Articles | Volume 19, issue 20
https://doi.org/10.5194/acp-19-13289-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-13289-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Semi-quantitative understanding of source contribution to nitrous acid (HONO) based on 1 year of continuous observation at the SORPES station in eastern China
Yuliang Liu
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Wei Nie
CORRESPONDING AUTHOR
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Zheng Xu
CORRESPONDING AUTHOR
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Tianyi Wang
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Ruoxian Wang
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Yuanyuan Li
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Lei Wang
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Xuguang Chi
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
Aijun Ding
Joint International Research Laboratory of Atmospheric and Earth
System Sciences, School of Atmospheric Sciences, Nanjing University,
Nanjing, Jiangsu Province, 210023, China
Jiangsu Provincial Collaborative Innovation Center of Climate Change, Nanjing, Jiangsu Province, 210023, China
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63 citations as recorded by crossref.
- Detection of nitrous acid in the atmospheric simulation chamber SAPHIR using open-path incoherent broadband cavity-enhanced absorption spectroscopy and extractive long-path absorption photometry S. Dixneuf et al. 10.5194/amt-15-945-2022
- The effect of nitrous acid (HONO) on ozone formation during pollution episodes in southeastern China: Results from model improvement and mechanism insights B. Hu et al. 10.1016/j.scitotenv.2023.164477
- Exploring HONO formation and its role in driving secondary pollutants formation during winter in the North China Plain S. Zhang et al. 10.1016/j.jes.2022.09.034
- Formation mechanisms and atmospheric implications of summertime nitrous acid (HONO) during clean, ozone pollution and double high-level PM2.5 and O3 pollution periods in Beijing H. Xuan et al. 10.1016/j.scitotenv.2022.159538
- Denitrification is the major nitrous acid production pathway in boreal agricultural soils H. Bhattarai et al. 10.1038/s43247-021-00125-7
- A review of indoor nitrous acid (HONO) pollution: Measurement techniques, pollution characteristics, sources, and sinks C. Liu et al. 10.1016/j.scitotenv.2024.171100
- Atmospheric oxidation capacity and secondary pollutant formation potentials based on photochemical loss of VOCs in a megacity of the Sichuan Basin, China L. Kong et al. 10.1016/j.scitotenv.2023.166259
- Measurement of HONO flux using the aerodynamic gradient method over an agricultural field in the Huaihe River Basin, China F. Meng et al. 10.1016/j.jes.2021.09.005
- Modeling the Formation of Organic Compounds across Full Volatility Ranges and Their Contribution to Nanoparticle Growth in a Polluted Atmosphere Z. Li et al. 10.1021/acs.est.3c06708
- The promotion effect of nitrous acid on aerosol formation in wintertime in Beijing: the possible contribution of traffic-related emissions Y. Liu et al. 10.5194/acp-20-13023-2020
- Response of organic aerosol characteristics to emission reduction in Yangtze River Delta region J. Wang et al. 10.1007/s11783-023-1714-0
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- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
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- Accurately Predicting Spatiotemporal Variations of Near-Surface Nitrous Acid (HONO) Based on a Deep Learning Approach X. Li et al. 10.1021/acs.est.4c02221
- Atmospheric HONO formation during and after the Spring Festival holidays in a coastal city of China X. Ni et al. 10.1016/j.jes.2022.05.043
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- Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels R. Miao et al. 10.5194/acp-21-16183-2021
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- Explainable Machine Learning Reveals the Unknown Sources of Atmospheric HONO during COVID-19 Z. Gao et al. 10.1021/acsestair.4c00087
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- Secondary aerosol formation and its linkage with synoptic conditions during winter haze pollution over eastern China T. Wang et al. 10.1016/j.scitotenv.2020.138888
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- Vertical distributions of wintertime atmospheric nitrogenous compounds and the corresponding OH radicals production in Leshan, southwest China C. Xing et al. 10.1016/j.jes.2020.11.019
- A systematic review of reactive nitrogen simulations with chemical transport models in China H. Zhang et al. 10.1016/j.atmosres.2024.107586
