Articles | Volume 19, issue 19
https://doi.org/10.5194/acp-19-12163-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-12163-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
01 Oct 2019
Research article |
| 01 Oct 2019
| 01 Oct 2019
Interactions between aerosol organic components and liquid water content during haze episodes in Beijing
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China
Shaojie Song
School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts 02138, USA
Wei Zhou
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China
Jiming Hao
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China
Douglas R. Worsnop
Institute for Atmospheric and Earth System Research/Physics, Faculty of Science, University of Helsinki, Helsinki, Finland
Aerodyne Research Inc., Billerica, Massachusetts 01821, USA
Jingkun Jiang
State Key Joint Laboratory of Environment Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing, 100084, China
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- Resolving Atmospheric Oxygenated Organic Molecules in Urban Beijing Using Online Ultrahigh-Resolution Chemical Ionization Mass Spectrometry Y. Yuan et al. 10.1021/acs.est.4c04214
- Estimation of interannual trends of ammonia emissions from agriculture in Jiangsu Province from 2000 to 2017 J. HUANG et al. 10.1080/16742834.2020.1736499
- In-situ measurement of secondary aerosol formation potential using a flow reactor: Livestock agricultural area F. Ashraf et al. 10.1016/j.atmosenv.2023.119695
- Hygroscopic behavior of aerosols generated from solutions of 3-methyl-1,2,3-butanetricarboxylic acid, its sodium salts, and its mixtures with NaCl L. Wu et al. 10.5194/acp-20-14103-2020
- Effects of simulated secondary organic aerosol water on PM1 levels and composition over the US S. Kakavas et al. 10.5194/acp-23-13555-2023
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- Distinct diurnal variation in organic aerosol hygroscopicity and its relationship with oxygenated organic aerosol Y. Kuang et al. 10.5194/acp-20-865-2020
- Multiphase Reactions between Organic Peroxides and Sulfur Dioxide in Internally Mixed Inorganic and Organic Particles: Key Roles of Particle Phase Separation and Acidity M. Yao et al. 10.1021/acs.est.3c04975
- Aerosol Hygroscopicity on A Single Particle Level Using Microscopic and Spectroscopic Techniques: A Review L. Wu & C. Ro 10.5572/ajae.2020.14.3.177
- Current Challenges in Visibility Improvement in Southern China W. Xu et al. 10.1021/acs.estlett.0c00274
- On the nature of sea salt aerosol at a coastal megacity: Insights from Manila, Philippines in Southeast Asia M. AzadiAghdam et al. 10.1016/j.atmosenv.2019.116922
- Direct Measurement of Aerosol Liquid Water Content: A Case Study in Summer in Nanjing, China D. Li et al. 10.3390/toxics12030164
- Aerosol liquid water content of PM2.5 and its influencing factors in Beijing, China J. Su et al. 10.1016/j.scitotenv.2022.156342
- Exploring wintertime regional haze in northeast China: role of coal and biomass burning J. Zhang et al. 10.5194/acp-20-5355-2020
- Effects of volatile organic compounds and new particle formation on real-time hygroscopicity of PM2.5 particles in Seosan, Republic of Korea J. Kim et al. 10.1016/j.scitotenv.2024.171516
- Exploring controls on perfluorocarboxylic acid (PFCA) gas–particle partitioning using a model with observational constraints Y. Tao et al. 10.1039/D2EM00261B
- Aerosol liquid water in PM2.5 and its roles in secondary aerosol formation at a regional site of Yangtze River Delta R. Shi et al. 10.1016/j.jes.2023.04.030
- Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China J. Li et al. 10.5194/acp-20-7291-2020
- High aerosol loading decreases the transpiration of poplars both in the day- and night-time B. Wang et al. 10.1016/j.agrformet.2022.109225
- Insight into wet scavenging effects on sulfur and nitrogen containing organic compounds in urban Beijing C. Zhang et al. 10.1038/s41612-024-00756-5
- Contrasting effects of secondary organic aerosol formations on organic aerosol hygroscopicity Y. Kuang et al. 10.5194/acp-21-10375-2021
- Particle phase state and aerosol liquid water greatly impact secondary aerosol formation: insights into phase transition and its role in haze events X. Meng et al. 10.5194/acp-24-2399-2024
- Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China D. Shang et al. 10.1007/s11783-020-1326-x
- Tropospheric aerosol hygroscopicity in China C. Peng et al. 10.5194/acp-20-13877-2020
- Molecular tracers, mass spectral tracers and oxidation of organic aerosols emitted from cooking and fossil fuel burning sources C. Liang et al. 10.1016/j.scitotenv.2023.161635
- Exploring the inorganic and organic nitrate aerosol formation regimes at a suburban site on the North China Plain W. Huang et al. 10.1016/j.scitotenv.2020.144538
- Mist cannon trucks can exacerbate the formation of water-soluble organic aerosol and PM2.5 pollution in the road environment Y. Xu et al. 10.5194/acp-23-6775-2023
- Spatial Inhomogeneity of New Particle Formation in the Urban and Mountainous Atmospheres of the North China Plain during the 2022 Winter Olympics D. Shang et al. 10.3390/atmos14091395
- A Review on Laboratory Studies and Field Measurements of Atmospheric Organic Aerosol Hygroscopicity and Its Parameterization Based on Oxidation Levels Y. Kuang et al. 10.1007/s40726-020-00164-2
28 citations as recorded by crossref.
