bin Jiang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, P.R. China
Yangzhi Mo
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, P.R. China
Jia Li
School of Environmental Science and Engineering, Yangzhou University,
Yangzhou 225127, P.R. China
Caiqing Yan
SKL-ESPC and BIC-EAST, College of Environmental Sciences and
Engineering, Peking University, Beijing 100871, P.R. China
Mei Zheng
SKL-ESPC and BIC-EAST, College of Environmental Sciences and
Engineering, Peking University, Beijing 100871, P.R. China
Zhiyong Xie
Centre for Materials and Coastal
Research, Institute of Coastal Research, Helmholtz-Zentrum Geesthacht, Geesthacht, 21502, Germany
Gan Zhang
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, P.R. China
Junyu Zheng
CORRESPONDING AUTHOR
Institute for Environmental and Climate Research, Jinan University, Guangzhou, 511443, P.R. China
Viewed
Total article views: 2,648 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 23 May 2019)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
1,782 | 812 | 54 | 2,648 | 336 | 58 | 89 |
- HTML: 1,782
- PDF: 812
- XML: 54
- Total: 2,648
- Supplement: 336
- BibTeX: 58
- EndNote: 89
Total article views: 2,009 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 20 Nov 2019)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
1,420 | 541 | 48 | 2,009 | 195 | 51 | 80 |
- HTML: 1,420
- PDF: 541
- XML: 48
- Total: 2,009
- Supplement: 195
- BibTeX: 51
- EndNote: 80
Total article views: 639 (including HTML, PDF, and XML)
Cumulative views and downloads
(calculated since 23 May 2019)
HTML | XML | Total | Supplement | BibTeX | EndNote | |
---|---|---|---|---|---|---|
362 | 271 | 6 | 639 | 141 | 7 | 9 |
- HTML: 362
- PDF: 271
- XML: 6
- Total: 639
- Supplement: 141
- BibTeX: 7
- EndNote: 9
Viewed (geographical distribution)
Total article views: 2,648 (including HTML, PDF, and XML)
Thereof 2,528 with geography defined
and 120 with unknown origin.
Total article views: 2,009 (including HTML, PDF, and XML)
Thereof 2,008 with geography defined
and 1 with unknown origin.
Total article views: 639 (including HTML, PDF, and XML)
Thereof 520 with geography defined
and 119 with unknown origin.
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Country | # | Views | % |
---|
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Total: | 0 |
HTML: | 0 |
PDF: | 0 |
XML: | 0 |
- 1
1
Cited
25 citations as recorded by crossref.
- Emission Characteristics and Formation Pathways of Intermediate Volatile Organic Compounds from Ocean-Going Vessels: Comparison of Engine Conditions and Fuel Types Z. Liu et al. 10.1021/acs.est.2c03589
- Biomass burning organic aerosols significantly influence the light absorption properties of polarity-dependent organic compounds in the Pearl River Delta Region, China H. Jiang et al. 10.1016/j.envint.2020.106079
- Spatial and diurnal variations of aerosol organosulfates in summertime Shanghai, China: potential influence of photochemical processes and anthropogenic sulfate pollution T. Yang et al. 10.5194/acp-23-13433-2023
- Variations in the oxidation potential of PM2.5 in an old industrial city in China from 2015 to 2018 Z. Wang et al. 10.1016/j.scitotenv.2024.174639
- Size‐dependent Molecular Characteristics and Possible Sources of Organic Aerosols at a Coastal New Particle Formation Hotspot of East China Y. Wan et al. 10.1029/2021JD034610