- Reduction and Photoreduction of NO2 in Humic Acid Films as a Source of HONO, ClNO, N2O, NOX, and Organic Nitrogen H. Ricker et al. 10.1021/acsearthspacechem.2c00282
- Dominant Processes of HONO Derived from Multiple Field Observations in Contrasting Environments Y. Jiang et al. 10.1021/acs.estlett.2c00004
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- Ground-level ozone pollution in China: a synthesis of recent findings on influencing factors and impacts T. Wang et al. 10.1088/1748-9326/ac69fe
- The Levels and Sources of Nitrous Acid (HONO) in Winter of Beijing and Sanmenxia X. Zhang et al. 10.1029/2021JD036278
- Budget of nitrous acid (HONO) at an urban site in the fall season of Guangzhou, China Y. Yu et al. 10.5194/acp-22-8951-2022
- Key Role of Equilibrium HONO Concentration over Soil in Quantifying Soil–Atmosphere HONO Fluxes F. Bao et al. 10.1021/acs.est.1c06716
- Pollution characteristics and potential sources of nitrous acid (HONO) in early autumn 2018 of Beijing C. Jia et al. 10.1016/j.scitotenv.2020.139317
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- Contribution of Vehicle Emission and NO2 Surface Conversion to Nitrous Acid (HONO) in Urban Environments: Implications from Tests in a Tunnel S. Li et al. 10.1021/acs.est.1c00405
- Exploring condensable organic vapors and their co-occurrence with PM2.5and O3in winter in Eastern China Y. Liu et al. 10.1039/D2EA00143H
- Atmospheric oxidizing capacity in autumn Beijing: Analysis of the O3 and PM2.5 episodes based on observation-based model C. Jia et al. 10.1016/j.jes.2021.11.020
- Investigation on the budget of peroxyacetyl nitrate (PAN) in the Yangtze River Delta: Unravelling local photochemistry and regional impact T. Xu et al. 10.1016/j.scitotenv.2024.170373
- Observations of the vertical distributions of summertime atmospheric pollutants in Nam Co: OH production and source analysis C. Xing et al. 10.5194/acp-24-10093-2024
- Machine learning revealing key factors influencing HONO chemistry in Beijing during heating and non-heating periods W. Zhang et al. 10.1016/j.atmosres.2023.107130
- Aerosol Promotes Peroxyacetyl Nitrate Formation During Winter in the North China Plain W. Xu et al. 10.1021/acs.est.0c08157
- Influence of ship direct emission on HONO sources in channel environment Y. Guo et al. 10.1016/j.atmosenv.2020.117819
- Unveiling the underestimated direct emissions of nitrous acid (HONO) Q. Zhang et al. 10.1073/pnas.2302048120
- Origins of atmospheric nitrous acid and their contributions to OH radical from ship plumes, marine atmosphere, and continental air masses over South China Sea X. Ni et al. 10.1016/j.scitotenv.2024.175841
- Investigating the sources of atmospheric nitrous acid (HONO) in the megacity of Beijing, China R. Gu et al. 10.1016/j.scitotenv.2021.152270
- Exploring the HONO source during the COVID-19 pandemic in a megacity in China M. Wang et al. 10.1016/j.jes.2023.12.021
- A new insight into the vertical differences in NO2 heterogeneous reaction to produce HONO over inland and marginal seas C. Xing et al. 10.5194/acp-23-5815-2023
- Exploration of the atmospheric chemistry of nitrous acid in a coastal city of southeastern China: results from measurements across four seasons B. Hu et al. 10.5194/acp-22-371-2022
- Effect of Different Combustion Processes on Atmospheric Nitrous Acid Formation Mechanisms: A Winter Comparative Observation in Urban, Suburban and Rural Areas of the North China Plain W. Zhang et al. 10.1021/acs.est.1c07784
- Observations of HONO and its precursors between urban and its surrounding agricultural fields: The vertical transports, sources and contribution to OH C. Xing et al. 10.1016/j.scitotenv.2023.169159
- Seasonality of nitrous acid near an industry zone in the Yangtze River Delta region of China: Formation mechanisms and contribution to the atmospheric oxidation capacity Y. Ge et al. 10.1016/j.atmosenv.2021.118420
- Formation of condensable organic vapors from anthropogenic and biogenic volatile organic compounds (VOCs) is strongly perturbed by NO<sub><i>x</i></sub> in eastern China Y. Liu et al. 10.5194/acp-21-14789-2021
- The impacts of marine-emitted halogens on OH radicals in East Asia during summer S. Fan & Y. Li 10.5194/acp-22-7331-2022
- Long-term winter observation of nitrous acid in the urban area of Beijing C. Lian et al. 10.1016/j.jes.2021.09.010
- An investigation into the chemistry of HONO in the marine boundary layer at Tudor Hill Marine Atmospheric Observatory in Bermuda Y. Zhu et al. 10.5194/acp-22-6327-2022
- Elucidating HONO formation mechanism and its essential contribution to OH during haze events X. Zhang et al. 10.1038/s41612-023-00371-w
63 citations as recorded by crossref.