- Resolving Atmospheric Oxygenated Organic Molecules in Urban Beijing Using Online Ultrahigh-Resolution Chemical Ionization Mass Spectrometry Y. Yuan et al. 10.1021/acs.est.4c04214
- Estimation of interannual trends of ammonia emissions from agriculture in Jiangsu Province from 2000 to 2017 J. HUANG et al. 10.1080/16742834.2020.1736499
- In-situ measurement of secondary aerosol formation potential using a flow reactor: Livestock agricultural area F. Ashraf et al. 10.1016/j.atmosenv.2023.119695
- Hygroscopic behavior of aerosols generated from solutions of 3-methyl-1,2,3-butanetricarboxylic acid, its sodium salts, and its mixtures with NaCl L. Wu et al. 10.5194/acp-20-14103-2020
- Effects of simulated secondary organic aerosol water on PM1 levels and composition over the US S. Kakavas et al. 10.5194/acp-23-13555-2023
- Hygroscopic growth and activation changed submicron aerosol composition and properties in the North China Plain W. Xu et al. 10.5194/acp-24-9387-2024
- Distinct diurnal variation in organic aerosol hygroscopicity and its relationship with oxygenated organic aerosol Y. Kuang et al. 10.5194/acp-20-865-2020
- Multiphase Reactions between Organic Peroxides and Sulfur Dioxide in Internally Mixed Inorganic and Organic Particles: Key Roles of Particle Phase Separation and Acidity M. Yao et al. 10.1021/acs.est.3c04975
- Aerosol Hygroscopicity on A Single Particle Level Using Microscopic and Spectroscopic Techniques: A Review L. Wu & C. Ro 10.5572/ajae.2020.14.3.177
- Current Challenges in Visibility Improvement in Southern China W. Xu et al. 10.1021/acs.estlett.0c00274
- On the nature of sea salt aerosol at a coastal megacity: Insights from Manila, Philippines in Southeast Asia M. AzadiAghdam et al. 10.1016/j.atmosenv.2019.116922
- Direct Measurement of Aerosol Liquid Water Content: A Case Study in Summer in Nanjing, China D. Li et al. 10.3390/toxics12030164
- Aerosol liquid water content of PM2.5 and its influencing factors in Beijing, China J. Su et al. 10.1016/j.scitotenv.2022.156342
- Exploring wintertime regional haze in northeast China: role of coal and biomass burning J. Zhang et al. 10.5194/acp-20-5355-2020
- Effects of volatile organic compounds and new particle formation on real-time hygroscopicity of PM2.5 particles in Seosan, Republic of Korea J. Kim et al. 10.1016/j.scitotenv.2024.171516
- Exploring controls on perfluorocarboxylic acid (PFCA) gas–particle partitioning using a model with observational constraints Y. Tao et al. 10.1039/D2EM00261B
- Aerosol liquid water in PM2.5 and its roles in secondary aerosol formation at a regional site of Yangtze River Delta R. Shi et al. 10.1016/j.jes.2023.04.030
- Impacts of water partitioning and polarity of organic compounds on secondary organic aerosol over eastern China J. Li et al. 10.5194/acp-20-7291-2020
- High aerosol loading decreases the transpiration of poplars both in the day- and night-time B. Wang et al. 10.1016/j.agrformet.2022.109225
- Insight into wet scavenging effects on sulfur and nitrogen containing organic compounds in urban Beijing C. Zhang et al. 10.1038/s41612-024-00756-5
- Contrasting effects of secondary organic aerosol formations on organic aerosol hygroscopicity Y. Kuang et al. 10.5194/acp-21-10375-2021
- Particle phase state and aerosol liquid water greatly impact secondary aerosol formation: insights into phase transition and its role in haze events X. Meng et al. 10.5194/acp-24-2399-2024
- Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China D. Shang et al. 10.1007/s11783-020-1326-x
- Tropospheric aerosol hygroscopicity in China C. Peng et al. 10.5194/acp-20-13877-2020
- Molecular tracers, mass spectral tracers and oxidation of organic aerosols emitted from cooking and fossil fuel burning sources C. Liang et al. 10.1016/j.scitotenv.2023.161635
- Exploring the inorganic and organic nitrate aerosol formation regimes at a suburban site on the North China Plain W. Huang et al. 10.1016/j.scitotenv.2020.144538
- Mist cannon trucks can exacerbate the formation of water-soluble organic aerosol and PM2.5 pollution in the road environment Y. Xu et al. 10.5194/acp-23-6775-2023
- Spatial Inhomogeneity of New Particle Formation in the Urban and Mountainous Atmospheres of the North China Plain during the 2022 Winter Olympics D. Shang et al. 10.3390/atmos14091395
Latest update: 20 Nov 2024
Short summary
Aerosol liquid water is ubiquitous in ambient aerosol. Using long-term aerosol chemical composition to model the aerosol water in Beijing, we found that water absorbed by organics contributes a significant fraction to the total aerosol water. We emphasize the hygroscopicity of organics is highly variable and should be taken into consideration in modelling. A positive feedback loop between organic hygroscopicity and aerosol water was found as one of the driving factors of severe haze in Beijing.
Aerosol liquid water is ubiquitous in ambient aerosol. Using long-term aerosol chemical...
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