- Impact of sulfur functional groups on physicochemical properties and oxidation reactivity of diesel soot particles B. Zhao et al. 10.1016/j.fuel.2022.125041
- Variability in real-world emissions and fuel consumption by diesel construction vehicles and policy implications C. Li et al. 10.1016/j.scitotenv.2021.147256
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- Molecular characteristics, sources, and formation pathways of organosulfur compounds in ambient aerosol in Guangzhou, South China H. Jiang et al. 10.5194/acp-22-6919-2022
- Impact of fossil and non-fossil fuel sources on the molecular compositions of water-soluble humic-like substances in PM2.5 at a suburban site of Yangtze River Delta, China M. Bao et al. 10.5194/acp-23-8305-2023
- Nitrogen‐Containing Functional Groups Dominate the Molecular Absorption of Water‐Soluble Humic‐Like Substances in Air From Nanjing, China Revealed by the Machine Learning Combined FT‐ICR‐MS Technique Y. Hong et al. 10.1029/2023JD039459
- Factors Influencing the Molecular Compositions and Distributions of Atmospheric Nitrogen‐Containing Compounds H. Jiang et al. 10.1029/2021JD036284
- Insight into the Variability of the Nitrogen Isotope Composition of Vehicular NOx in China Z. Zong et al. 10.1021/acs.est.0c04749
- Source profiles of molecular structure and light absorption of PM2.5 brown carbon from residential coal combustion emission in Northwestern China Q. Zhang et al. 10.1016/j.envpol.2022.118866
- Molecular characterization of major oxidative potential active species in ambient PM2.5: Emissions from biomass burning and ship exhaust C. Xing et al. 10.1016/j.envpol.2024.125291
- Characteristics of polar organic compounds from diesel truck emissions measured by FT-ICR MS C. Min et al. 10.1016/j.atmosenv.2023.120319
- Molecular Characterization of Water‐Soluble Brown Carbon Chromophores in Beijing, China C. Yan et al. 10.1029/2019JD032018
- Parent and methyl polycyclic aromatic hydrocarbons and n-alkanes emitted by construction machinery in China M. Cui et al. 10.1016/j.scitotenv.2020.144759
- Molecular characterization of atmospheric particulate organosulfates in a port environment using ultrahigh resolution mass spectrometry: Identification of traffic emissions L. Qi et al. 10.1016/j.jhazmat.2021.126431
- Molecular Dynamics and Light Absorption Properties of Atmospheric Dissolved Organic Matter H. Jiang et al. 10.1021/acs.est.1c01770
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Seasonal dynamics of airborne biomolecules influence the size distribution of Arctic aerosols E. Jang et al. 10.1016/j.ese.2024.100458
- Molecular Signatures and Sources of Fluorescent Components in Atmospheric Organic Matter in South China H. Jiang et al. 10.1021/acs.estlett.2c00629
- Humic-like Substances (HULIS) in Ship Engine Emissions: Molecular Composition Effected by Fuel Type, Engine Mode, and Wet Scrubber Usage E. Schneider et al. 10.1021/acs.est.3c04390
- Molecular Characterization of Water- and Methanol-Soluble Organic Compounds Emitted from Residential Coal Combustion Using Ultrahigh-Resolution Electrospray Ionization Fourier Transform Ion Cyclotron Resonance Mass Spectrometry J. Song et al. 10.1021/acs.est.9b04331
24 citations as recorded by crossref.