- Detection of nitrous acid in the atmospheric simulation chamber SAPHIR using open-path incoherent broadband cavity-enhanced absorption spectroscopy and extractive long-path absorption photometry S. Dixneuf et al. 10.5194/amt-15-945-2022
- The effect of nitrous acid (HONO) on ozone formation during pollution episodes in southeastern China: Results from model improvement and mechanism insights B. Hu et al. 10.1016/j.scitotenv.2023.164477
- Exploring HONO formation and its role in driving secondary pollutants formation during winter in the North China Plain S. Zhang et al. 10.1016/j.jes.2022.09.034
- Formation mechanisms and atmospheric implications of summertime nitrous acid (HONO) during clean, ozone pollution and double high-level PM2.5 and O3 pollution periods in Beijing H. Xuan et al. 10.1016/j.scitotenv.2022.159538
- Denitrification is the major nitrous acid production pathway in boreal agricultural soils H. Bhattarai et al. 10.1038/s43247-021-00125-7
- A review of indoor nitrous acid (HONO) pollution: Measurement techniques, pollution characteristics, sources, and sinks C. Liu et al. 10.1016/j.scitotenv.2024.171100
- Atmospheric oxidation capacity and secondary pollutant formation potentials based on photochemical loss of VOCs in a megacity of the Sichuan Basin, China L. Kong et al. 10.1016/j.scitotenv.2023.166259
- Measurement of HONO flux using the aerodynamic gradient method over an agricultural field in the Huaihe River Basin, China F. Meng et al. 10.1016/j.jes.2021.09.005
- Modeling the Formation of Organic Compounds across Full Volatility Ranges and Their Contribution to Nanoparticle Growth in a Polluted Atmosphere Z. Li et al. 10.1021/acs.est.3c06708
- The promotion effect of nitrous acid on aerosol formation in wintertime in Beijing: the possible contribution of traffic-related emissions Y. Liu et al. 10.5194/acp-20-13023-2020
- Response of organic aerosol characteristics to emission reduction in Yangtze River Delta region J. Wang et al. 10.1007/s11783-023-1714-0
- Atmospheric nitrous acid (HONO) in an alternate process of haze pollution and ozone pollution in urban Beijing in summertime: Variations, sources and contribution to atmospheric photochemistry Y. Li et al. 10.1016/j.atmosres.2021.105689
- Toward Building a Physical Proxy for Gas-Phase Sulfuric Acid Concentration Based on Its Budget Analysis in Polluted Yangtze River Delta, East China L. Yang et al. 10.1021/acs.est.1c00738
- Springtime HONO budget and its impact on the O3 production in Zibo, Shandong, China Z. Qin et al. 10.1016/j.apr.2023.101935
- Accurately Predicting Spatiotemporal Variations of Near-Surface Nitrous Acid (HONO) Based on a Deep Learning Approach X. Li et al. 10.1021/acs.est.4c02221
- Atmospheric HONO formation during and after the Spring Festival holidays in a coastal city of China X. Ni et al. 10.1016/j.jes.2022.05.043
- HONO chemistry at a suburban site during the EXPLORE-YRD campaign in 2018: formation mechanisms and impacts on O3 production C. Ye et al. 10.5194/acp-23-15455-2023
- Process-based and observation-constrained SOA simulations in China: the role of semivolatile and intermediate-volatility organic compounds and OH levels R. Miao et al. 10.5194/acp-21-16183-2021
- Seasonal Characteristics of HONO Variations in Seoul during 2021~2022 J. Gil et al. 10.5572/KOSAE.2023.39.3.308
- Explainable Machine Learning Reveals the Unknown Sources of Atmospheric HONO during COVID-19 Z. Gao et al. 10.1021/acsestair.4c00087
- Impact of international shipping emissions on ozone and PM<sub>2.5</sub> in East Asia during summer: the important role of HONO and ClNO<sub>2</sub> J. Dai & T. Wang 10.5194/acp-21-8747-2021