- Emission Characteristics and Formation Pathways of Intermediate Volatile Organic Compounds from Ocean-Going Vessels: Comparison of Engine Conditions and Fuel Types Z. Liu et al. 10.1021/acs.est.2c03589
- Biomass burning organic aerosols significantly influence the light absorption properties of polarity-dependent organic compounds in the Pearl River Delta Region, China H. Jiang et al. 10.1016/j.envint.2020.106079
- Spatial and diurnal variations of aerosol organosulfates in summertime Shanghai, China: potential influence of photochemical processes and anthropogenic sulfate pollution T. Yang et al. 10.5194/acp-23-13433-2023
- Variations in the oxidation potential of PM2.5 in an old industrial city in China from 2015 to 2018 Z. Wang et al. 10.1016/j.scitotenv.2024.174639
- Size‐dependent Molecular Characteristics and Possible Sources of Organic Aerosols at a Coastal New Particle Formation Hotspot of East China Y. Wan et al. 10.1029/2021JD034610
- Impact of sulfur functional groups on physicochemical properties and oxidation reactivity of diesel soot particles B. Zhao et al. 10.1016/j.fuel.2022.125041
- Variability in real-world emissions and fuel consumption by diesel construction vehicles and policy implications C. Li et al. 10.1016/j.scitotenv.2021.147256
- Measurement report: Changes in light absorption and molecular composition of water-soluble humic-like substances during a winter haze bloom-decay process in Guangzhou, China C. Zou et al. 10.5194/acp-23-963-2023
- Molecular characteristics, sources, and formation pathways of organosulfur compounds in ambient aerosol in Guangzhou, South China H. Jiang et al. 10.5194/acp-22-6919-2022
- Impact of fossil and non-fossil fuel sources on the molecular compositions of water-soluble humic-like substances in PM2.5 at a suburban site of Yangtze River Delta, China M. Bao et al. 10.5194/acp-23-8305-2023
- Nitrogen‐Containing Functional Groups Dominate the Molecular Absorption of Water‐Soluble Humic‐Like Substances in Air From Nanjing, China Revealed by the Machine Learning Combined FT‐ICR‐MS Technique Y. Hong et al. 10.1029/2023JD039459
- Factors Influencing the Molecular Compositions and Distributions of Atmospheric Nitrogen‐Containing Compounds H. Jiang et al. 10.1029/2021JD036284
- Insight into the Variability of the Nitrogen Isotope Composition of Vehicular NOx in China Z. Zong et al. 10.1021/acs.est.0c04749
- Source profiles of molecular structure and light absorption of PM2.5 brown carbon from residential coal combustion emission in Northwestern China Q. Zhang et al. 10.1016/j.envpol.2022.118866
- Molecular characterization of major oxidative potential active species in ambient PM2.5: Emissions from biomass burning and ship exhaust C. Xing et al. 10.1016/j.envpol.2024.125291
- Characteristics of polar organic compounds from diesel truck emissions measured by FT-ICR MS C. Min et al. 10.1016/j.atmosenv.2023.120319
- Molecular Characterization of Water‐Soluble Brown Carbon Chromophores in Beijing, China C. Yan et al. 10.1029/2019JD032018
- Parent and methyl polycyclic aromatic hydrocarbons and n-alkanes emitted by construction machinery in China M. Cui et al. 10.1016/j.scitotenv.2020.144759
- Molecular characterization of atmospheric particulate organosulfates in a port environment using ultrahigh resolution mass spectrometry: Identification of traffic emissions L. Qi et al. 10.1016/j.jhazmat.2021.126431
- Molecular Dynamics and Light Absorption Properties of Atmospheric Dissolved Organic Matter H. Jiang et al. 10.1021/acs.est.1c01770
- Influence of organic aerosol molecular composition on particle absorptive properties in autumn Beijing J. Cai et al. 10.5194/acp-22-1251-2022
- Seasonal dynamics of airborne biomolecules influence the size distribution of Arctic aerosols E. Jang et al. 10.1016/j.ese.2024.100458
- Molecular Signatures and Sources of Fluorescent Components in Atmospheric Organic Matter in South China H. Jiang et al. 10.1021/acs.estlett.2c00629
- Humic-like Substances (HULIS) in Ship Engine Emissions: Molecular Composition Effected by Fuel Type, Engine Mode, and Wet Scrubber Usage E. Schneider et al. 10.1021/acs.est.3c04390
1 citations as recorded by crossref.
Latest update: 14 Dec 2024
Short summary
Refined source apportionment is urgently needed but hard to achieve due to a lack of specific biomarkers. Recently, Fourier transform ion cyclotron resonance mass spectrometry has been used to analyse the probable chemical structure of polar organic matter emitted from off-road engines. We found more condensed aromatic rings in S-containing compounds for HFO-fueled vessels, while more abundant aliphatic chains were observed in emissions from diesel equipment.
Refined source apportionment is urgently needed but hard to achieve due to a lack of specific...
Altmetrics
Final-revised paper
Preprint