- Secondary aerosol formation and its linkage with synoptic conditions during winter haze pollution over eastern China T. Wang et al. 10.1016/j.scitotenv.2020.138888
- High crop yield losses induced by potential HONO sources — A modelling study in the North China Plain J. Zhang et al. 10.1016/j.scitotenv.2021.149929
- Vertical distributions of wintertime atmospheric nitrogenous compounds and the corresponding OH radicals production in Leshan, southwest China C. Xing et al. 10.1016/j.jes.2020.11.019
- A systematic review of reactive nitrogen simulations with chemical transport models in China H. Zhang et al. 10.1016/j.atmosres.2024.107586
- Reduction and Photoreduction of NO2 in Humic Acid Films as a Source of HONO, ClNO, N2O, NOX, and Organic Nitrogen H. Ricker et al. 10.1021/acsearthspacechem.2c00282
- Dominant Processes of HONO Derived from Multiple Field Observations in Contrasting Environments Y. Jiang et al. 10.1021/acs.estlett.2c00004
- Characteristics of HONO and its impact on O3 formation in the Seoul Metropolitan Area during the Korea-US Air Quality study J. Gil et al. 10.1016/j.atmosenv.2020.118182
- Impact of air transport and secondary formation on haze pollution in the Yangtze River Delta: In situ online observations in Shanghai and Nanjing P. Sun et al. 10.1016/j.atmosenv.2020.117350
- Concentration and source changes of nitrous acid (HONO) during the COVID-19 lockdown in Beijing Y. Zhang et al. 10.5194/acp-24-8569-2024
- Ground-level ozone pollution in China: a synthesis of recent findings on influencing factors and impacts T. Wang et al. 10.1088/1748-9326/ac69fe
- The Levels and Sources of Nitrous Acid (HONO) in Winter of Beijing and Sanmenxia X. Zhang et al. 10.1029/2021JD036278
- Budget of nitrous acid (HONO) at an urban site in the fall season of Guangzhou, China Y. Yu et al. 10.5194/acp-22-8951-2022
- Key Role of Equilibrium HONO Concentration over Soil in Quantifying Soil–Atmosphere HONO Fluxes F. Bao et al. 10.1021/acs.est.1c06716
- Pollution characteristics and potential sources of nitrous acid (HONO) in early autumn 2018 of Beijing C. Jia et al. 10.1016/j.scitotenv.2020.139317
- Direct Observation of HONO Emissions from Real-World Residential Natural Gas Heating in China X. Ding et al. 10.1021/acs.est.2c09386
- Budget of atmospheric nitrous acid (HONO) during the haze and clean periods in Shanghai: Importance of heterogeneous reactions J. Feng et al. 10.1016/j.scitotenv.2023.165717
- High-resolution vertical distribution and sources of HONO and NO<sub>2</sub> in the nocturnal boundary layer in urban Beijing, China F. Meng et al. 10.5194/acp-20-5071-2020
- Elucidating the effect of HONO on O3 pollution by a case study in southwest China Y. Yang et al. 10.1016/j.scitotenv.2020.144127
- Formation Mechanisms and Atmospheric Implications of Summertime Nitrous Acid (HONO) During Clean, Ozone Pollution and Double High Pollution Periods in Beijing H. Xuan et al. 10.2139/ssrn.4197029
- Formation mechanisms of nitrous acid (HONO) during the haze and non-haze periods in Beijing, China D. Lin et al. 10.1016/j.jes.2021.09.013
- Contribution of Vehicle Emission and NO2 Surface Conversion to Nitrous Acid (HONO) in Urban Environments: Implications from Tests in a Tunnel S. Li et al. 10.1021/acs.est.1c00405
- Exploring condensable organic vapors and their co-occurrence with PM2.5and O3in winter in Eastern China Y. Liu et al. 10.1039/D2EA00143H
- Atmospheric oxidizing capacity in autumn Beijing: Analysis of the O3 and PM2.5 episodes based on observation-based model C. Jia et al. 10.1016/j.jes.2021.11.020
- Investigation on the budget of peroxyacetyl nitrate (PAN) in the Yangtze River Delta: Unravelling local photochemistry and regional impact T. Xu et al. 10.1016/j.scitotenv.2024.170373
- Observations of the vertical distributions of summertime atmospheric pollutants in Nam Co: OH production and source analysis C. Xing et al. 10.5194/acp-24-10093-2024
- Machine learning revealing key factors influencing HONO chemistry in Beijing during heating and non-heating periods W. Zhang et al. 10.1016/j.atmosres.2023.107130
- Aerosol Promotes Peroxyacetyl Nitrate Formation During Winter in the North China Plain W. Xu et al. 10.1021/acs.est.0c08157
- Influence of ship direct emission on HONO sources in channel environment Y. Guo et al. 10.1016/j.atmosenv.2020.117819
- Unveiling the underestimated direct emissions of nitrous acid (HONO) Q. Zhang et al. 10.1073/pnas.2302048120
- Origins of atmospheric nitrous acid and their contributions to OH radical from ship plumes, marine atmosphere, and continental air masses over South China Sea X. Ni et al. 10.1016/j.scitotenv.2024.175841
- Investigating the sources of atmospheric nitrous acid (HONO) in the megacity of Beijing, China R. Gu et al. 10.1016/j.scitotenv.2021.152270
- Exploring the HONO source during the COVID-19 pandemic in a megacity in China M. Wang et al. 10.1016/j.jes.2023.12.021
- A new insight into the vertical differences in NO2 heterogeneous reaction to produce HONO over inland and marginal seas C. Xing et al. 10.5194/acp-23-5815-2023
- Exploration of the atmospheric chemistry of nitrous acid in a coastal city of southeastern China: results from measurements across four seasons B. Hu et al. 10.5194/acp-22-371-2022
- Effect of Different Combustion Processes on Atmospheric Nitrous Acid Formation Mechanisms: A Winter Comparative Observation in Urban, Suburban and Rural Areas of the North China Plain W. Zhang et al. 10.1021/acs.est.1c07784
- Observations of HONO and its precursors between urban and its surrounding agricultural fields: The vertical transports, sources and contribution to OH C. Xing et al. 10.1016/j.scitotenv.2023.169159
- Seasonality of nitrous acid near an industry zone in the Yangtze River Delta region of China: Formation mechanisms and contribution to the atmospheric oxidation capacity Y. Ge et al. 10.1016/j.atmosenv.2021.118420
- Formation of condensable organic vapors from anthropogenic and biogenic volatile organic compounds (VOCs) is strongly perturbed by NO<sub><i>x</i></sub> in eastern China Y. Liu et al. 10.5194/acp-21-14789-2021
- The impacts of marine-emitted halogens on OH radicals in East Asia during summer S. Fan & Y. Li 10.5194/acp-22-7331-2022
- Long-term winter observation of nitrous acid in the urban area of Beijing C. Lian et al. 10.1016/j.jes.2021.09.010
- An investigation into the chemistry of HONO in the marine boundary layer at Tudor Hill Marine Atmospheric Observatory in Bermuda Y. Zhu et al. 10.5194/acp-22-6327-2022
- Elucidating HONO formation mechanism and its essential contribution to OH during haze events X. Zhang et al. 10.1038/s41612-023-00371-w
Latest update: 08 Dec 2024
Short summary
We conducted 1-year continuous measurement of HONO at the SORPES station. We obtained seasonal and diurnal variations of HONO and evaluated the contribution of HONO photolysis to OH radical and the missing daytime source of HONO. We separated the sources of nocturnal HONO into four parts: combustion emissions, soil emission, formation on ground and formation on aerosol, and estimate their contribution semi-quantitatively. The results highlighted ever-changing contributions of HONO sources.
We conducted 1-year continuous measurement of HONO at the SORPES station. We obtained seasonal...
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